<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys-discuss.net/inc/acpd/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>9</volume_number>
		<issue_number>4</issue_number>
		<publication_year>2009</publication_year>
	</journal>
	<doi>10.5194/acpd-9-16607-2009</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/9/16607/2009/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/9/16607/2009/acpd-9-16607-2009.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/9/16607/2009/acpd-9-16607-2009.pdf</fulltext_pdf>
	<start_page>16607</start_page>
	<end_page>16682</end_page>
	<publication_date>2009-08-07</publication_date>
	<article_title content_type="html">Cirrus clouds in a global climate model with a statistical cirrus cloud scheme</article_title>
	<authors>
		<author numeration="1" affiliations="1,2">
			<name>M. Wang</name>
			<email>minghuai.wang@pnl.gov</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>J. E. Penner</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Department of Atmospheric, Oceanic, and Space Sciences, University of Michigan, USA</affiliation>
		<affiliation numeration="2" content_type="html">now at: Pacific Northwest National Laboratory, Richland, Washington, USA</affiliation>
	</affiliations>
	<abstract content_type="html">A statistical cirrus cloud scheme that accounts for mesoscale temperature
perturbations is implemented into a coupled aerosol and atmospheric
circulation model to better represent both cloud fraction and subgrid-scale
supersaturation in global climate models. This new scheme is able to better
simulate the observed probability distribution of relative humidity than the
scheme that was implemented in an older version of the model. Heterogeneous
ice nuclei (IN) are shown to affect not only high level cirrus clouds
through their effect on ice crystal number concentration but also low level
liquid clouds through the moistening effect of settling and evaporating ice
crystals. As a result, the change in the net cloud forcing is not very
sensitive to the change in ice crystal concentrations associated with
heterogeneous IN because changes in high cirrus clouds and low level liquid
clouds tend to cancel. Nevertheless, the change in the net radiative flux at
the top of the atmosphere due to changes in IN is still large because of
changes in the greenhouse effect of water vapor caused by the changes in ice
crystal number concentrations. Changes in the magnitude of the assumed
mesoscale temperature perturbations by 25% alter the ice crystal number
concentrations and radiative fluxes by an amount that is similar to that
from a factor of 10 change in the heterogeneous IN number concentrations.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Abbatt, J. P. D., Benz, S., Cziczo, D. J., Kanji, Z., Lohmann, U., and Möhler, O.: Solid ammonium sulfate aerosols as ice nuclei: A pathway for cirrus cloud formation, Science, 313, 1770–1773, doi:10.1126/science.1129726, 2006. </reference>
		<reference numeration="2" content_type="text"> Abdul-Razzak, H. and Ghan, S. J.: A parameterization of aerosol activation 2. Multiple aerosol types, J. Geophys. Res., 105, 6837–6844, 2000. </reference>
		<reference numeration="3" content_type="text">Abdul-Razzak, H. and Ghan, S. J.: A parameterization of aerosol activation 3. Sectional representation, J. Geophys. Res., 107, 4026, doi:10.1029/2001JD000483, 2002. </reference>
		<reference numeration="4" content_type="text"> Andres, R. J. and Kasgnoc, A. D.: A time-averaged inventory of subaerial volcanic sulfur emissions, J. Geophys. Res., 103, 25251–25261, 1998. </reference>
		<reference numeration="5" content_type="text"> Bacmeister, J. T., Eckermann, S. D., Tsias, A., Carslaw, K. S., and Peter, T.: Mesoscale temperature fluctuations induced by a spectrum of gravity waves: A comparison of parameterizations and their impact on stratospheric microphysics, J. Atmos. Sci., 56, 1913–1924, 1999. </reference>
		<reference numeration="6" content_type="text"> Beheng, K. D.: A parameterization of warm cloud microphysical conversion processes, Atmos. Res., 33, 193–206, 1994. </reference>
		<reference numeration="7" content_type="text"> Boville, B. A., Rasch, P. J., Hack, J. J., and McCaa, J. R.: Representation of clouds and precipitation processes in the Community Atmosphere Model version 3 (CAM3), J. Climate, 19, 2184–2198, 2006. </reference>
		<reference numeration="8" content_type="text"> Burkhardt, U., Kärcher, B., Ponater, M., Gierens, K., and Gettelman, A.: Contrail cirrus supporting areas in model and observations, Geophys. Res. Lett., 35, L16808, doi:10.1029/2008gl034056, 2008. </reference>
		<reference numeration="9" content_type="text"> Cantrell, W. and Heymsfield, A.: Production of ice in tropospheric clouds - A review, B. Am. Meteor. Soc., 86, 795–807, 2005. </reference>
