<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys-discuss.net/inc/acpd/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>9</volume_number>
		<issue_number>6</issue_number>
		<publication_year>2009</publication_year>
	</journal>
	<doi>10.5194/acpd-9-25275-2009</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/9/25275/2009/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/9/25275/2009/acpd-9-25275-2009.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/9/25275/2009/acpd-9-25275-2009.pdf</fulltext_pdf>
	<start_page>25275</start_page>
	<end_page>25321</end_page>
	<publication_date>2009-11-25</publication_date>
	<article_title content_type="html">Subseasonal variability of low cloud radiative properties over the southeast Pacific Ocean</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>R. C. George</name>
			<email>rheag@atmos.washington.edu</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>R. Wood</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">University of Washington, Seattle, Washington, USA</affiliation>
	</affiliations>
	<abstract content_type="html">Subseasonal variability of cloud radiative properties in the persistent
southeast Pacific stratocumulus deck is investigated using MODIS satellite
observations and NCEP reanalysis data. A once-daily albedo proxy is derived
based on the fractional coverage of low cloud (a macrophysical field) and
the cloud albedo, with the latter broken down into contributions from
microphysics (cloud droplet concentration) and macrophysics (liquid water
path). Subseasonal albedo variability is dominated by the contribution of
low cloud fraction variability, except within 10–15&amp;deg; of the South
American coast, where cloud albedo variability contributes significantly.
Covariance between cloud fraction and cloud albedo also contributes
significantly and positively to the variance in albedo, which highlights how
complex and inseparable the factors controlling albedo are. Droplet
concentration variability contributes only weakly to the subseasonal
variability of albedo, which emphasizes that attributing albedo variability
to the indirect effects of aerosols against the backdrop of natural
meteorological variability is extremely challenging.
&lt;br&gt;&lt;br&gt;
The dominant large scale meteorological variability is associated with the
subtropical high pressure system. Two indices representing changes in the
subtropical high strength and extent explain 80–90% of this variability,
and significantly modulate the cloud microphysical, macrophysical, and
radiative cloud properties. Variations in droplet concentration of up to
50% of the mean are associated with the meteorological driving. We
hypothesize that these fluctuations in droplet concentration are a result of
the large scale meteorology and their correlation with cloud macrophysical
properties should not be used as evidence of aerosol effects. Mechanisms by
which large scale meteorology affects cloud properties are explored. Our
results support existing hypotheses linking cloud cover variability to
changes in cold advection, subsidence, and lower tropospheric stability.
Within 10&amp;deg; of the coast interactions between variability in the surface
high pressure system and the orography appear to modulate both cloud
macrophysical properties and aerosol transport through suppression of the
marine boundary layer depth near the coast. This suggests one possible way
in which cloud macrophysical properties and droplet concentration may be
correlated independently of the second aerosol indirect effect. The results
provide variability constraints for models that strive to represent both
