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Discussion papers | Copyright
https://doi.org/10.5194/acp-2018-858
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 08 Oct 2018

Research article | 08 Oct 2018

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This discussion paper is a preprint. It is a manuscript under review for the journal Atmospheric Chemistry and Physics (ACP).

Development of a unit-based industrial emission inventory in the Beijing-Tianjin-Hebei region and resulting improvement in air quality modeling

Haotian Zheng1,*, Siyi Cai1,*, Shuxiao Wang1, Bin Zhao2, Xing Chang1, and Jiming Hao1 Haotian Zheng et al.
  • 1School of Environment and State Key Joint Laboratory of Environment Simulation and Pollution Control, Tsinghua University, Beijing 100084, China
  • 2Joint Institute for Regional Earth System Science and Engineering and Department of Atmospheric and Oceanic Sciences, University of California, Los Angeles, CA 90095, USA
  • *These authors contributed equally to this study.

Abstract. The Beijing-Tianjin-Hebei (BTH) region is a metropolitan area with the most severe fine particle (PM2.5) pollution in China. Accurate emission inventory plays an important role in air pollution control policy making. In this study, we develop a unit-based emission inventory for industrial sectors in the BTH region, including power plants, industrial boilers, and steel, non-ferrous metal, coking, cement, glass, brick, lime, ceramics, refinery, and chemical industries, based on detailed information for each enterprise, such as location, annual production, production technology/process and air pollution control facilities. In the BTH region, the emissions of sulfur dioxide (SO2), nitrogen oxide (NOx), particulate matter with diameter less than 10μm (PM10), PM2.5, black carbon (BC), organic carbon (OC), and non-methane volatile organic compounds (NMVOCs) from industrial sectors are 869kt, 1164kt, 910kt, 622kt, 71kt, 63kt and 1390kt in 2014, respectively, accounting for 61%, 55%, 62%, 56%, 58%, 22% and 36%, respectively, of the total emissions. Compared with the traditional proxy-based emission inventory, much less emissions in the high-resolution unit-based inventory are allocated to the urban center because of the accurate positioning of industrial enterprises. We apply the Community Multi-scale Air Quality (CMAQ) model simulation to evaluate the unit-based inventory. The simulation results show that the unit-based emission inventory gives better performance of both PM2.5 and gaseous pollutants than the proxy-based emission inventory. The normalized mean biases (NMBs) are 81%, 21%, 1% and −7% for concentrations of SO2, NO2, ozone and PM2.5, respectively, with the unit-based inventory, in contrast to 124%, 39%, −8% and 9% with the proxy-based inventory. Furthermore, the concentration gradients of PM2.5, which are defined as the ratio of urban concentration to suburban concentration, are 1.6, 2.1 and 1.5 in January and 1.3, 1.5 and 1.3 in July, for simulations with the unit-based inventory, simulations with the proxy-based inventory, and observations, respectively, in Beijing. For ozone, the corresponding gradients are 0.7, 0.5 and 0.9 in January and 0.9, 0.8 and 1.1 in July, implying that the unit-based emission inventory better reproduces the distributions of pollutant emissions between the urban and suburban areas.

Haotian Zheng et al.
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