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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>9</volume_number>
		<issue_number>3</issue_number>
		<publication_year>2009</publication_year>
	</journal>
	<doi>10.5194/acpd-9-12731-2009</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/9/12731/2009/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/9/12731/2009/acpd-9-12731-2009.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/9/12731/2009/acpd-9-12731-2009.pdf</fulltext_pdf>
	<start_page>12731</start_page>
	<end_page>12779</end_page>
	<publication_date>2009-06-04</publication_date>
	<article_title content_type="html">Aerosol indirect effects â€“ general circulation model intercomparison and evaluation with satellite data</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>J. Quaas</name>
			<email>johannes.quaas@zmaw.de</email>
		</author>
		<author numeration="2" affiliations="2">
			<name>Y. Ming</name>
		</author>
		<author numeration="3" affiliations="3,4">
			<name>S. Menon</name>
		</author>
		<author numeration="4" affiliations="5">
			<name>T. Takemura</name>
		</author>
		<author numeration="5" affiliations="6">
			<name>M. Wang</name>
		</author>
		<author numeration="6" affiliations="6">
			<name>J. E. Penner</name>
		</author>
		<author numeration="7" affiliations="7">
			<name>A. Gettelman</name>
		</author>
		<author numeration="8" affiliations="8">
			<name>U. Lohmann</name>
		</author>
		<author numeration="9" affiliations="9">
			<name>N. Bellouin</name>
		</author>
		<author numeration="10" affiliations="9">
			<name>O. Boucher</name>
		</author>
		<author numeration="11" affiliations="10">
			<name>A. M. Sayer</name>
		</author>
		<author numeration="12" affiliations="10">
			<name>G. E. Thomas</name>
		</author>
		<author numeration="13" affiliations="11">
			<name>A. McComiskey</name>
		</author>
		<author numeration="14" affiliations="11">
			<name>G. Feingold</name>
		</author>
		<author numeration="15" affiliations="12">
			<name>C. Hoose</name>
		</author>
		<author numeration="16" affiliations="12">
			<name>J. E. KristjÃ¡nsson</name>
		</author>
		<author numeration="17" affiliations="13">
			<name>X. Liu</name>
		</author>
		<author numeration="18" affiliations="14">
			<name>Y. Balkanski</name>
		</author>
		<author numeration="19" affiliations="2">
			<name>L. J. Donner</name>
		</author>
		<author numeration="20" affiliations="2">
			<name>P. A. Ginoux</name>
		</author>
		<author numeration="21" affiliations="10">
			<name>P. Stier</name>
		</author>
		<author numeration="22" affiliations="1">
			<name>J. Feichter</name>
		</author>
		<author numeration="23" affiliations="3">
			<name>I. Sednev</name>
		</author>
		<author numeration="24" affiliations="4">
			<name>S. E. Bauer</name>
		</author>
		<author numeration="25" affiliations="4">
			<name>D. Koch</name>
		</author>
		<author numeration="26" affiliations="10">
			<name>R. G. Grainger</name>
		</author>
		<author numeration="27" affiliations="15">
			<name>A. Kirkev&amp;aring;g</name>
		</author>
		<author numeration="28" affiliations="12,15">
			<name>T. Iversen</name>
		</author>
		<author numeration="29" affiliations="15">
			<name>Ã˜. Seland</name>
		</author>
		<author numeration="30" affiliations="13">
			<name>R. Easter</name>
		</author>
		<author numeration="31" affiliations="13">
			<name>S. J. Ghan</name>
		</author>
		<author numeration="32" affiliations="13">
			<name>P. J. Rasch</name>
		</author>
		<author numeration="33" affiliations="7">
			<name>H. Morrison</name>
		</author>
		<author numeration="34" affiliations="7">
			<name>J.-F. Lamarque</name>
		</author>
		<author numeration="35" affiliations="16">
			<name>M. J. Iacono</name>
		</author>
		<author numeration="36" affiliations="1">
			<name>S. Kinne</name>
		</author>
		<author numeration="37" affiliations="14">
			<name>M. Schulz</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Max Planck Institute for Meteorology, Hamburg, Germany</affiliation>
		<affiliation numeration="2" content_type="html">Geophysical Fluid Dynamics Laboratory/NOAA, Princeton, USA</affiliation>
		<affiliation numeration="3" content_type="html">Lawrence Berkeley National Laboratory, Berkeley, USA</affiliation>
		<affiliation numeration="4" content_type="html">Goddard Institute for Space Studies/NASA, New York, USA</affiliation>
		<affiliation numeration="5" content_type="html">Kyushu University, Fukoka, Japan</affiliation>
		<affiliation numeration="6" content_type="html">University of Michigan, Ann Arbor, USA</affiliation>
		<affiliation numeration="7" content_type="html">National Center for Atmospheric Research, Boulder, USA</affiliation>
		<affiliation numeration="8" content_type="html">Institute for Atmospheric and Climate Science/ETH Zurich, Switzerland</affiliation>
