Atmos. Chem. Phys. Discuss., 9, 135-173, 2009
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Time-span and spatial-scale of regional new particle formation events over Finland and Southern Sweden
T. Hussein1, H. Junninen1, P. Tunved2, A. Kristensson3,4, M. Dal Maso1, I. Riipinen1, P. P. Aalto1, H.-C. Hansson4, E. Swietlicki2, and M. Kulmala1
1University of Helsinki, Department of Physics, Helsinki, Finland
2Institute for Applied Environmental Research, Stockholm University, Stockholm, Sweden
3Lund University, Division of Nuclear Physics, Lund, Sweden
4University of Copenhagen, Department of Chemistry, Copenhagen Centre for Atmospheric Research (CCAR), Copenhagen, Denmark

Abstract. We investigated the time-span and spatial-scale of regional new particle formation (NPF) events in Finland and Southern Sweden using measured particle number size distributions at five background stations. We define the time-span of a NPF event as the time period from the first moment when the newly formed mode of aerosol particles is observable below 25 nm until the newly formed mode is not any more distinguishable from other modes of aerosol particles after growing to bigger sizes. We identified the spatial-scale of regional NPF events based on two independent approaches. The first approach is based on the observation within a network of stationary measurement stations, and the second approach is based on the time-span and the history of back-trajectories. According to the second approach, about 60% and 28% of the events can be traced to distances longer than 220 km upwind from where the events were observed in southern Finland (Hyytiälä) and northern Finland (Värriö). The analysis also showed that the observed regional NPF events started over the continents or over major ship routes but not over the Atlantic Ocean. The first approach showed that although large spatial-scale NPF events are frequently observed at several locations simultaneously, they are rarely identical (similar characteristics and temporal variations) due to differences in the initial meteorological and geographical conditions between the stations. On median, the growth of the newly formed particles during large spatial-scale NPF events can be followed for more than 30 h where the newly formed aerosol particles end up in the Aitken mode and accumulation mode size ranges (diameter >25 nm). This study showed clear evidences that regional NPF events can pose a significant source for accumulation mode particles over the European continent provided that these findings can be generalized to many of the air parcels traveling over the European continent.

Citation: Hussein, T., Junninen, H., Tunved, P., Kristensson, A., Dal Maso, M., Riipinen, I., Aalto, P. P., Hansson, H.-C., Swietlicki, E., and Kulmala, M.: Time-span and spatial-scale of regional new particle formation events over Finland and Southern Sweden, Atmos. Chem. Phys. Discuss., 9, 135-173, doi:10.5194/acpd-9-135-2009, 2009.
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