Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
https://doi.org/10.5194/acp-2017-745
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.
Research article
30 Aug 2017
Review status
This discussion paper is a preprint. It is a manuscript under review for the journal Atmospheric Chemistry and Physics (ACP).
Measurements of aerosol and CCN properties in the Mackenzie River delta (Canadian Arctic) during Spring-Summer transition in May 2014
Paul Herenz1, Heike Wex1, Silvia Henning1, Thomas Bjerring Kristensen1,a, Florian Rubach2, Anja Roth2, Stephan Borrmann2, Heiko Bozem3, Hannes Schulz4, and Frank Stratmann1 1Leibniz Institute for Tropospheric Research, Leipzig, Germany
2Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
3Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
4Alfred Wegener Institute, Helmholtz Center for Polar and Marine Research, Bremerhaven, Germany
anow at: Division of Nuclear Physics, Lund University, Box 118, Lund 22100, Sweden
Abstract. Within the framework of the RACEPAC (Radiation-Aerosol-Cloud Experiment in the Arctic Circle) project, the Arctic aerosol, arriving at a ground based station in Tuktoyaktuk (Mackenzie River delta area, Canada), was characterized during a period of 3 weeks in May 2014. The observations of basic meteorological parameters and particle number size distributions (PNSDs) were indicative for the rapid transition from Arctic spring to summer that took place during the measurement period. Two distinct types of air masses were found. One type were typical Arctic haze air masses, termed as spring-type air masses, characterized by a mono-modal PNSD with a pronounced accumulation mode at sizes above 100 nm. These air masses were observed during a period when back trajectories indicate an air mass origin in the north east of Canada. The other air mass type is characterized by a bi-modal PNSD with a clear minimum around 90 nm, and with an Aitken mode consisting of freshly formed aerosol particles. Back trajectories indicate that these air masses, termed as summer-type air masses, originated from the northern Pacific. Generally total particle number concentrations (NCN) ranged from 20 to 500 cm−3, while cloud condensation nuclei (CCN) number concentrations were found to cover a range between less than 10 up to 250 cm−3 for a supersaturation (SS) between 0.1 and 0.7 %. The hygroscopicity parameter κ of the CCN was determined to be 0.23 on average and variations in kappa were largely attributed to measurement uncertainties.

Furthermore, simultaneous PNSD measurements at the ground station and on the Polar 6 research aircraft were performed. We found a good agreement of ground based PNSDs with those measured between 200 and 1200 m. During two of the four overflights, particle number concentrations at 3000 m were found to be up to twenty times higher than those measured below 2000 m, and for one of these two flights, PNSDs measured above 2000 m showed a different shape than those measured at lower altitudes. This is indicative for long range transport from lower latitudes into the Arctic that can advect aerosol from different regions in different heights.


Citation: Herenz, P., Wex, H., Henning, S., Kristensen, T. B., Rubach, F., Roth, A., Borrmann, S., Bozem, H., Schulz, H., and Stratmann, F.: Measurements of aerosol and CCN properties in the Mackenzie River delta (Canadian Arctic) during Spring-Summer transition in May 2014, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-745, in review, 2017.
Paul Herenz et al.
Paul Herenz et al.
Paul Herenz et al.

Viewed

Total article views: 294 (including HTML, PDF, and XML)

HTML PDF XML Total BibTeX EndNote
218 70 6 294 5 8

Views and downloads (calculated since 30 Aug 2017)

Cumulative views and downloads (calculated since 30 Aug 2017)

Viewed (geographical distribution)

Total article views: 294 (including HTML, PDF, and XML)

Thereof 290 with geography defined and 4 with unknown origin.

Country # Views %
  • 1

Saved

Discussed

Latest update: 19 Nov 2017
Publications Copernicus
Download
Short summary
The Arctic climate is changing much faster than other regions on Earth. Hence, it is necessary to investigate the processes that are able for this phenomena and to document the current situation in the Arctic. Therefore, we measured the number and also the size of aerosol particles. It turned out that we captured the transition from the Arctic spring to the Arctic summer and that the according air masses show differences in particle properties. Also, the particles have a low water receptivity.
The Arctic climate is changing much faster than other regions on Earth. Hence, it is necessary...
Share