		<reference numeration="10" content_type="text"> Chen, Y. L., Kreidenweis, S. M., McInnes, L. M., Rogers, D. C., and DeMott, P. J.: Single particle analyses of ice nucleating aerosols in the upper troposphere and lower stratosphere, Geophys. Res. Lett., 25, 1391–1394, 1998. </reference>
		<reference numeration="11" content_type="text"> Chen, T., Rossow, W. B., and Zhang, Y. C.: Radiative effects of cloud-type variations, J. Climate, 13, 264–286, 2000. </reference>
		<reference numeration="12" content_type="text"> Chen, Y.: Aerosol indirect effects on clouds and global climate, PhD, Department of Atmospheric, Oceanic, and Space Sciences, University of Michigan, Ann Arbor, MI, 218~pp., 2006. </reference>
		<reference numeration="13" content_type="text"> Collins, W. D.: Parameterization of generalized cloud overlap for radiative calculations in general circulation models, J. Atmos. Sci., 58, 3224–3242, 2001. </reference>
		<reference numeration="14" content_type="text"> Collins, W. D., Bitz, C. M., Blackmon, M. L., Bonan, G. B., Bretherton, C. S., Carton, J. A., Chang, P., Doney, S. C., Hack, J. J., Henderson, T. B., Kiehl, J. T., Large, W. G., McKenna, D. S., Santer, B. D., and Smith, R. D.: The Community Climate System Model version 3 (CCSM3), J. Climate, 19, 2122–2143, 2006. </reference>
		<reference numeration="15" content_type="text"> Collins, W. D., Rasch, P. J., Boville, B. A., Hack, J. J., McCaa, J. R., Williamson, D. L., Briegleb, B. P., Bitz, C. M., Lin, S. J., and Zhang, M. H.: The formulation and atmospheric simulation of the Community Atmosphere Model version 3 (CAM3), J. Climate, 19, 2144–2161, 2006. </reference>
		<reference numeration="16" content_type="text"> Cziczo, D. J., Murphy, D. M., Hudson, P. K., and Thomson, D. S.: Single particle measurements of the chemical composition of cirrus ice residue during CRYSTAL-FACE, J. Geophys. Res., 109, D04201, doi:10.1029/2003JD004032, 2004. </reference>
		<reference numeration="17" content_type="text"> Cziczo, D. J., Stetzer, O., Worringen, A., Ebert, M., Weinbruch, S., Kamphus, M., Gallavardin, S. J., Curtius, J., Borrmann, S., Froyd, K. D., Mertes, S., Möhler, O., and Lohmann, U: Inadvertent climate modification due to anthropogenic lead, Nature Geoscience, 2, 333–336, doi:10.1038/NGEO499, 2009. </reference>
		<reference numeration="18" content_type="text"> de Reus, M., Dentener, F., Thomas, A., Borrmann, S., Ström, J., and Lelieveld, J.: Airborne observations of dust aerosol over the North Atlantic Ocean during ACE 2: Indications for heterogeneous ozone destruction, J. Geophys. Res., 105, 15263–15275, 2000. </reference>
		<reference numeration="19" content_type="text"> DeMott, P. J., Rogers, D. C., and Kreidenweis, S. M.: The susceptibility of ice formation in upper tropospheric clouds to insoluble aerosol components, J. Geophys. Res., 102, 19575–19584, 1997. </reference>
		<reference numeration="20" content_type="text"> DeMott, P. J., Sassen, K., Poellot, M. R., Baumgardner, D., Rogers, D. C., Brooks, S. D., Prenni, A. J., and Kreidenweis, S. M.: African dust aerosols as atmospheric ice nuclei, Geophys. Res. Lett., 30, 1732, doi:10.1029/2003GL017410, 2003. </reference>
		<reference numeration="21" content_type="text"> Eyers, C. J., Norman, P., Middel, J., Plohr, M., Michot, S., Atkinson, K., and Christou, R. A.: AERO2k Global Aviation Emissions Inventories for 2002 and 2025, QinetiQ/-4/01113, online available at: http://www.cate.mmu.ac.uk/reports_aero2k.asp?chg=projects&amp;chg2=2&gt;http://www.cate.mmu.ac.uk/reports_aero2k.asp?chg=projects&amp;chg2=2, 2004. </reference>
		<reference numeration="22" content_type="text"> Ferraro, R. R., Weng, F. Z., Grody, N. C., and Basist, A.: An eight-year (1987-1994) time series of rainfall, clouds, water vapor, snow cover, and sea ice derived from SSM/I measurements, B. Am. Meteor. Soc., 77, 891–905, 1996. </reference>
		<reference numeration="23" content_type="text"> Forster, P. M. D. and Shine, K. P.: Assessing the climate impact of trends in stratospheric water vapor, Geophys. Res. Lett., 29, 1086, doi:10.1029/2001gl013909, 2002. </reference>
		<reference numeration="24" content_type="text"> Fritts, D. C. and Alexander, M. J.: Gravity wave dynamics and effects in the middle atmosphere, Rev. Geophys., 41, 1003, doi:10.1029/2001rg000106, 2003. </reference>
		<reference numeration="25" content_type="text"> Gallagher, M. W., Connolly, P. J., Whiteway, J., Figueras-Nieto, D., Flynn, M., Choularton, T. W., Bower, K. N., Cook, C., Busen, R., and Hacker, J.: An overview of the microphysical structure of cirrus clouds observed during EMERALD-1, Q. J. Roy. Meteorol. Soc., 131, 1143–1169, doi:10.1256/Qj.03.138, 2005. </reference>
		<reference numeration="26" content_type="text"> Gary, B. L.: Mesoscale temperature fluctuations in the stratosphere, Atmos. Chem. Phys., 6, 4577–4589, 2006. </reference>
