<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-9-13569-2009</article-id>
<title-group>
<article-title>UV aerosol indices from SCIAMACHY: introducing the SCattering Index (SCI)</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Penning de Vries</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Beirle</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Wagner</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Max Planck Institute for Chemistry, J.-J.-Becherweg 27, 55128 Mainz, Germany</addr-line>
</aff>
<pub-date pub-type="epub">
<day>19</day>
<month>06</month>
<year>2009</year>
</pub-date>
<volume>9</volume>
<issue>3</issue>
<fpage>13569</fpage>
<lpage>13592</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/9/13569/2009/acpd-9-13569-2009.html">This article is available from http://www.atmos-chem-phys-discuss.net/9/13569/2009/acpd-9-13569-2009.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/9/13569/2009/acpd-9-13569-2009.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/9/13569/2009/acpd-9-13569-2009.pdf</self-uri>
<abstract>
<p>The Absorbing Aerosol Index (AAI) is a useful tool for detecting aerosols
that absorb UV radiation – especially in cases where other aerosol
retrievals fail, such as over bright surfaces (e.g. desert) and in the
presence of clouds. The AAI does not, however, consider contributions from
&quot;scattering&quot; (hardly absorbing) aerosols and clouds: they cause negative
AAI values and are usually discarded. In this paper, we demonstrate the use
of the AAI&apos;s negative counterpart, the SCattering Index (SCI) to detect
&quot;scattering&quot; aerosols. Maps of seasonally averaged SCI show significantly
enhanced values in summer in Southeast USA and Southeast Asia, pointing
to high production of &quot;scattering&quot; aerosols (presumably mainly sulphate
aerosols and organic aerosols) in this season. The application of a cloud
filter makes the presence of &quot;scattering&quot; aerosols even more clear. In a
comparison of AOT from AERONET and our Aerosol Indices from SCIAMACHY, good
agreement was found for two AERONET stations in Southeast USA, and two
stations in Africa. This fact confirms the suitability of SCI as a tool to
detect &quot;scattering&quot; aerosols.

&lt;br&gt;&lt;br&gt;

The combination of the UV Aerosol Indices AAI and SCI provides the unique
possibility to characterise absorbing properties of aerosols from space.
Accurate knowledge about aerosol absorption is crucial for the correct
determination of the contribution of aerosols to the radiative budget.</p>
</abstract>
<counts><page-count count="24"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Barnard, J. C., Volkamer, R., and Kassianov, E. I.: Estimation of the mass absorption cross section of the organic carbon component of aerosols in the Mexico City Metropolitan Area, Atmos. Chem. Phys., 8, 6665–6679, 2008. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Bovensmann, H., Burrows, J. P., Buchwitz, M., Frerick, J., No\&quot;el, S., Rozanov, V. V., Chance, K. V., and Goede, A. P. H.: SCIAMACHY: Mission objectives and measurements modes, J. Atmos. Sci., 56, 127–150, 1999. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Chand, D., Anderson, T. L., Wood, R., Charlson, R. J., Hu, Y., Liu, Z., and Vaughan, M.: Quantifying above-cloud aerosol using spaceborne lidar for improved understanding of cloudy-sky direct climate forcing, J. Geophys. Res., 113, D13206, doi:10.1029/2007JD009433, 2008. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Chiapello, I., Prospero, J. M., Herman, J. R., and Hsu, N. C.: Detection of mineral dust over the North Atlantic Ocean and Africa with the Nimbus 7 TOMS, J. Geophys. Res., 104(D8), 9277–9291, 1999. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Darmenova, K., Sokolik, I. N., and Darmenov, A.: Characterization of east Asian dust outbreaks in the spring of 2001 using ground-based and satellite data, J. Geophys. Res., 110, D02204, doi:10.1029/2004JD004842, 2005. