Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.
Research article
23 Nov 2017
Review status
This discussion paper is a preprint. It is a manuscript under review for the journal Atmospheric Chemistry and Physics (ACP).
Decrease in tropospheric O3 levels of the Northern Hemisphere observed by IASI
Catherine Wespes1, Daniel Hurtmans1, Cathy Clerbaux1,2, Anne Boynard2, and Pierre-François Coheur1 1Spectroscopie de l'Atmosphère, Service de Chimie Quantique et Photophysique, Faculté des Sciences, Université Libre de Bruxelles (ULB), Brux elles, Belgique
2LATMOS/IPSL, UPMC Univ. Paris 06 Sorbonne Universités, UVSQ, CNRS, Paris, France
Abstract. In this study, we describe the recent changes in the tropospheric ozone (O3) columns (TOCs) measured by the Infrared Atmospheric Sounding Interferometer (IASI) onboard the Metop satellite during the first 9 years of the IASI operation (January 2008 to May 2017). Using appropriate multivariate regression methods, we discriminate significant linear trends from other sources of O3 variations captured by IASI. The geographical patterns of the adjusted O3 trends are provided and discussed on the global scale. Given the large contribution of the natural variability in comparison with that of the trend (25–85 % vs 15–50 %, respectively) to the total O3 variations, we estimate that additional years of IASI measurements are generally required to detect the estimated O3 trends with a high precision. Globally, additional 6 months to 6 years of measurements, depending on the regions and the seasons, are needed to detect a trend of  |5| DU/decade. An exception is interestingly found during summer in the mid-high latitudes of the North Hemisphere (N.H.; ~ 40° N–75° N) where the large absolute fitted trend values (~ |0.5| DU/yr on average) combined with the small model residuals (~ 10 %) allow the detection of a band-like pattern of significant negative trends. This finding supports the reported decrease in O3 precursor emissions in recent years, especially in Europe and US. The influence of continental pollution on that latitudinal band is further investigated and supported by the analysis of the O3–CO relationship (in terms of correlation coefficient, regression slope and covariance) that we found to be the strongest at the northern mid-latitudes in summer.

Citation: Wespes, C., Hurtmans, D., Clerbaux, C., Boynard, A., and Coheur, P.-F.: Decrease in tropospheric O3 levels of the Northern Hemisphere observed by IASI, Atmos. Chem. Phys. Discuss.,, in review, 2017.
Catherine Wespes et al.
Catherine Wespes et al.
Catherine Wespes et al.


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