		<reference numeration="27" content_type="text"> Gary, B. L.: Mesoscale temperature fluctuations in the Southern Hemisphere stratosphere, Atmos. Chem. Phys., 8, 4677–4681, 2008. </reference>
		<reference numeration="28" content_type="text"> Gayet, J. F., Auriol, F., Minikin, A., Ström, J., Seifert, M., Krejci, R., Petzold, A., Febvre, G., and Schumann, U.: Quantitative measurement of the microphysical and optical properties of cirrus clouds with four different in situ probes: Evidence of small ice crystals, Geophys. Res. Lett., 29, 2230, doi:10.1029/2001gl014342, 2002. </reference>
		<reference numeration="29" content_type="text"> Gayet, J. F., Ovarlez, J., Shcherbakov, V., Ström, J., Schumann, U., Minikin, A., Auriol, F., Petzold, A., and Monier, M.: Cirrus cloud microphysical and optical properties at southern and northern midlatitudes during the INCA experiment, J. Geophys. Res., 109, D20206, doi:10.1029/2004jd004803, 2004. </reference>
		<reference numeration="30" content_type="text"> Gayet, J. F., Shcherbakov, V., Mannstein, H., Minikin, A., Schumann, U., Ström, J., Petzold, A., Ovarlez, J., and Immler, F.: Microphysical and optical properties of midlatitude cirrus clouds observed in the southern hemisphere during INCA, Q. J. Roy. Meteorol. Soc., 132, 2719–2748, doi:10.1256/Qj.05.162, 2006. </reference>
		<reference numeration="31" content_type="text"> Gettelman, A., Morrison, H., and Ghan, S. J.: A new two-moment bulk stratiform cloud microphysics scheme in the community atmosphere model, version 3 (CAM3). Part II: Single-colunm and global results, J. Climate, 21, 3660–3679, 2008. </reference>
		<reference numeration="32" content_type="text"> Ghan, S., Laulainen, N., Easter, R., Wagener, R., Nemesure, S., Chapman, E., Zhang, Y., and Leung, R.: Evaluation of aerosol direct radiative forcing in MIRAGE, J. Geophys. Res., 106, 5295–5316, 2001. </reference>
		<reference numeration="33" content_type="text"> Gierens, K.: On the transition between heterogeneous and homogeneous freezing, Atmos. Chem. Phys., 3, 437–446, 2003. </reference>
		<reference numeration="34" content_type="text"> Ginoux, P., Chin, M., Tegen, I., Prospero, J. M., Holben, B., Dubovik, O., and Lin, S. J.: Sources and distributions of dust aerosols simulated with the GOCART model, J. Geophys. Res., 106, 20255–20273, 2001. </reference>
		<reference numeration="35" content_type="text"> Gong, S. L., Barrie, L. A., and Blanchet, J. P.: Modeling sea-salt aerosols in the atmosphere .1. Model development, J. Geophys. Res., 102, 3805–3818, 1997. </reference>
		<reference numeration="36" content_type="text"> Grabowski, W. W.: Cloud microphysics and the tropical climate: Cloud-resolving model perspective, J. Climate, 13, 2306–2322, 2000. </reference>
		<reference numeration="37" content_type="text"> Greenwald, T. J., Stephens, G. L., Vonderhaar, T. H., and Jackson, D. L.: A physical retrieval of cloud liquid water over the global oceans using special sensor microwave imager (SSM/I) observations, J. Geophys. Res., 98, 18471–18488, 1993. </reference>
		<reference numeration="38" content_type="text"> Haag, W., Kärcher, B., Ström, J., Minikin, A., Lohmann, U., Ovarlez, J., and Stohl, A.: Freezing thresholds and cirrus cloud formation mechanisms inferred from in situ measurements of relative humidity, Atmos. Chem. Phys., 3, 1791–1806, 2003. </reference>
		<reference numeration="39" content_type="text"> Haag, W. and Kärcher, B.: The impact of aerosols and gravity waves on cirrus clouds at midlatitudes, J. Geophys. Res., 109, D12202, doi:10.1029/2004JD004579, 2004. </reference>
		<reference numeration="40" content_type="text"> Hall, W. D. and Pruppacher, H. R.: Survival of Ice Particles Falling from Cirrus Clouds in Subsaturated Air, J. Atmos. Sci., 33, 1995–2006, 1976. </reference>
		<reference numeration="41" content_type="text"> Han, Q. Y., Rossow, W. B., and Lacis, A. A.: Near-Global survey of effective droplet radii in liquid water clouds using ISCCP data, J. Climate, 7, 465–497, 1994. </reference>
		<reference numeration="42" content_type="text"> Han, Q. Y., Rossow, W. B., Chou, J., and Welch, R. M.: Global variation of column droplet concentration in low-level clouds, Geophys. Res. Lett., 25, 1419–1422, 1998. </reference>
		<reference numeration="43" content_type="text"> Hendricks, J., Kärcher, B., Döpelheuer, A., Feichter, J., Lohmann, U., and Baumgardner, D.: Simulating the global atmospheric black carbon cycle: a revisit to the contribution of aircraft emissions, Atmos. Chem. Phys., 4, 2521–2541, 2004. </reference>
		<reference numeration="44" content_type="text"> Hendricks, J., Kärcher, B., Lohmann, U., and Ponater, M.: Do aircraft black carbon emissions affect cirrus clouds on the global scale?, Geophys. Res. Lett., 32, L12814, doi:10.1029/2005gl022740, 2005. </reference>