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> de Graaf, M., Stammes, P., Torres, O., and Koelemeijer, R. B. A.: Absorbing Aerosol Index – Sensitivity analysis, application to GOME and comparison with TOMS, J. Geophys. Res., 110, D01202, doi:10.1029/2004JD005178, 2005. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> de Graaf, M. and Stammes, P.: SCIAMACHY Absorbing Aerosol Index – calibration issues and global results from 2002–2004, Atmos. Chem. Phys., 5, 2385–2394, 2005b. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> de Graaf, M., Stammes, P., and Aben, E. A. A.: Analysis of reflectance spectra of UV-absorbing aerosol scenes measured by SCIAMACHY, J. Geophys. Res., 112, D02206, doi:10.1029/2006JD007249, 2007. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Deutschmann, T.: Diploma Thesis, University of Heidelberg, 2008. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Dubovik, O., Holben, B., Eck, T. F., Smirnov, A., Kaufman, Y. J., King, M. D., Tanré, D., and Slutsker, I.: Variability of absorption and optical properties of key aerosol types observed in worldwide locations, J. Atmos. Sci., 59, 590–608, 2002. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Fromm, M., Bevilacqua, R., Servanckx, R., Rosen, J., Thayer, J. P., Herman, J., and Larko, D.: Pyro-cumulonimbus injection of smoke to the stratosphere: Observations and impact of a super blowup in northwestern Canada on 3–4 August 1998, J. Geophys. Res., 110, D08205, doi:10.1029/2004JD005350, 2005. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Fromm, M., Tupper, A., Rosenfeld, D., Servanckx, R., and McRae, R.: Violent pyro-convective storm devastates Australia&apos;s capital and pollutes the stratosphere, Geophys. Res. Lett., 33, L05815, doi:10.1029/2005GL025161, 2006. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Gleason, J. F., Hsu, N. C., and Torres, O.: Biomass burning smoke measured using backscattered ultraviolet radiation: SCAR-B and Brazilian smoke interannual variability, J. Geophys. Res., 103(D24), 31969–31978, 1998. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Goldstein, A. H., Koven, C. D., Heald, C. L., and Fung, I. Y.: Biogenic carbon and anthropogenic pollutants combine to form a cooling haze over the southeastern United States, Proc. Nat. Acad. Sci. 106, 8835–8840, doi:10.1073/PNAS.0904128106, 2009. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Grzegorski, M., Wenig, M., Platt, U., Stammes, P., Fournier, N., and Wagner, T.: The Heidelberg iterative cloud retrieval utilities (HICRU) and its application to GOME data, Atmos. Chem. Phys., 6, 4461–4476, 2006. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Herman, J. R., Bhartia, P. K., Torres, O., Hsu, C., Seftor, C., and Celarier, E.: Global distribution of UV-absorbing aerosols from Nimbus 7/TOMS data, J. Geophys. Res., 102(D14), 16911–16922, 1997. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Holben, B. N., Eck, T. F., Slutsker, I., Tanré, D., Buis, J. P., Setzer, A., Vermote, E., Raegan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F., Jankowiak, I., and Smirnov, A.: AERONET – A federated instrument network and data archive for aerosol characterization, Remote Sens. Environ., 66, 1–16, 1998. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Hsu, N. C., Herman, J. R., Bhartia, P. K., Seftor, C. J., Torres, O., Thompson, A. M., Gleason, J. F., Eck, T. F., and Holben, B. N.: Detection of biomass burning smoke from TOMS measurements, Geophys. Res. Lett., 23(7), 745–748, 1996. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Hsu, N., Herman, J., Torres, O., Holben, B., Tanre, D., Eck, T., Smirnov, A., Chatenet, B., and Lavenu, F.: Comparisons of the TOMS aerosol index with Sun-photometer aerosol optical thickness: Results and applications, J. Geophys. Res., 104(D6), 6269–6279, 1999. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Hsu, N. C., Herman, J. R., and Tsay, S.-C.: Radiative impacts from biomass burning in the presence of clouds during boreal spring in southeast Asia, Geophys. Res. Lett., 30, 1224, doi:10.1029/2002GL016485, 2003. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Kirchstetter, T. W., Novakov, T., and Hobbs, P. V.: Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon, J. Geophys. Res., 109, D21208, doi:10.1029/2004JD004999, 2004. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Koelemeijer, R. B. A., Stammes, P., Hovenier, J. W., de Haan, J. F.: A fast method for retrieval of cloud parameters using oxygen A band measurements from the Global Ozone Monitoring Experiment, J. Geophys. Res., 106, 3475–3490, 2001. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Mahowald, N. M. and Dufresne, J.-L.: Sensitivity of TOMS aerosol index to boundary layer height: Implications for detection of mineral aerosol sources, Geophys. Res. Lett., 31, L03103, doi:10.1029/2003GL018865, 2004. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Mishchenko, M. I., Lacis, A. A., and Travis, L. D.: Errors induced by the neglect of polarisation in radiance calculations for Rayleigh-scattering atmospheres, J. Quant. Spectrosc. Radiat. Transfer, 51(3), 491–510, 1994. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Platt, U.: Differential Optical Absorption Spectroscopy (DOAS), in: Air monitoring by spectrometric techniques, edited by: Sigrist, M., pp. 27–84, John Wiley, New York, 1994. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Rozanov, V. V., Buchwitz, M., Eichmann, K.-U., de Beek, R., and Burrows, J. P.: SCIATRAN – A new radiative transfer model for geophysical applications in the 240–2400 nm spectral region: the pseudo-spherical version, Adv. Space Res., 29(11), 1831–1835, 2002. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Rozanov, A., Rozanov, V., Buchwitz, M., Kokhanovsky, A., and Burrows, J. P.: SCIATRAN 2.0 – A new radiative transfer model for geophysical applications in the 175–2400 nm spectral region, Adv. Space Res., 36, 1015–1019, 2005. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Tilstra, L. G., de Graaf, M., No\&quot;el, S., Aben, I., and Stammes, P.: SCIAMACHY&apos;s Absorbing Aerosol Index and the consequences of instrument degradation, Proc. ACVE-3, 2007 </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Tilstra, L. G.: SCIAMACHY Absorbing Aerosol Index Algorithm Theoretical Basis Document, SRON-EOS-RP-08-023, 2008. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Torres, O., Bhartia, P. K., Herman, J. R., Ahmad, Z., and Gleason, J.: Derivation of aerosol properties from satellite measurements of backscattered ultraviolet radiation: Theoretical basis, J. Geophys. Res., 103(D14), 17099–17110, 1998. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Torres O., Tanskanen, A., Veihelmann, B., Ahn, C., Braak, R., Bhartia, P. K., Veefkind, P., and Levelt, P.: Aerosols and surface UV products from Ozone Monitoring Instrument observations: An overview, J. Geophys. Res., 112, D24S47, doi:10.1029/2007JD008809, 2007. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> van Diedenhoven, B., Hasekamp, O. P., and Aben, I.: Surface pressure retrieval from SCIAMACHY measurements in the O&lt;sub&gt;2&lt;/sub&gt; A Band: validation of the measurements and sensitivity on aerosols, Atmos. Chem. Phys., 5, 2109–2120, 2005. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Wagner, T., Dix, B., v. Friedeburg, C., Friess, U., Sanghavi, S., Sinreich, R., and Platt, U.: MAX-DOAS O&lt;sub&gt;4&lt;/sub&gt; measurements – A new technique to derive information on atmospheric aerosols, J. Geophys. Res., 109, D22205, doi:10.1029/2004JD004904, 2004. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Wagner, T., Beirle, S., Deutschmann, T., Eigemeier, E., Frankenberg, C., Grzegorski, M., Liu, C., Marbach, T., Platt, U., and Penning de Vries, M.: Monitoring of atmospheric trace gases, clouds, aerosols and surface properties from UV/vis/NIR satellite instruments, J. Opt. A: Pure Appl. Opt., 10, 104019, doi:10.1088/1464-4258/10/10/104019, 2008. </mixed-citation>
</ref>
</ref-list>
</back>
</article>