meteorological and aerosol impacts on stratocumulus clouds.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Ackerman, A. S., Kirkpatrick, M. P., Stevens, D. E., and Toon, O. B.: The impact of humidity above stratiform clouds on indirect aerosol climate forcing, Nature, 432, 1014–1017, doi:10.1038/nature03174, 2004. </reference>
		<reference numeration="2" content_type="text"> Albrecht, B. A.: Aerosols, cloud microphysics, and fractional cloudiness, Science, 245, 1227–1230, 1989. </reference>
		<reference numeration="3" content_type="text"> Bates, T. S., Lamb, B. K., Guenther, A., Dignon, J., and Stoiber, R. E.: Sulfur emissions to the atmosphere from natural sources, J. Atmos. Chem., 14, 315–337, 1992. </reference>
		<reference numeration="4" content_type="text"> Benkovitz, C. M., Scholtz, M. T., Pacyna, J., Tarrason, L., Dignon, J., Voldner, E. C., Spiro, P. A., Logan, J. A., and Graedel, T. E.: Global gridded inventories of anthropogenic emissions of sulfur and nitrogen, J. Geophys. Res.-Atmos., 101, 29239–29253, 1996. </reference>
		<reference numeration="5" content_type="text"> Bennartz, R. and Harshvardhan: Global assessment of marine boundary layer cloud droplet number concentration from satellite, J. Geophys. Res.-Atmos., 112, D02201, doi:10.1029/2007jd008841, 2007. </reference>
		<reference numeration="6" content_type="text"> Bony, S., Letreut, H., Duvel, J. P., and Kandel, R. S.: Satellite validation of GCM-simulated annual cycle of the earth radiation budget and cloud forcing, J. Geophys. Res.-Atmos., 97, 18061–18081, 1992. </reference>
		<reference numeration="7" content_type="text"> Brenguier, J. L., Pawlowska, H., and Schuller, L.: Cloud microphysical and radiative properties for parameterization and satellite monitoring of the indirect effect of aerosol on climate, J. Geophys. Res.-Atmos., 108(14), 8632, doi:10.1029/2002jd002682, 2003. </reference>
		<reference numeration="8" content_type="text"> Bretherton, C. S., Blossey, P. N., and Uchida, J.: Cloud droplet sedimentation, entrainment efficiency, and subtropical stratocumulus albedo, Geophys. Res. Lett., 34, L03813, doi:10.1029/2006gl027648, 2007. </reference>
		<reference numeration="9" content_type="text"> Bretherton, C. S. and Hartmann, D. L.: Large-scale controls on cloudiness, in: Clouds in the perturbed climate system: Their relationship to energy balance, atmospheric dynamics and precipitation, edited by: Heintzenberg, J. and Charleson, R. J., Strungmann forum reports, MIT Press, 217–234, 2009. </reference>
		<reference numeration="10" content_type="text"> Bretherton, C. S., Uttal, T., Fairall, C. W., Yuter, S. E., Weller, R. A., Baumgardner, D., Comstock, K., Wood, R., and Raga, G. B.: The EPIC 2001 stratocumulus study, B. Am. Meteor. Soc., 85, 976–977, doi:10.1175/bams-85-7-967, 2004. </reference>
		<reference numeration="11" content_type="text"> Bretherton, C. S., Widmann, M., Dymnikov, V. P., Wallace, J. M., and Blade, I.: The effective number of spatial degrees of freedom of a time-varying field, J. Climate, 12, 1990–2009, 1999. </reference>
		<reference numeration="12" content_type="text"> Cahalan, R. F., Ridgway, W., Wiscombe, W. J., Bell, T. L., and Snider, J. B.: The albedo of fractal stratocumulus clouds, J. Atmos. Sci., 51, 2434–2455, 1994. </reference>
		<reference numeration="13" content_type="text"> Caldwell, P., Bretherton, C. S., and Wood, R.: Mixed-layer budget analysis of the diurnal cycle of entrainment in southeast Pacific stratocumulus, J. Atmos. Sci., 62, 3775–3791, 2005. </reference>
		<reference numeration="14" content_type="text"> Cess, R. D.: Climate change – appraisal of atmospheric feedback mechanisms employing zonal climatology, J. Atmos. Sci., 33, 1831–1843, 1976. </reference>
