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Discussion papers
https://doi.org/10.5194/acp-2018-1109
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-2018-1109
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 20 Dec 2018

Research article | 20 Dec 2018

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This discussion paper is a preprint. It is a manuscript under review for the journal Atmospheric Chemistry and Physics (ACP).

Vertical and horizontal distribution of sub-micron aerosol chemical composition and physical characteristics across Northern India, during the pre-monsoon and monsoon seasons

James Brooks1, James D. Allan1,2, Paul I. Williams1,2, Dantong Liu3, Cathryn Fox4, Jim Haywood4,5, Justin M. Langridge4, Ellie J. Highwood6, Sobhan K. Kompalli7, Debbie O'Sullivan4, Suresh S. Babu7, Sreedharan K. Satheesh8, Andrew G. Turner3,6, and Hugh Coe1 James Brooks et al.
  • 1Centre for Atmospheric Science, School of Earth and Environmental Sciences, University of Manchester, Manchester, UK
  • 2National Centre for Atmospheric Science, UK
  • 3School of Earth Sciences, Zhejiang University, China
  • 4Observation Based Research, Met Office, Exeter, UK
  • 5College of Engineering, Mathematics & Physical Sciences, Exeter, UK
  • 6Department of Meteorology, University of Reading, UK
  • 7Space Physics Laboratory, Vikram Sarabhai Space Centre, India
  • 8Centre for Atmospheric & Oceanic Sciences, Indian Institute of Science, India

Abstract. The vertical distribution in the physical and chemical properties of submicron aerosol has been characterised across northern India for the first time using airborne in-situ measurements. This study focusses primarily on the Indo-Gangetic Plain, a low-lying area in the north of India which commonly experiences high aerosol mass concentrations prior to the monsoon season. Data presented are from the UK Facility for Airborne Atmospheric Measurements BAe-146 research aircraft that performed flights in the region during the 2016 pre-monsoon (11th and 12th June) and monsoon (30th June to 11th July) seasons.

Inside the Indo-Gangetic Plain boundary layer, organic matter dominated the submicron aerosol mass (43%) followed by sulphate (29%), ammonium (14%), nitrate (7%) and black carbon (7%). However, outside the Indo-Gangetic Plain, sulphate was the dominant species contributing 44% to the total submicron aerosol mass in the boundary layer, followed by organic matter (30%), ammonium (14%), nitrate (6%) and black carbon (6%). Chlorine mass concentrations were negligible throughout the campaign. Black carbon mass concentrations were higher inside the Indo-Gangetic Plain (2µg/m3 std) compared to outside (1µg/m3 std). Nitrate appeared to be controlled by thermodynamic processes, with increased mass concentration in conditions of lower temperature and higher relative humidity. Increased mass and number concentrations were observed inside the Indo-Gangetic Plain and the aerosol was more absorbing in this region, whereas outside the Indo-Gangetic Plain the aerosol was larger in size and more scattering in nature, suggesting greater dust presence especially in northwest India. The aerosol composition remained largely similar as the monsoon season progressed, but the total aerosol mass concentrations decreased by ~50% as the rainfall arrived; the pre-monsoon average total mass concentration was 30µg/m3 std compared to a monsoon average total mass concentration of 10–20µg/m3 std. However, this mass concentration decrease was less noteworthy (~20–30%) over the Indo-Gangetic Plain, likely due to the strength of emission sources in this region. Decreases occurred in coarse mode aerosol, with the fine mode fraction increasing with monsoon arrival. In the aerosol vertical profile, inside the Indo-Gangetic Plain during the pre-monsoon, organic aerosol and absorbing aerosol species dominated in the lower atmosphere (<1.5km) with sulphate, dust and other scattering aerosol species enhanced in an elevated aerosol layer above 1.5km with maximum aerosol height ~6km. As the monsoon progressed into this region, the elevated aerosol layer diminished, the aerosol maximum height reduced to ~2km and the total mass concentrations decreased by ~50%. The dust and sulphate-dominated aerosol layer aloft was removed upon monsoon arrival, highlighted by an increase in fine mode fraction throughout the profile.

James Brooks et al.
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Our study, for the first time, presents measurements of aerosol chemical composition and physical characteristics across northern India in the pre-monsoon and monsoon seasons of 2016 using the FAAM BAe-146 UK research aircraft. Across northern India, an elevated aerosol layer dominated by sulphate aerosol exists that diminishes with monsoon arrival. The Indo-Gangetic Plain (IGP) boundary layer is dominated by organics, whereas outside the IGP sulphate dominates with increased scattering aerosol.
Our study, for the first time, presents measurements of aerosol chemical composition and...
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