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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
doi:10.5194/acp-2016-922
© Author(s) 2016. This work is distributed
under the Creative Commons Attribution 3.0 License.
Research article
29 Nov 2016
Review status
This discussion paper is under review for the journal Atmospheric Chemistry and Physics (ACP).
The impact of fluctuations and correlations in droplet growth by collision-coalescence revisited. Part I: Numerical calculation of post-gel droplet size distribution
Lester Alfonso1 and Graciela B. Raga2 1Universidad Autónoma de la Ciudad de México, México City, 09790 México
2Centro de Ciencias de la Atmósfera, UNAM, México City, 04510 México
Abstract. The impact of stochastic fluctuations in cloud droplet growth is a matter of broad interest, since stochastic effects are one of the possible explanations of how cloud droplets cross the size-gap and form the raindrop embryos that trigger warm rain development in cumulus clouds. Most theoretical studies in this topic rely on the use of the kinetic collection equation, or the stochastic simulation algorithm (Gillespie 1975). However, the kinetic collection equation is a deterministic equation with no stochastic fluctuations. Moreover, the traditional calculations using the kinetic collection equation are not valid when the system undergoes a transition from a continuous distribution to a distribution plus a runaway raindrop embryo (known as the sol-gel transition). On the other hand, the stochastic simulation algorithm, although intrinsically stochastic, fails to reproduce adequately the large end of the droplet size distribution due to the huge number of realizations required. Therefore, the full stochastic description of cloud droplet growth must be obtained from the solution of the master equation for stochastic coalescence.

In this study the master equation is used to calculate the evolution of the droplet size distribution after the sol-gel transition. These calculations show that after the formation of the raindrop embryo, the expected droplet mass distribution strongly differs from the results obtained with the kinetic collection equation. Furthermore, the low mass bins and bins from the gel fraction are strongly anti-correlated in the vicinity of the critical time, this being one of the possible explanations for the differences between the kinetic and stochastic approaches after the sol-gel transition. Calculations performed within the stochastic framework provide insight into the inability of explicit microphysics cloud models to explain the droplet spectral broadening observed in small, warm clouds.


Citation: Alfonso, L. and Raga, G. B.: The impact of fluctuations and correlations in droplet growth by collision-coalescence revisited. Part I: Numerical calculation of post-gel droplet size distribution, Atmos. Chem. Phys. Discuss., doi:10.5194/acp-2016-922, in review, 2016.
Lester Alfonso and Graciela B. Raga
Lester Alfonso and Graciela B. Raga
Lester Alfonso and Graciela B. Raga

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The main hypothesis of this work is that the discrepancy between the observations and the theoretical models of precipitation formation in warm clouds, could be explained by the formation of embryo droplets in the context of a sol-gel transition. By using novel numerical techniques, our calculations show that after the formation of the raindrop embryo, the droplet mass distribution strongly differs from the results obtained by using the traditional approaches.
The main hypothesis of this work is that the discrepancy between the observations and the...
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