		<reference numeration="15" content_type="text"> Garreaud, R. D. and Munoz, R. C.: The low-level jet off the west coast of subtropical South America: Structure and variability, Mon. Weather Rev., 133, 2246–2261, 2005. </reference>
		<reference numeration="16" content_type="text"> Garreaud, R. D., Rutllant, J., Quintana, J., Carrasco, J., and Minnis, P.: Cimar-5: A snapshot of the lower troposphere over the subtropical southeast Pacific, B. Am. Meteor. Soc., 82, 2193–2207, 2001. </reference>
		<reference numeration="17" content_type="text"> Garreaud, R. D. and Rutllant, J.: Coastal lows along the subtropical west coast of south america: Numerical simulation of a typical case, Mon. Wea. Rev., 131, 891–908, 2003. </reference>
		<reference numeration="18" content_type="text"> Han, Q. Y., Rossow, W. B., and Lacis, A. A.: Near-global survey of effective droplet radii in liquid water clouds using isccp data, J. Climate, 7, 465–497, 1994. </reference>
		<reference numeration="19" content_type="text"> Holton, J. R.: An introduction to dynamic meteorology, Third edition ed., Academic Press, San Diego, USA, 213–219, 1992. </reference>
		<reference numeration="20" content_type="text"> Huneeus, N., Gallardo, L., and Rutllant, J. A.: Offshore transport episodes of anthropogenic sulfur in northern Chile: Potential impact on the stratocumulus cloud deck, Geophys. Res. Lett., 33, L19819, doi:10.1029/2006gl026921, 2006. </reference>
		<reference numeration="21" content_type="text"> Kalnay, E., Kanamitsu, M., Kistler, R., Collins, W., Deaven, D., Gandin, L., Iredell, M., Saha, S., White, G., Woollen, J., Zhu, Y., Chelliah, M., Ebisuzaki, W., Higgins, W., Janowiak, J., Mo, K. C., Ropelewski, C., Wang, J., Leetmaa, A., Reynolds, R., Jenne, R., and Joseph, D.: The NCEP/NCAR 40-year reanalysis project, B. Am. Meteor. Soc., 77, 437–471, 1996. </reference>
		<reference numeration="22" content_type="text"> Kaufman, Y. J., Koren, I., Remer, L. A., Rosenfeld, D., and Rudich, Y.: The effect of smoke, dust, and pollution aerosol on shallow cloud development over the Atlantic ocean, Proc. Natl. Acad. Sci., 102, 11207–11212, doi:10.1073/pnas.0505191102, 2005. </reference>
		<reference numeration="23" content_type="text"> King, M. D. and Harshvardhan: Comparative accuracy of selected multiple-scattering approximations, J. Atmos. Sci., 43, 784–801, 1986. </reference>
		<reference numeration="24" content_type="text"> King, M. D., Tsay, S.-C., Platnick, S. E., Wang, M., and Liou, K.-N.: Cloud retrieval algorithms for MODIS: Optical thickness, effective particle radius, and thermodynamic phase, in, NASA, MODIS Algorithm Theoretical Basis Doc, 1997. </reference>
		<reference numeration="25" content_type="text"> Klein, S. A., Hartmann, D. L., and Norris, J. R.: On the relationships among low-cloud structure, sea-surface temperature, and atmospheric circulation in the summertime northeast Pacific, J. Climate, 8, 1140–1155, 1995. </reference>
		<reference numeration="26" content_type="text"> Klein, S. A. and Hartmann, D. L.: The seasonal cycle of low stratiform clouds, J. Climate, 6, 1587–1606, 1993. </reference>
		<reference numeration="27" content_type="text"> Klein, S. A.: Synoptic variability of low-cloud properties and meteorological parameters in the subtropical trade wind boundary layer, J. Climate, 10, 2018-2039, 1997. </reference>
		<reference numeration="28" content_type="text"> Lebsock, M. D., Stephens, G. L., and Kummerow, C.: Multisensor satellite observations of aerosol effects on warm clouds, J. Geophys. Res., 113, D15205, doi:10.1029/2008jd009876, 2008. </reference>
		<reference numeration="29" content_type="text"> Loeb, N. G., and Kato, S.: Top-of-atmosphere direct radiative effect of aerosols over the tropical oceans from the clouds and the earth&apos;s radiant energy system (CERES) satellite instrument, J. Climate, 15, 1474–1484, 2002. </reference>