		<reference numeration="45" content_type="text"> Heymsfield, A. J.: Precipitation development in stratiform ice clouds - microphysical and dynamical study, J. Atmos. Sci., 34, 367–381, 1977. </reference>
		<reference numeration="46" content_type="text"> Heymsfield, A. J. and Sabin, R. M.: Cirrus crystal nucleation by homogeneous freezing of solution droplets, J. Atmos. Sci., 46, 2252–2264, 1989. </reference>
		<reference numeration="47" content_type="text"> Hoyle, C. R., Luo, B. P., and Peter, T.: The origin of high ice crystal number densities in cirrus clouds, J. Atmos. Sci., 62, 2568–2579, 2005. </reference>
		<reference numeration="48" content_type="text"> Immler, F., Krüger, K., Fujiwara, M., Verver, G., Rex, M., and Schrems, O.: Correlation between equatorial Kelvin waves and the occurrence of extremely thin ice clouds at the tropical tropopause, Atmos. Chem. Phys., 8, 4019–4026, 2008. </reference>
		<reference numeration="49" content_type="text"> Ito, A. and Penner, J. E.: Historical emissions of carbonaceous aerosols from biomass and fossil fuel burning for the period 1870-2000, Global Biogeochem. Cy., 19, GB2028, doi:10.1029/2004GB002374, 2005. </reference>
		<reference numeration="50" content_type="text"> Jensen, E. J., Toon, O. B., Westphal, D. L., Kinne, S., and Heysmfield, A. J.: Microphysical modeling of cirrus.1. Comparison with 1986 FIRE IFO measurements, J. Geophys. Res., 99, 10421–10442, 1994. </reference>
		<reference numeration="51" content_type="text"> Jensen, E. J. and Toon, O. B.: The potential impact of soot particles from aircraft exhaust on cirrus clouds, Geophys. Res. Lett., 24, 249–252, 1997. </reference>
		<reference numeration="52" content_type="text"> Jensen, E. and Pfister, L.: Transport and freeze-drying in the tropical tropopause layer, J. Geophys. Res., 109, D02207, doi:10.1029/2003JD004022, 2004. </reference>
		<reference numeration="53" content_type="text"> Jensen, E. J., Pfister, L., Bui, T. V., Lawson, P., Baker, B., Mo, Q., Baumgardner, D., Weinstock, E. M., Smith, J. B., Moyer, E. J., Hanisco, T. F., Sayres, D. S., Clair, J. M. St., Alexander, M. J., Toon, O. B., and Smith, J. A.: Formation of large (&amp;#x2243;100 μm) ice crystals near the tropical tropopause, Atmos. Chem. Phys., 8, 1621–1633, 2008. </reference>
		<reference numeration="54" content_type="text"> Kärcher, B. and Lohmann, U.: A parameterization of cirrus cloud formation: Homogeneous freezing of supercooled aerosols, J. Geophys. Res., 107, 4010, doi:10.1029/2001jd000470, 2002. </reference>
		<reference numeration="55" content_type="text"> Kärcher, B. and Ström, J.: The roles of dynamical variability and aerosols in cirrus cloud formation, Atmos. Chem. Phys., 3, 823–838, 2003. </reference>
		<reference numeration="56" content_type="text"> Kärcher, B., Hendricks, J., and Lohmann, U.: Physically based parameterization of cirrus cloud formation for use in global atmospheric models, J. Geophys. Res., 111, D01205, doi:10.1029/2005JD006219, 2006. </reference>
		<reference numeration="57" content_type="text"> Kärcher, B. and Burkhardt, U.: A cirrus cloud scheme for general circulation models, Q. J. Roy. Meteorol. Soc., 134, 1439–1461, doi:10.1002/Qj.301, 2008. </reference>
		<reference numeration="58" content_type="text"> Kettle, A. J. and Andreae, M. O.: Flux of dimethylsulfide from the oceans: A comparison of updated data seas and flux models, J. Geophys. Res., 105, 26793–26808, 2000. </reference>
		<reference numeration="59" content_type="text"> Khvorostyanov, V. I., Morrison, H., Curry, J. A., Baumgardner, D., and Lawson, P.: High supersaturation and modes of ice nucleation in thin tropopause cirrus: Simulation of the 13 July 2002 Cirrus Regional Study of Tropical Anvils and Cirrus Layers case, J. Geophys. Res., 111, D02201, doi:10.1029/2004JD005235, 2006. </reference>
		<reference numeration="60" content_type="text"> Kiehl, J. T. and Trenberth, K. E.: Earth&apos;s annual global mean energy budget, B. Am. Meteor. Soc., 78, 197–208, 1997. </reference>
		<reference numeration="61" content_type="text"> King, M. D., Menzel, W. P., Kaufman, Y. J., Tanre, D., Gao, B. C., Platnick, S., Ackerman, S. A., Remer, L. A., Pincus, R., and Hubanks, P. A.: Cloud and aerosol properties, precipitable water, and profiles of temperature and water vapor from MODIS, IEEE T. Geosci. Remote, 41, 442–458, doi:10.1109/Tgrs.2002.808226, 2003. </reference>
		<reference numeration="62" content_type="text"> Kinne, S., Schulz, M., Textor, C., Guibert, S., Balkanski, Y., Bauer, S. E., Berntsen, T., Berglen, T. F., Boucher, O., Chin, M., Collins, W., Dentener, F., Diehl, T., Easter, R., Feichter, J., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Herzog, M., Horowitz, L., Isaksen, I., Iversen, T., Kirkev&amp;aring;g, A., Kloster, S., Koch, D., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Lesins, G., Liu, X., Lohmann, U., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, O., Stier, P., Takemura, T., and Tie, X.: An AeroCom initial assessment – optical properties in aerosol component modules of global models, Atmos. Chem. Phys., 6, 1815–1834, 2006. </reference>
