Atmos. Chem. Phys. Discuss., 9, 17429-17463, 2009
www.atmos-chem-phys-discuss.net/9/17429/2009/
doi:10.5194/acpd-9-17429-2009
© Author(s) 2009. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Regional N2O fluxes in Amazonia derived from aircraft vertical profiles
M. T. S. D'Amelio1, L. V. Gatti1, J. B. Miller2,3, and P. Tans2
1Instituto de Pesquisas Energéticas e Nucleares (IPEN), São Paulo, Brazil
2National Oceanic and Atmospheric Administration (NOAA), Colorado
3Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Colorado

Abstract. Nitrous oxide (N2O) is the third most important anthropogenic greenhouse gas. Globally, the main sources of N2O are nitrification and denitrification in soils. About two thirds of the soil emissions occur in the tropics and approximately 20% originate in wet rainforest ecosystems, like the Amazon forest. The work presented here involves aircraft vertical profiles of N2O from the surface to 4 km over two sites in the Eastern and Central Amazon: Tapajós National Forest (SAN) and Cuieiras Biologic Reserve (MAN), and the estimation of N2O fluxes for regions upwind of these sites. To our knowledge, these regional scale N2O measurements in Amazonia are unique and represent a new approach to looking regional scale emissions. The fluxes upwind of MAN exhibited little seasonality, and the annual mean was 2.1±1.0 mg N2O m−2 day−1, higher than that for fluxes upwind of SAN, which averaged 1.5±1.6 mg N2O m−2 day−1. The higher rainfall around the MAN site could explain the higher N2O emissions. For fluxes from the coast to SAN seasonality is present for all years, with high fluxes in the months of March through May, and in November through December. The first peak of N2O flux is strongly associated with the wet season. The second peak of high N2O flux recorded at SAN occurs during the dry season and can not be easily explained. However, about half of the dry season profiles exhibit significant correlations with CO, indicating a larger than expected source of N2O from biomass burning. The average CO:N2O ratio for all profiles sampled during the dry season is 94±77 mol CO:mol N2O and suggests a larger biomass burning contribution to the global N2O budget than previously reported.

Citation: D'Amelio, M. T. S., Gatti, L. V., Miller, J. B., and Tans, P.: Regional N2O fluxes in Amazonia derived from aircraft vertical profiles, Atmos. Chem. Phys. Discuss., 9, 17429-17463, doi:10.5194/acpd-9-17429-2009, 2009.
 
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