		<reference numeration="30" content_type="text"> Lohmann, U. and Feichter, J.: Global indirect aerosol effects: A review, Atmos. Chem. and Phys., 5, 715–737, 2005. </reference>
		<reference numeration="31" content_type="text"> Martin, G. M., Johnson, D. W., and Spice, A.: The measurement and parameterization of effective radius of droplets in warm stratocumulus clouds, J. Atmos. Sci., 51, 1823–1842, 1994. </reference>
		<reference numeration="32" content_type="text"> Matheson, M. A., Coakley, J. A., and Tahnk, W. R.: Aerosol and cloud property relationships for summertime stratiform clouds in the northeastern Atlantic from advanced very high resolution radiometer observations, J. Geophys. Res.-Atmos., 110, D24204, doi:10.1029/2005jd006165, 2005. </reference>
		<reference numeration="33" content_type="text"> Mauger, G. S. and Norris, J. R.: Meteorological bias in satellite estimates of aerosol-cloud relationships, Geophys. Res. Lett., 34, L16824, doi:10.1029/2007gl029952, 2007. </reference>
		<reference numeration="34" content_type="text"> Norris, J. R. and Leovy, C. B.: Interannual variability in stratiform cloudiness and sea-surface temperature, J. Climate, 7, 1915–1925, 1994. </reference>
		<reference numeration="35" content_type="text"> North, G. R., Bell, T. L., Cahalan, R. F., and Moeng, F. J.: Sampling errors in the estimation of empirical orthogonal functions, Mon. Weather Rev., 110, 699–706, 1982. </reference>
		<reference numeration="36" content_type="text"> Platnick, S. and Twomey, S.: Determining the susceptibility of cloud albedo to changes in droplet concentration with the advanced very high-resolution radiometer, J. Appl. Meteorol., 33, 334–347, 1994. </reference>
		<reference numeration="37" content_type="text"> Quaas, J., Boucher, O., Bellouin, N., and Kinne, S.: Satellite-based estimate of the direct and indirect aerosol climate forcing, J. Geophys. Res.-Atmos., 113, D05204, doi:10.1029/2007jd008962, 2008. </reference>
		<reference numeration="38" content_type="text"> Richter, I. and Mechoso, C. R.: Orographic influences on the annual cycle of Namibian stratocumulus clouds, Geophys. Res. Lett., 31, L24108, doi10.1029/2004gl020814, 2004. </reference>
		<reference numeration="39" content_type="text"> Rozendaal, M. A., Leovy, C. B., and Klein, S. A.: An observational study of diurnal-variations of marine stratiform cloud, J. Climate, 8, 1795–1809, 1995. </reference>
		<reference numeration="40" content_type="text"> Rutllant, J. A. and Garreaud, R. D.: Episodes of strong flow down the western slope of the subtropical Andes, Mon. Weather Rev., 132, 611–622, 2004. </reference>
		<reference numeration="41" content_type="text"> Slingo, A. and Schrecker, H. M.: On the shortwave radiative properties of stratiform water clouds, Q. J. Roy. Meteor. Soc., 108, 407–426, 1982. </reference>
		<reference numeration="42" content_type="text"> Stevens, B. and Brenguier, J.-L.: Cloud controlling factors: Low clouds, in: Clouds in the perturbed climate system: Their relationship to energy balance, atmospheric dynamics and precipitation, edited by: Heintzenberg, J. and Charleson, R. J., Strungmann forum reports, MIT Press, 173–196, 2009. </reference>
		<reference numeration="43" content_type="text"> Szczodrak, M., Austin, P. H., and Krummel, P. B.: Variability of optical depth and effective radius in marine stratocumulus clouds, J. Atmos. Sci., 58, 2912–2926, 2001. </reference>
		<reference numeration="44" content_type="text"> Takahashi, K. and Battisti, D. S.: Processes controlling the mean tropical Pacific precipitation pattern. Part ii: The SPCZ and the southeast Pacific dry zone, J. Climate, 20, 5696–5706, doi:10.1175/2007jcli1656.1, 2007. </reference>