		<reference numeration="63" content_type="text"> Koop, T., Luo, B. P., Tsias, A., and Peter, T.: Water activity as the determinant for homogeneous ice nucleation in aqueous solutions, Nature, 406, 611–614, 2000. </reference>
		<reference numeration="64" content_type="text"> Krämer, M., Schiller, C., Afchine, A., Bauer, R., Gensch, I., Mangold, A., Schlicht, S., Spelten, N., Sitnikov, N., Borrmann, S., de Reus, M., and Spichtinger, P.: Ice supersaturations and cirrus cloud crystal numbers, Atmos. Chem. Phys., 9, 3505–3522, 2009. </reference>
		<reference numeration="65" content_type="text"> Lee, D. S., Owen, B., Graham, A., Fichter, C., Lim, L. L., and Dimitriu, D.: Study of the allocation of aviation emissions from scheduled air traffic – present day and historical, Final Report to DEFRA Global Atmosphere Division, Manchester Metropolitan University, 62~pp., online available at: Available from http://www.cate.mmu.ac.uk/project_view.asp?chg=projects&amp;chg2=2&amp;d=2&gt;http://www.cate.mmu.ac.uk/project_view.asp?chg=projects&amp;chg2=2&amp;id=2, 2005. </reference>
		<reference numeration="66" content_type="text"> Li, J. L., Waliser, D. E., Jiang, J. H., Wu, D. L., Read, W., Waters, J. W., Tompkins, A. M., Donner, L. J., Chern, J. D., Tao, W. K., Atlas, R., Gu, Y., Liou, K. N., Del Genio, A., Khairoutdinov, M., and Gettelman, A.: Comparisons of EOS MLS cloud ice measurements with ECMWF analyses and GCM simulations: Initial results, Geophys. Res. Lett., 32, L18710, doi:10.1029/2005GL023788 2005. </reference>
		<reference numeration="67" content_type="text"> Liu, X. H. and Penner, J. E.: Effect of Mount Pinatubo H2SO4/H2O aerosol on ice nucleation in the upper troposphere using a global chemistry and transport model, J. Geophys. Res., 107, 4141, doi:10.1029/2001JD000455, 2002. </reference>
		<reference numeration="68" content_type="text"> Liu, X. H. and Penner, J. E.: Ice nucleation parameterization for global models, Meteor. Z., 14, 499–514, doi:10.1127/0941-2948/2005/0059, 2005. </reference>
		<reference numeration="69" content_type="text"> Liu, X., Penner, J. E., Ghan, S. J., and Wang, M.: Inclusion of ice microphysics in the NCAR community atmospheric model version 3 (CAM3), J. Climate, 20, 4526–4547, 2007. </reference>
		<reference numeration="70" content_type="text"> Liu, X. H., Xie, S. C., and Ghan, S. J.: Evaluation of a new mixed-phase cloud microphysics parameterization with CAM3 single-column model and M-PACE observations, Geophys. Res. Lett., 34, L23712 doi:10.1029/2007GL031446, 2007. </reference>
		<reference numeration="71" content_type="text"> Liu, X. H., Penner, J. E., and Wang, M. H.: Influence of anthropogenic sulfate and black carbon on upper tropospheric clouds in the NCAR CAM3 model coupled to the IMPACT global aerosol model, J. Geophys. Res., 114, D03204, doi:10.1029/2008JD010492 2009. </reference>
		<reference numeration="72" content_type="text"> Lohmann, U., Feichter, J., Chuang, C. C., and Penner, J. E.: Prediction of the number of cloud droplets in the ECHAM GCM, J. Geophys. Res., 104, 9169–9198, 1999. </reference>
		<reference numeration="73" content_type="text"> Lohmann, U. and Kärcher, B.: First interactive simulations of cirrus clouds formed by homogeneous freezing in the ECHAM general circulation model, J. Geophys. Res., 107, 4105, doi:10.1029/2001JD000767, 2002. </reference>
		<reference numeration="74" content_type="text"> Lohmann, U., Stier, P., Hoose, C., Ferrachat, S., Kloster, S., Roeckner, E., and Zhang, J.: Cloud microphysics and aerosol indirect effects in the global climate model ECHAM5-HAM, Atmos. Chem. Phys., 7, 3425–3446, 2007. </reference>
		<reference numeration="75" content_type="text"> Mace, G. G., Clothiaux, E. E., and Ackerman, T. P.: The composite characteristics of cirrus clouds: Bulk properties revealed by one year of continuous cloud radar data, J. Climate, 14, 2185–2203, 2001. </reference>
		<reference numeration="76" content_type="text"> Marcolli, C., Gedamke, S., Peter, T., and Zobrist, B.: Efficiency of immersion mode ice nucleation on surrogates of mineral dust, Atmos. Chem. Phys., 7, 5081–5091, 2007. </reference>
		<reference numeration="77" content_type="text"> Meyers, M. P., DeMott, P. J., and Cotton, W. R.: New primary ice nucleation parameterizations in an explicit cloud model, J. Appl. Meteorol., 31, 708–721, 1992. </reference>
		<reference numeration="78" content_type="text"> Mitchell, D. L., Rasch, P., Ivanova, D., McFarquhar, G., and Nousiainen, T.: Impact of small ice crystal assumptions on ice sedimentation rates in cirrus clouds and GCM simulations, Geophys. Res. Lett., 35, L09806, doi:10.1029/2008GL033552 2008. </reference>
