<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys-discuss.net/inc/acpd/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>8</volume_number>
		<issue_number>3</issue_number>
		<publication_year>2008</publication_year>
	</journal>
	<doi>10.5194/acpd-8-8585-2008</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/8/8585/2008/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/8/8585/2008/acpd-8-8585-2008.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/8/8585/2008/acpd-8-8585-2008.pdf</fulltext_pdf>
	<start_page>8585</start_page>
	<end_page>8628</end_page>
	<publication_date>2008-05-09</publication_date>
	<article_title content_type="html">Direct SW aerosol radiative forcing over Portugal</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>D. Santos</name>
			<email>dinas@uevora.pt</email>
		</author>
		<author numeration="2" affiliations="1,2">
			<name>M. J. Costa</name>
		</author>
		<author numeration="3" affiliations="1,2">
			<name>A. M. Silva</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Geophysics Centre of Évora, Univ. Évora, Évora, Portugal</affiliation>
		<affiliation numeration="2" content_type="html">Departament of Physics, Univ. Évora, Évora, Portugal</affiliation>
	</affiliations>
	<abstract content_type="html">The estimation of radiative forcing due to desert dust and forest fires
aerosols is a very important issue since these particles are very efficient
at scattering and absorbing both short and longwave radiation. In this work,
the evaluation of the aerosol radiative forcing at the top of the atmosphere
over the south of Portugal is made, particularly in the regions of Évora
and of Cabo da Roca.
&lt;br&gt;&lt;/br&gt;
The radiative transfer calculations combine ground-based and satellite
measurements, to estimate the top of the atmosphere direct SW aerosol
radiative forcing. The method developed to retrieve the surface spectral
reflectance is also presented, based on ground-based measurements of the
aerosol optical properties combined with the satellite-measured radiances.
&lt;br&gt;&lt;/br&gt;
The aerosol direct radiative effect is shown to be very sensitive to the
underlying surface, since different surface spectral reflectance values may
originate different forcing values. The results obtained also illustrate the
importance of considering the actual aerosol properties, in this case
measured by ground-based instrumentation, particularly the aerosol single
scattering albedo, because different aerosol single scattering albedo values
can flip the sign of the direct SW aerosol radiative forcing.
&lt;br&gt;&lt;/br&gt;
The instantaneous direct SW aerosol radiative forcing values obtained at the top of the
atmosphere are, in the majority of the cases, negative, indicating a tendency for cooling the
Earth. For Desert Dust aerosols, over Évora land region, the average forcing efficiency is
estimated to be &amp;minus;25 W/m&lt;sup&gt;2&lt;/sup&gt;/AOT&lt;sub&gt;0.55&lt;/sub&gt; whereas for Cabo da Roca area, the average forcing
efficiency is &amp;minus;46 W/m&lt;sup&gt;2&lt;/sup&gt;/AOT&lt;sub&gt;0.55&lt;/sub&gt;. In the presence of Forest Fire aerosols, over Cabo da Roca
region, the average value of forcing efficiency is &amp;minus;28 W/m&lt;sup&gt;2&lt;/sup&gt;/AOT&lt;sub&gt;0.55&lt;/sub&gt; and over Évora region an
average value of &amp;minus;33 W/m&lt;sup&gt;2&lt;/sup&gt;/AOT&lt;sub&gt;0.55&lt;/sub&gt; is found.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Andreae, M. and Merlet, P.: Emission of trace gases and aerosols from biomass burning, Glob. Biogeochem. Cy., 15, 955&amp;ndash;966, 2001. </reference>
		<reference numeration="2" content_type="text"> Barnes, W. L., Pagano, T. S., and Salomonson, V. V.: Prelaunch characteristics of the MODerate Resolution Imaging Spectroradiometer (MODIS) on EOS-AM1, IEEE Trans. Geosci. Remote Sens., 36, 1088&amp;ndash;1100, 1998. </reference>