		<reference numeration="45" content_type="text"> Twohy, C. H., Petters, M. D., Snider, J. R., Stevens, B., Tahnk, W., Wetzel, M., Russell, L., and Burnet, F.: Evaluation of the aerosol indirect effect in marine stratocumulus clouds: Droplet number, size, liquid water path, and radiative impact, J. Geophys. Res.-Atmos., 110, D08203, doi:10.1029/2004jd005116, 2005. </reference>
		<reference numeration="46" content_type="text"> Twomey, S.: Pollution and planetary albedo, Atmos. Environ., 8, 1251–1256, 1974. </reference>
		<reference numeration="47" content_type="text"> Wang, S. P., Wang, Q., and Feingold, G.: Turbulence, condensation, and liquid water transport in numerically simulated nonprecipitating stratocumulus clouds, J. Atmos. Sci., 60, 262–278, 2003. </reference>
		<reference numeration="48" content_type="text"> Wood, R., Bretherton, C. S., and Hartmann, D. L.: Diurnal cycle of liquid water path over the subtropical and tropical oceans, Geophys. Res. Lett., 29, D08203, doi:10.1029/2002gl015371, 2002. </reference>
		<reference numeration="49" content_type="text"> Wood, R. and Bretherton, C. S.: Boundary layer depth, entrainment, and decoupling in the cloud-capped subtropical and tropical marine boundary layer, J. Climate, 17, 3576–3588, 2004. </reference>
		<reference numeration="50" content_type="text"> Wood, R. and Bretherton, C. S.: On the relationship between stratiform low cloud cover and lower-tropospheric stability, J. Climate, 19, 6425–6432, 2006. </reference>
		<reference numeration="51" content_type="text"> Wood, R., Comstock, K. K., Bretherton, C. S., Cornish, C., Tomlinson, J., Collins, D. R., and Fairall, C.: Open cellular structure in marine stratocumulus sheets, J. Geophys. Res.-Atmos., 113, D12207, doi:10.1029/2007jd009371, 2008. </reference>
		<reference numeration="52" content_type="text"> Wood, R. and Hartmann, D. L.: Spatial variability of liquid water path in marine low cloud: The importance of mesoscale cellular convection, J. Climate, 19, 1748–1764, 2006. </reference>
		<reference numeration="53" content_type="text"> Wood, R.: Cancellation of aerosol indirect effects in marine stratocumulus through cloud thinning, J. Atmos. Sci., 64, 2657–2669, doi:10.1175/jas3942.1, 2007. </reference>
		<reference numeration="54" content_type="text"> Xu, H. M., Xie, S. P., and Wang, Y. Q.: Subseasonal variability of the southeast Pacific stratus cloud deck, J. Climate, 18, 131–142, 2005. </reference>
		<reference numeration="55" content_type="text"> Xue, H. W. and Feingold, G.: Large-eddy simulations of trade wind cumuli: Investigation of aerosol indirect effects, J. Atmos. Sci., 63, 1605–1622, 2006. </reference>
		<reference numeration="56" content_type="text"> Zhang, M. H., Lin, W. Y., Klein, S. A., Bacmeister, J. T., Bony, S., Cederwall, R. T., Del Genio, A. D., Hack, J. J., Loeb, N. G., Lohmann, U., Minnis, P., Musat, I., Pincus, R., Stier, P., Suarez, M. J., Webb, M. J., Wu, J. B., Xie, S. C., Yao, M. S., and Zhang, J. H.: Comparing clouds and their seasonal variations in 10 atmospheric general circulation models with satellite measurements, J. Geophys. Res.-Atmos., 110, doi:10.1029/2004jd005021, 2005. </reference>
		<reference numeration="57" content_type="text"> Zhou, M. Y., Zeng, X. B., Brunke, M., Zhang, Z. H., and Fairall, C.: An analysis of statistical characteristics of stratus and stratocumulus over eastern Pacific, Geophys. Res. Lett., 33, L02807, doi:10.1029/2005gl024796, 2006. </reference>
		<reference numeration="58" content_type="text"> Zuidema, P., Painemal, D., de Szoeke, S., and Fairall, C.: Stratocumulus cloud-top height estimates and their climatic implications, J. Climate, 22, 4652–4666, doi:10.1175/2009jcli2708.1, 2009. </reference>
	</references>
</article>