		<reference numeration="79" content_type="text"> Möhler, O., Field, P. R., Connolly, P., Benz, S., Saathoff, H., Schnaiter, M., Wagner, R., Cotton, R., Krämer, M., Mangold, A., and Heymsfield, A. J.: Efficiency of the deposition mode ice nucleation on mineral dust particles, Atmos. Chem. Phys., 6, 3007–3021, 2006. </reference>
		<reference numeration="80" content_type="text"> Murphy, D. M. and Koop, T.: Review of the vapour pressures of ice and supercooled water for atmospheric applications, Q. J. Roy. Meteorol. Soc., 131, 1539–1565, doi:10.1256/Qj.04.94, 2005. </reference>
		<reference numeration="81" content_type="text"> Penner, J. E., Andreae, M. O., Annegarn, H., Barrie, L., Feichter, J., Hegg, D., Jayaraman, A., Leaitch, R., Murphy, D., Nganga, J., and Pitari, G.: Aerosols, their Direct and Indirect Effects, in: Climate Change 2001: The Scientific Basis, Contribution of working group I to the Third Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Houghton, J. T., Ding, Y., Griggs, D. J., Noguer, M., Van der Linden, P. J., Dai, X., Maskell, K., and Johnson, C. A., Cambridge University Press, New York, 881, 2001. </reference>
		<reference numeration="82" content_type="text"> Penner, J. E., Chen, Y., Wang, M., and Liu, X.: Possible influence of anthropogenic aerosols on cirrus clouds and anthropogenic forcing, Atmos. Chem. Phys., 9, 879–896, 2009. </reference>
		<reference numeration="83" content_type="text"> Petzold, A. and Schröder, F. P.: Jet engine exhaust aerosol characterization, Aerosol Sci. Tech., 28, 62–76, 1998. </reference>
		<reference numeration="84" content_type="text"> Phillips, V. T. J., DeMott, P. J., and Andronache, C.: An empirical parameterization of heterogeneous ice nucleation for multiple chemical species of aerosol, J. Atmos. Sci., 65, 2757–2783, doi:10.1175/2007jas2546.1, 2008. </reference>
		<reference numeration="85" content_type="text"> Platnick, S., King, M. D., Ackerman, S. A., Menzel, W. P., Baum, B. A., Riedi, J. C., and Frey, R. A.: The MODIS cloud products: Algorithms and examples from Terra, IEEE T. Geosci. Remote, 41, 459–473, 2003. </reference>
		<reference numeration="86" content_type="text"> Pruppacher, H. R. and Klett, J. D.: Microphysics of Cloud and Precipitation, Springer, New York, 954~pp., 1997. </reference>
		<reference numeration="87" content_type="text"> Pusechel, R. F., Blake, D. F., Snetsinger, K. G., Hansen, A. D. A., Verma, S., and Kato, K.: Black carbon (Soot) aerosol in the lower stratosphere and upper troposphere, Geophys. Res. Lett., 19, 1659–1662, 1992. </reference>
		<reference numeration="88" content_type="text"> Quaas, J., Boucher, O., and Breon, F. M.: Aerosol indirect effects in POLDER satellite data and the Laboratoire de Meteorologie Dynamique-Zoom (LMDZ) general circulation model, J. Geophys. Res., 109, D08205, doi:10.1029/2003jd004317, 2004. </reference>
		<reference numeration="89" content_type="text"> Quaas, J., Boucher, O., and Lohmann, U.: Constraining the total aerosol indirect effect in the LMDZ and ECHAM4 GCMs using MODIS satellite data, Atmos. Chem. Phys., 6, 947–955, 2006. </reference>
		<reference numeration="90" content_type="text"> Quinn, P. K. and Coffman, D. J.: Local closure during the First Aerosol Characterization Experiment (ACE 1): Aerosol mass concentration and scattering and backscattering coefficients, J. Geophys. Res., 103, 16575–16596, 1998. </reference>
		<reference numeration="91" content_type="text"> Ramanathan, V. and Collins, W.: Thermodynamic regulation of ocean warming by cirrus clouds deduced from observations of the 1987 El-Nino, Nature, 351, 27–32, 1991. </reference>
		<reference numeration="92" content_type="text"> Rasch, P. J. and Kristjansson, J. E.: A comparison of the CCM3 model climate using diagnosed and predicted condensate parameterizations, J. Climate, 11, 1587–1614, 1998. </reference>
		<reference numeration="93" content_type="text"> Raval, A. and Ramanathan, V.: Observational determination of the greenhouse-effect, Nature, 342, 758–761, 1989. </reference>
		<reference numeration="94" content_type="text"> Read, W. G., Waters, J. W., Wu, D. L., Stone, E. M., Shippony, Z., Smedley, A. C., Smallcomb, C. C., Oltmans, S., Kley, D., Smit, H. G. J., Mergenthaler, J. L., and Karki, M. K.: UARS microwave limb sounder upper tropospheric humidity measurement: Method and validation, J. Geophys. Res., 106, 32207–32258, 2001. </reference>
		<reference numeration="95" content_type="text"> Rossow, W. B. and Schiffer, R. A.: Advances in understanding clouds from ISCCP, B. Amer. Meteor. Soc., 80, 2261–2287, 1999. </reference>
		<reference numeration="96" content_type="text"> Rotstayn, L. D., Ryan, B. F., and Katzfey, J. J.: A scheme for calculation of the liquid fraction in mixed-phase stratiform clouds in large-scale models, Mon. Weather Rev., 128, 1070–1088, 2000. </reference>