		<reference numeration="3" content_type="text"> Christopher, S. A., Li, X., Welch, R. M., Reid, J. S., Hobbs, P. V., Eck, T. F., and Holben, B.: Estimation of Surface and Top-of-Atmosphere Shortwave Irradiance in Biomass-Burning Regions during SCAR-B, J. Appl. Meteorol., 39, 1742&amp;ndash;1753, 1999. </reference>
		<reference numeration="4" content_type="text"> Costa, M. J.: Aerosol and cloud satellite remote sensing: monitoring and modelling using passive sensors. Ph.D. thesis, Dep. Physics, Univ. Évora, Portugal, 233 pp., 2004. </reference>
		<reference numeration="5" content_type="text"> Costa, M. J., Silva, A. M., and Levizzani, V.: Aerosol Characterization and Direct Radiative Forcing Assessment over the Ocean. Part I: Methodology and Sensitivity Analysis, J. Appl. Meteorol., 43, 1799&amp;ndash;1817, 2004. </reference>
		<reference numeration="6" content_type="text"> Costa, M. J., Sohn, B. J., Levizzani, V., and Silva, A. M.: Radiative Forcing of Asian Dust Determined from the Synergized GOME and GMS Satellite Data&amp;ndash;A Case Study, J. Meteorol. Soc. Jpn., 84, 85&amp;ndash;95, 2006. </reference>
		<reference numeration="7" content_type="text"> DGRF, Divisão de Defesa da Floresta contra incêndios: Incêndios Florestais Relatório de 2005, 26 pp., 2006. </reference>
		<reference numeration="8" content_type="text"> Draxler, R. R. and Hess, G. D.: An overview of the Hysplit_4 modelling system for trajectories, Aust. Meteorol. Mag., 47, 295&amp;ndash;308, 1998. </reference>
		<reference numeration="9" content_type="text"> Dubovik, O. and King, M.: A flexible inversion algorithm for retrieval of aerosol optical properties from Sun and sky radiance measurements, J. Geophys. Res., 105, 20 673&amp;ndash;20 696, 2000. </reference>
		<reference numeration="10" content_type="text"> Dubovik, O., Smirnov, A., Holben, B. N., King, M., Kaufman, Y. J., Eck, T. F., and Slutsker, I.: Accuracy assessment of aerosol optical properties retrieval from AERONET Sun and sky radiance measurements, J. Geophys. Res., 105, 9791&amp;ndash;9806, 2000. </reference>
		<reference numeration="11" content_type="text"> Eck, T. F., Holben, B., Sluster, I., and Setzer, A.: Characterization of the optical properties of biomass burning aerosols in Zambia during the 1997 ZIBBEE field campaign, J. Geophys. Res., 106, 3425&amp;ndash;3448, 2001. </reference>
		<reference numeration="12" content_type="text"> Elias, T., Silva, A. M., Figueira, M. J., Belo, N., Pereira, S., Formenti, P., and Helas, G.: Aerosol extinction and absorption in: Évora, Portugal, during the European 2003 summer heat wave. Remote Sensing of Clouds and the Atmosphere IX., edited by: Schäfer, K. P., Comerón, A., Carleer, M. R., Picard, R. H., and Sifakis, N. I., Proceedings of the SPIE, 5571, 270&amp;ndash;281, 2004. </reference>
		<reference numeration="13" content_type="text"> Elias, T., Silva, A. M., Belo, N., Pereira, S., Formenti, P., Helas, G., and Wagner, F.: Aerosol extinction in a remote continental region of the Iberian Peninsula during summer, J. Geophys. Res., 111, D14204, doi:10.1029/2005JD006610, 2006. </reference>
		<reference numeration="14" content_type="text"> Hansen, J. E., Sato, M., and Ruedy, R.: Radiative forcing and climate response. J. Geophys. Res., 102, 6831&amp;ndash;6864, 1997. </reference>
		<reference numeration="15" content_type="text"> Haywood, J. P. and Shine, K. P.: The effect of anthropogenic sulfate and soot aerosols on clear sky planetary radiation budget, Geophys. Res. Lett., 22, 603&amp;ndash;606, 1995. </reference>
		<reference numeration="16" content_type="text"> Haywood, J. and Boucher, O.: estimates of the direct and indirect radiative forcing due to tropospheric aerosols; a review. Rev. Geophys., 38, 513&amp;ndash;543, 2000. </reference>
		<reference numeration="17" content_type="text"> Holben, B., Eck, T. F., Slutsker, I., Tanre, D., Buis, J. P., Setzer, A., Vermote, E., Reagan, J.A., Kaufman, Y., Nakajima, T., Lavenu, F., Jankowiak, I, and Smirnov, A.: AERONET-A federated instrument network and data archived for aerosol characterization, Remote Sens. Environ., 66, 1&amp;ndash;16, 1998. </reference>
