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Discussion papers
https://doi.org/10.5194/acp-2018-620
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-2018-620
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 18 Sep 2018

Research article | 18 Sep 2018

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This discussion paper is a preprint. It is a manuscript under review for the journal Atmospheric Chemistry and Physics (ACP).

Drivers of variations in the vertical profile of ozone over Summit Station, Greenland: An analysis of ozonesonde data

Shima Bahramvash Shams1, Von P. Walden1, Samuel Oltmans2, Irina Petropavlovskikh2, Bryan Johnson2, Patrick Cullis2, Chance W. Sterling2, Laura Thölix3, Quentin Errera4, and Rigel Kivi5 Shima Bahramvash Shams et al.
  • 1Laboratory of Atmospheric Research, Department of Civil and Environmental Engineering, Washington State University, Pullman, Washington, USA
  • 2National Oceanic and Atmospheric Administration, Global Monitoring Division, Boulder, Colorado, USA
  • 3Climate Research, Finnish Meteorological Institute (FMI), Helsinki, Finland
  • 4Belgian Institute for Space Aeronomy, Uccle, Belgium
  • 5Space and Earth Observation Centre, Finnish Meteorological Institute, Sodankylä, Finland

Abstract. Understanding the drivers of atmospheric ozone variations in the Arctic is difficult because there are few long-term records of vertical ozone profiles in this region. We present 12 years of ozone profiles over Summit Station, Greenland (72.6 N, 38.4 W; 3200 meters) that were measured from 2005 to 2016. These profiles are subjected to data screening and are extended to 60km using a robust extrapolation method. The total column ozone and the partial column ozone in four atmospheric layers (troposphere to upper stratosphere) are analyzed. The monthly mean total column ozone reaches a maximum of about 400DU in April, then decreases to minimum values between 275 and 300DU in the late summer and early fall. The partial column ozone values peak at different times between late winter and early summer. There is a positive trend in the total column that is likely due to increases in springtime ozone, however, these trends are not robust given the short period of record. A stepwise multiple regression analysis is performed to determine the primary drivers of ozone variations over Summit Station. This analysis shows that the variations in total column ozone are due primarily to changes in the tropopause pressure, the quasi-biennial oscillation (QBO), and the volume of polar stratospheric clouds. The eddy heat flux is also important for variations in the partial column ozone in the different altitude regions. The importance of the QBO appears to be a unique characteristic for ozone variations over the Greenland Ice Sheet (when compared to other nearby Arctic Stations) and may be related to the fact that Greenland is particularly sensitive to the phase of the QBO.

Shima Bahramvash Shams et al.
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Shima Bahramvash Shams et al.
Shima Bahramvash Shams et al.
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Short summary
The Arctic plays a very important role in the global ozone cycle. We use direct measurements of the vertical profile of ozone from 2005 to 2016 to create a climatology of ozone over one of the most remote regions of the Arctic: Summit Station, Greenland. The trends in ozone at different altitudes are investigated to understand the Arctic ozone cycle. We develop a mathematical model to understand how ozone fluctuations can be explained by various parameters.
The Arctic plays a very important role in the global ozone cycle. We use direct measurements of...
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