Atmos. Chem. Phys. Discuss., 8, 8715-8742, 2008
www.atmos-chem-phys-discuss.net/8/8715/2008/
doi:10.5194/acpd-8-8715-2008
© Author(s) 2008. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Asian dust outflow in the PBL and free atmosphere retrieved by NASA CALIPSO and an assimilated dust transport model
Y. Hara1, K. Yumimoto2, I. Uno3, A. Shimizu1, N. Sugimoto1, Z. Liu4, and D. M. Winker5
1National Institute for Environmental Study, Tsukuba, Ibaraki, Japan
2Dept. of Earth System Science and Tech., Kyushu University, Fukuoka, Japan
3Research Institute for Applied Mechanics, Kyushu University, Fukuoka, Japan
4National Institute of Aerospace, Hampton, VA 23666, USA
5NASA Langley Research Center, Hampton, VA23681, USA

Abstract. Three-dimensional structures of Asian dust transport in the planetary boundary layer (PBL) and free atmosphere occurring successively during the end of May 2007 were clarified using results of space-borne backscatter lidar, Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), and results simulated using a data-assimilated version of a dust transport model (RC4) based on a ground-based NIES lidar network. Assimilated results mitigated overestimation of dust concentration by reducing 17.4% of dust emissions and improved the root mean square difference (RMSD) of dust AOT between the model and NIES lidar by 31.2–66.9%. The dust layer depths, vertical and horizontal structure simulated by RC4 agreed with CALIOP from the dust source region to a long-range downwind region for which 3-D distribution of dust clouds had not been clarified previously. Based on CALIOP and RC4, two significant transport mechanisms of Asian dust in the PBL and free atmosphere were clarified: a low level dust outbreak within the dry slot region of a well developed low-pressure system, and formation of an elevated dust layer within the warm sector of a low-pressure system. Finally, the aging of pure dust particles was investigated using the particle depolarization ratio (PDR) at 532 nm and the color ratio (CR) at 1064 nm and 532 nm for the low-altitude dust transport case. Aerosols with high PDR were observed uniformly over the dust source region. As the dust cloud was transported to the eastern downwind regions, aerosols with low PDR and high CR were found in the layer of less than 1 km height, suggesting changes from the external to internal mixing state of spherical aerosols and dust in the surface layer.

Citation: Hara, Y., Yumimoto, K., Uno, I., Shimizu, A., Sugimoto, N., Liu, Z., and Winker, D. M.: Asian dust outflow in the PBL and free atmosphere retrieved by NASA CALIPSO and an assimilated dust transport model, Atmos. Chem. Phys. Discuss., 8, 8715-8742, doi:10.5194/acpd-8-8715-2008, 2008.
 
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