		<reference numeration="97" content_type="text"> Rotstayn, L. D. and Liu, Y. G.: Sensitivity of the first indirect aerosol effect to an increase of cloud droplet spectral dispersion with droplet number concentration, J. Climate, 16, 3476–3481, 2003. </reference>
		<reference numeration="98" content_type="text"> Rotstayn, L. D., Cai, W. J., Dix, M. R., Farquhar, G. D., Feng, Y., Ginoux, P., Herzog, M., Ito, A., Penner, J. E., Roderick, M. L., and Wang, M. H.: Have Australian rainfall and cloudiness increased due to the remote effects of Asian anthropogenic aerosols?, J. Geophys. Res., 112, D09202, doi:10.1029/2006jd007712, 2007. </reference>
		<reference numeration="99" content_type="text"> Sanderson, B. M., Piani, C., Ingram, W. J., Stone, D. A., and Allen, M. R.: Towards constraining climate sensitivity by linear analysis of feedback patterns in thousands of perturbed-physics GCM simulations, Clim. Dynam., 30, 175–190, 2008. </reference>
		<reference numeration="100" content_type="text"> Schroder, F., Kärcher, B., Duroure, C., Ström, J., Petzold, A., Gayet, J. F., Strauss, B., Wendling, P., and Borrmann, S.: On the transition of contrails into cirrus clouds, J. Atmos. Sci., 57, 464–480, 2000. </reference>
		<reference numeration="101" content_type="text"> Schulz, M., Textor, C., Kinne, S., Balkanski, Y., Bauer, S., Berntsen, T., Berglen, T., Boucher, O., Dentener, F., Guibert, S., Isaksen, I. S. A., Iversen, T., Koch, D., Kirkev&amp;aring;g, A., Liu, X., Montanaro, V., Myhre, G., Penner, J. E., Pitari, G., Reddy, S., Seland, Ø., Stier, P., and Takemura, T.: Radiative forcing by aerosols as derived from the AeroCom present-day and pre-industrial simulations, Atmos. Chem. Phys., 6, 5225–5246, 2006. </reference>
		<reference numeration="102" content_type="text"> Seifert, M., Ström, J., Krejci, R., Minikin, A., Petzold, A., Gayet, J.-F., Schumann, U., and Ovarlez, J.: In-situ observations of aerosol particles remaining from evaporated cirrus crystals: Comparing clean and polluted air masses, Atmos. Chem. Phys., 3, 1037–1049, 2003. </reference>
		<reference numeration="103" content_type="text"> Smith, W. L., Ackerman, S., Revercomb, H., Huang, H., DeSlover, D. H., Feltz, W., Gumley, L., and Collard, A.: Infrared spectral absorption of nearly invisible cirrus clouds, Geophys. Res. Lett., 25, 1137–1140, 1998. </reference>
		<reference numeration="104" content_type="text"> Smith, S. J., Pitcher, H., and Wigley, T. M. L.: Global and regional anthropogenic sulfur dioxide emissions, Global Planet. Change, 29, 99–119, 2001. </reference>
		<reference numeration="105" content_type="text"> Smith, S., Andres, R., Conception, L., and Lurz, J.: Historical sulfur dioxide emissions 1850–2000: Methods and resutls, JGCRI Research report PNNL 14537, Paciific Northwest National Laboratory, Richland, WA, USA14537, 16, 2004. </reference>
		<reference numeration="106" content_type="text"> Spichtinger, P., Gierens, K., and Read, W.: The global distribution of ice-supersaturated regions as seen by the Microwave Limb Sounder, Q. J. Roy. Meteorol. Soc., 129, 3391–3410, 2003. </reference>
		<reference numeration="107" content_type="text"> Spichtinger, P., Gierens, K., Smit, H. G. J., Ovarlez, J., and Gayet, J.-F.: On the distribution of relative humidity in cirrus clouds, Atmos. Chem. Phys., 4, 639–647, 2004. </reference>
		<reference numeration="108" content_type="text"> Stephens, G. L., Tsay, S. C., Stackhouse, P. W., and Flatau, P. J.: The relevance of the microphysical and radiative properties of cirrus clouds to climate and climatic feedback, J. Atmos. Sci., 47, 1742–1753, 1990. </reference>
		<reference numeration="109" content_type="text"> Storelvmo, T., Kristjansson, J. E., and Lohmann, U.: Aerosol influence on mixed-phase clouds in CAM-Oslo, J. Atmos. Sci., 65, 3214–3230, doi:10.1175/2008jas2430.1, 2008. </reference>
		<reference numeration="110" content_type="text"> Ström, J. and Heintzenberg, J.: Water-vapor, condensed Water, and crystal concentration in orographically influenced cirrus clouds, J. Atmos. Sci., 51, 2368–2383, 1994. </reference>
		<reference numeration="111" content_type="text"> Ström, J., Strauss, B., Anderson, T., Schroder, F., Heintzenberg, J., and Wendling, P.: In situ observations of the microphysical properties of young cirrus clouds, J. Atmos. Sci., 54, 2542–2553, 1997. </reference>
		<reference numeration="112" content_type="text"> Ström, J. and Ohlsson, S.: In situ measurements of enhanced crystal number densities in cirrus clouds caused by aircraft exhaust, J. Geophys. Res., 103, 11355–11361, 1998. </reference>
		<reference numeration="113" content_type="text"> Ström, J. and Ohlsson, S.: Real-time measurement of absorbing material in contrail ice using a counterflow virtual impactor, J. Geophys. Res., 103, 8737–8741, 1998. </reference>
