Atmos. Chem. Phys. Discuss., 9, 1407-1446, 2009
www.atmos-chem-phys-discuss.net/9/1407/2009/
doi:10.5194/acpd-9-1407-2009
© Author(s) 2009. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Quantifying transport into the Arctic lowermost stratosphere
A. Werner1, C. M. Volk1,*, E. V. Ivanova1, T. Wetter1, C. Schiller2, H. Schlager3, and P. Konopka2
1Institute for Atmospheric and Environmental Sciences, University of Frankfurt, Germany
2Institute of Chemistry and Dynamics of the Geosphere, Research Center Jülich, Germany
3Deutsches Zentrum für Luft und Raumfahrt, Institute of Atmospheric Physics, Oberpfaffenhofen, Germany
*now at: Department of Physics, University of Wuppertal, Germany

Abstract. In-situ measurements of the long-lived trace gases N2O, CFC-11 (CCl3F), H-1211 (CBrClF2), CH4, O3 and H2O performed in the Arctic winter 2003 on board the high-altitude aircraft M55 Geophysica are presented and used to study transport into the lowermost stratosphere (LMS). Fractions of air in the LMS originating in i) the troposphere, ii) the extra-vortex stratosphere above 400 K and iii) the Arctic vortex above 400 K are determined using a simple mass balance calculation. The analysis exhibits a strong tropospheric influence of 50% or more in the lowest 20 K of the high-latitude LMS. Above this region the LMS is dominated by air masses having descended from above 400 K. Below the Arctic vortex region at potential temperatures above 360 K, air in the LMS is a mixture of extra-vortex stratospheric and vortex air masses. The vortex fraction increases from about 40% at 360 K to 100% at 400 K for equivalent latitudes >70° N. This influence of air masses descending through the bottom of the polar vortex increases over the course of the winter. By the end of winter a significant fraction of 30% vortex air in the LMS is found even at an equivalent latitude of 40° N. Since the chemical and dynamical history of vortex air is distinct from that of mid-latitude stratospheric air masses, this study implies that the composition of the mid- to high-latitude LMS during late winter and spring is significantly influenced by the Arctic vortex.

Citation: Werner, A., Volk, C. M., Ivanova, E. V., Wetter, T., Schiller, C., Schlager, H., and Konopka, P.: Quantifying transport into the Arctic lowermost stratosphere, Atmos. Chem. Phys. Discuss., 9, 1407-1446, doi:10.5194/acpd-9-1407-2009, 2009.
 
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