		<reference numeration="18" content_type="text"> Holben, B., N., Tanre, D., Smirnov, A., Eck, T. F., Slutsker, I., Abuhassan, N., Newcomb, W. W., Schafer, J., Chatenet, B., Lavenue, F., Kaufman, Y. J., Castle, J., Setzer, A., Markham, B., Clark, D., Frouin, R., Halthore, R., Karnieli, A., O&apos;Neill, N. T., Pietras, C., Pinker, R.T., Voss, K., and Zibordi, G.: An emerging ground-based aerosol climatology: Aerosol optical depth from AERONET, J. Geophys. Res., 106, 12 067&amp;ndash;12 097, 2001. </reference>
		<reference numeration="19" content_type="text"> IPCC: Climate Change 2007: The Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L. (eds.), Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 996 pp., 2007. </reference>
		<reference numeration="20" content_type="text"> Kaufman, Y. J., Tanré, D., and Boucher, O.: A satellite view of aerosols in the climate system, Nature, 419, 215&amp;ndash;223, 2002. </reference>
		<reference numeration="21" content_type="text"> Liao, H. and Seinfeld, J. H.: Radiative forcing by mineral dust aerosols: sensitivity to key variables, J. Geophys. Res., 103, 31 637&amp;ndash;31 645, 1998. </reference>
		<reference numeration="22" content_type="text"> Ramos A. M.: Modela&amp;#x00E7;ão Numérica do Transporte de Poluentes Atmosféricos em Portugal e suas Rela&amp;#x00E7;ões com as Condi&amp;#x00E7;ões Meteorológicas. Ph.D. thesis, Dep. Physics, Univ. Évora, Portugal, 233 pp., 2006. </reference>
		<reference numeration="23" content_type="text"> Reid, J. S. and Hobbs, P. V.: Physical and optical properties of young smoke from individual biomass fires in Brazil. J. Geophys. Res., 103, 32 013&amp;ndash;32 031, 1998. </reference>
		<reference numeration="24" content_type="text"> Russel, P. B., Redemann, J., Schmid, B., Bergstrom, R. W., Livingston, J. M., McIntosh, D. M., Ramirez, S. A., Hartley, S. A., Hobbs, P. V., Quinn, P. K., Carrico, C. M., Rood, M. J., Ostrom, E., Noone, K. J., von Hoyningen-Huene, W., and Remer, L.: Comparison of aerosol single scattering albedos derived by diverse technique in two North Atlantic experiments, J. Atmos. Sci., 59, 609&amp;ndash;619, 2002. </reference>
		<reference numeration="25" content_type="text"> Satheesh, S. K.: Aerosol radiative forcing over land: effect of surface and cloud reflection. Ann. Geophys. 20, 2105&amp;ndash;2109, 2002. </reference>
		<reference numeration="26" content_type="text"> Silva, A. M., Costa M. J., Elias, T., Formenti, P., Belo, N., and Pereira, S.: Ground based aerosol monitoring at Évora, Portugal, Global Change Newsletter, 56, 6&amp;ndash;9, 2003. </reference>
		<reference numeration="27" content_type="text"> Takemura, T., Nakajima, T., Dubovik, O., Holben, B. N., and Kinne, S.: Single scattering albedo and radiative forcing of various aerosol species with a global three dimensional model, J. Climate, 15, 333&amp;ndash;352, 2002. </reference>
		<reference numeration="28" content_type="text"> Tegen, I. and Lacis, A. A.: Modeling of particle size distribution and its influence on the radiative properties of mineral dust aerosol, J. Geophys. Res., 101, 19 237&amp;ndash;19 244, 1996. </reference>
		<reference numeration="29" content_type="text"> Vermote, E. F., Tanré, D., Deuze, J.-L., Herman, M., and Morcrette, J.-J.,: Second simulation of the satellite signal in the solar spectrum: An overview, IEEE Trans. Geosci. Remote Sens., 35, 675&amp;ndash;686, 1997a. </reference>
		<reference numeration="30" content_type="text"> Vermote, E. F., Tanré, D., Deuze, J.-L., Herman, M., and Morcrette, J.-J.: Second simulation of the satellite signal in the solar spectrum: User guide Version 2, 218 pp., 1997b. </reference>
		<reference numeration="31" content_type="text"> Verver, G., Raes, F., Vogelezang, D., and Johnson, D.: The 2nd Aerosol Characterization experiment: meteorological and chemical overview, Tellus, 52B, 126&amp;ndash;140, 2000. </reference>
	</references>
</article>