		<reference numeration="114" content_type="text"> Ström, J., Seifert, M., Kärcher, B., Ovarlez, J., Minikin, A., Gayet, J.-F., Krejci, R., Petzold, A., Auriol, F., Haag, W., Busen, R., Schumann, U., and Hansson, H. C.: Cirrus cloud occurrence as function of ambient relative humidity: a comparison of observations obtained during the INCA experiment, Atmos. Chem. Phys., 3, 1807–1816, 2003. </reference>
		<reference numeration="115" content_type="text"> Textor, C., Schulz, M., Guibert, S., Kinne, S., Balkanski, Y., Bauer, S., Berntsen, T., Berglen, T., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Feichter, H., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Horowitz, L., Huang, P., Isaksen, I., Iversen, I., Kloster, S., Koch, D., Kirkev&amp;aring;g, A., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Liu, X., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, Ø., Stier, P., Takemura, T., and Tie, X.: Analysis and quantification of the diversities of aerosol life cycles within AeroCom, Atmos. Chem. Phys., 6, 1777–1813, 2006. </reference>
		<reference numeration="116" content_type="text"> Tiedtke, M.: Representation of clouds in large-scale models, Mon. Weather Rev., 121, 3040–3061, 1993. </reference>
		<reference numeration="117" content_type="text"> Tompkins, A. M., Gierens, K., and Radel, G.: Ice supersaturation in the ECMWF integrated forecast system, Q. J. Roy. Meteorol. Soc., 133, 53–63, 2007. </reference>
		<reference numeration="118" content_type="text"> Waliser, D. E., Li, J. L. F., Woods, C. P., Austin, R. T., Bacmeister, J., Chern, J., Del Genio, A., Jiang, J. H., Kuang, Z. M., Meng, H., Minnis, P., Platnick, S., Rossow, W. B., Stephens, G. L., Sun-Mack, S., Tao, W. K., Tompkins, A. M., Vane, D. G., Walker, C., and Wu, D.: Cloud ice: A climate model challenge with signs and expectations of progress, J. Geophys. Res., 114, D00A21, doi:10.1029/2008JD010015, 2009. </reference>
		<reference numeration="119" content_type="text"> Wang, P. H., Minnis, P., McCormick, M. P., Kent, G. S., and Skeens, K. M.: A 6-year climatology of cloud occurrence frequency from stratospheric aerosol and gas experiment II observations (1985–1990), J. Geophys. Res., 101, 29407–29429, 1996. </reference>
		<reference numeration="120" content_type="text"> Wang, M. and Penner, J. E.: Aerosol indirect forcing in a global model with particle nucleation, Atmos. Chem. Phys., 9, 239–260, 2009. </reference>
		<reference numeration="121" content_type="text"> Wang, M. H., Penner, J. E., and Liu, X. H.: Coupled IMPACT aerosol and NCAR CAM3 model: Evaluation of predicted aerosol number and size distribution, J. Geophys. Res., 114, D06302, doi:10.1029/2008jd010459, 2009. </reference>
		<reference numeration="122" content_type="text"> Weng, F. Z. and Grody, N. C.: Retrieval of cloud liquid water using the Special Sensor Microwave Imager (SSM/I), J. Geophys. Res., 99, 25535–25551, 1994. </reference>
		<reference numeration="123" content_type="text"> Wu, X. Q.: Effects of ice microphysics on tropical radiative-convective-oceanic quasi-equilibrium states, J. Atmos. Sci., 59, 1885–1897, 2002. </reference>
		<reference numeration="124" content_type="text"> Wu, D. L., Jiang, J. H., and Davis, C. P.: EOS MLS cloud ice measurements and cloudy-sky radiative transfer model, IEEE T. Geosci. Remote, 44, 1156–1165, 2006. </reference>
		<reference numeration="125" content_type="text"> Wu, D. L., Austin, R. T., Deng, M., Durden, S. L., Heymsfield, A. J., Jiang, J. H., Lambert, A., Li, J.-L., Livesey, N. J., McFarquhar, G. M., Pittman, J. V., Stephens, G. L., Tanelli, S., Vane, D. G., and Waliser, D. E.: Comparisons of global cloud ice from MLS, CloudSat, and correlative data sets, J. Geophys. Res., 114, D00A24, doi:10.1029/2008JD009946, 2009. </reference>
		<reference numeration="126" content_type="text"> Wylie, D. P. and Menzel, W. P.: Eight years of high cloud statistics using HIRS, J. Climate, 12, 170–184, 1999. </reference>
		<reference numeration="127" content_type="text"> Xie, S. C., Boyle, J., Klein, S. A., Liu, X. H., and Ghan, S.: Simulations of Arctic mixed-phase clouds in forecasts with CAM3 and AM2 for M-PACE, J. Geophys. Res., 113, D04211, doi:10.1029/2007JD009225, 2008. </reference>
		<reference numeration="128" content_type="text"> Zhang, M. H., Lin, W. Y., Bretherton, C. S., Hack, J. J., and Rasch, P. J.: A modified formulation of fractional stratiform condensation rate in the NCAR Community Atmospheric Model (CAM2), J. Geophys. Res., 108, 4035, doi:10.1029/2002JD002523, 2003. </reference>
		<reference numeration="129" content_type="text"> Zobrist, B., Koop, T., Luo, B. P., Marcolli, C., and Peter, T.: Heterogeneous ice nucleation rate coefficient of water droplets coated by a nonadecanol monolayer, J. Phys. Chem. C, 111, 2149–2155, doi:10.1021/Jp066080w, 2007. </reference>
	</references>
</article>