		<affiliation numeration="9" content_type="html">Met Office Hadley Centre, Exeter, UK</affiliation>
		<affiliation numeration="10" content_type="html">Atmospheric, Oceanic and Planetary Physics, University of Oxford, UK</affiliation>
		<affiliation numeration="11" content_type="html">NOAA Earth System Research Laboratory, Boulder, USA</affiliation>
		<affiliation numeration="12" content_type="html">Department of Geosciences, University of Oslo, Norway</affiliation>
		<affiliation numeration="13" content_type="html">Pacific Northwest National Laboratory, Richland, USA</affiliation>
		<affiliation numeration="14" content_type="html">Laboratoire des Sciences du Climat et de l&apos;Environnement/IPSL, Gif-sur-Yvette, France</affiliation>
		<affiliation numeration="15" content_type="html">Norwegian Meteorological Institute, Oslo, Norway</affiliation>
		<affiliation numeration="16" content_type="html">Atmospheric and Environmental Research, Inc., Lexington, USA</affiliation>
	</affiliations>
	<abstract content_type="html">Aerosol indirect effects continue to constitute one of the most
important uncertainties for anthropogenic climate perturbations. Within the
international AEROCOM initiative, the representation of
aerosol-cloud-radiation interactions in ten different general circulation
models (GCMs) is evaluated using three satellite datasets. The focus is on
stratiform liquid water clouds since most GCMs do not include ice nucleation
effects, and none of the models explicitly parameterizes aerosol effects on
convective clouds. We compute statistical relationships between aerosol
optical depth (Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt;) and various cloud
and radiation quantities in a manner that is consistent between the models
and the satellite data. It is found that the model-simulated influence of
aerosols on cloud droplet number concentration
(&lt;i&gt;N&lt;sub&gt;d&lt;/sub&gt;&lt;/i&gt;) compares relatively well to the
satellite data at least over the ocean. The relationship between
Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; and liquid water path is simulated
much too strongly by the models. It is shown that this is partly related to
the representation of the second aerosol indirect effect in terms of
autoconversion. A positive relationship between total cloud fraction
(&lt;i&gt;f&lt;/i&gt;&lt;sub&gt;cld&lt;/sub&gt;) and Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; as found in the satellite data is
simulated by the majority of the models, albeit less strongly than that in
the satellite data in most of them. In a discussion of the hypotheses
proposed in the literature to explain the satellite-derived strong
&lt;i&gt;f&lt;/i&gt;&lt;sub&gt;cld&lt;/sub&gt; â€“ Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; relationship, our results indicate that none can be identified as
unique explanation. Relationships similar to the ones found in satellite
data between Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; and cloud top
temperature or outgoing long-wave radiation (OLR) are simulated by only a
few GCMs. The GCMs that simulate a negative OLR â€“ Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; relationship show a strong positive correlation between
Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; and &lt;i&gt;f&lt;/i&gt;&lt;sub&gt;cld&lt;/sub&gt;. The short-wave total aerosol radiative
forcing as simulated by the GCMs is strongly influenced by the simulated
anthropogenic fraction of Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt;, and
parameterisation assumptions such as a lower bound on
&lt;i&gt;N&lt;sub&gt;d&lt;/sub&gt;&lt;/i&gt;. Nevertheless, the strengths of the
statistical relationships are good predictors for the aerosol forcings in
the models. An estimate of the total short-wave aerosol forcing inferred
from the combination of these predictors for the modelled forcings with the
satellite-derived statistical relationships yields a global annual mean
value of &amp;minus;1.5&amp;plusmn;0.5 Wm&lt;sup&gt;&amp;minus;2&lt;/sup&gt;. An alternative estimate obtained
by scaling the simulated clear- and cloudy-sky forcings with estimates of
anthropogenic Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; and
satellite-retrieved &lt;i&gt;N&lt;sub&gt;d&lt;/sub&gt;&lt;/i&gt; â€“ Ï„&lt;sub&gt;&lt;i&gt;a&lt;/i&gt;&lt;/sub&gt; regression slopes, respectively,
yields a global annual mean clear-sky (aerosol direct effect) estimate of
&amp;minus;0.4&amp;plusmn;0.2 Wm&lt;sup&gt;&amp;minus;2&lt;/sup&gt; and a cloudy-sky (aerosol indirect effect)
estimate of &amp;minus;0.7&amp;plusmn;0.5 Wm&lt;sup&gt;&amp;minus;2&lt;/sup&gt;, with a total estimate of
&amp;minus;1.2&amp;plusmn;0.4 Wm&lt;sup&gt;&amp;minus;2&lt;/sup&gt;.</abstract>
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