Atmos. Chem. Phys. Discuss., 9, 6855-6887, 2009
www.atmos-chem-phys-discuss.net/9/6855/2009/
doi:10.5194/acpd-9-6855-2009
© Author(s) 2009. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
A new insight on tropospheric methane in the Tropics – first year from IASI hyperspectral infrared observations
C. Crevoisier1, D. Nobileau1, A. M. Fiore2, R. Armante1, A. Chédin1, and N. A. Scott1
1Laboratoire de Météorologie Dynamique/CNRS/IPSL, Ecole Polytechnique, Palaiseau, France
2Geophysical Fluid Dynamics Laboratory/NOAA, Princeton, New Jersey, USA

Abstract. Simultaneous observations from the Infrared Atmospheric Sounding Interferometer (IASI) and from the Advanced Microwave Sounding Unit (AMSU), launched together onboard the European MetOp platform in October 2006, are used to retrieve a mid-to-upper tropospheric content of methane (CH4) in clear-sky conditions, in the Tropics, over sea, for the first 16 months of operation of MetOp (July 2007–October 2008). With its very high spectral resolution, IASI provides nine channels in the 7.7 μm band highly sensitive to CH4 with reduced sensitivities to other atmospheric variables. These channels, sensitive to both CH4 and temperature, are used in conjunction with AMSU channels, only sensitive to temperature, to decorrelate both signals through a non-linear inference scheme based on neural networks. A key point of this approach is that no use is made of prior information in terms of methane seasonality, trend, or geographical patterns. The accuracy of the retrieval is estimated to be about 16 ppbv (~0.9%). Features of the retrieved methane space-time distribution include: (1) a strong seasonal cycle of 30 ppbv in the Northern Tropics with a maximum in January–March and a minimum in July–September, and a flat seasonal cycle in the Southern Tropics, in agreement with in-situ measurements; (2) a latitudinal decrease of 30 ppbv from 20° N to 20° S, in boreal spring and summer, lower than what is observed at the surface but in excellent agreement with tropospheric aircraft measurements; (3) geographical patterns in good agreement with simulations from the atmospheric transport and chemistry model MOZART-2, but with a higher variability and a higher concentration in boreal winter; (4) signatures of CH4 emissions transported to the middle troposphere such as a large plume of elevated tropospheric methane south of the Asian continent, which might be due to Asian emissions from rice paddies uplifted by deep convection during the monsoon period and then transported towards Indonesia. In addition to bringing a greatly improved view of methane distribution, these results from IASI should provide a means to observe and understand atmospheric transport pathways of methane from the surface to the upper troposphere.

Citation: Crevoisier, C., Nobileau, D., Fiore, A. M., Armante, R., Chédin, A., and Scott, N. A.: A new insight on tropospheric methane in the Tropics – first year from IASI hyperspectral infrared observations, Atmos. Chem. Phys. Discuss., 9, 6855-6887, doi:10.5194/acpd-9-6855-2009, 2009.
 
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