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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>8</volume_number>
		<issue_number>4</issue_number>
		<publication_year>2008</publication_year>
	</journal>
	<doi>10.5194/acpd-8-16027-2008</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/8/16027/2008/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/8/16027/2008/acpd-8-16027-2008.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/8/16027/2008/acpd-8-16027-2008.pdf</fulltext_pdf>
	<start_page>16027</start_page>
	<end_page>16059</end_page>
	<publication_date>2008-08-22</publication_date>
	<article_title content_type="html">Global error maps of aerosol optical properties: an error propagation analysis</article_title>
	<authors>
		<author numeration="1" affiliations="1,3">
			<name>K. Tsigaridis</name>
			<email>ktsigaridis@giss.nasa.gov</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>Y. Balkanski</name>
		</author>
		<author numeration="3" affiliations="1">
			<name>M. Schulz</name>
		</author>
		<author numeration="4" affiliations="2">
			<name>A. Benedetti</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Lab. des Sciences du Climat et de l&apos;Environnement (LSCE), 91191 Gif-sur-Yvette, France</affiliation>
		<affiliation numeration="2" content_type="html">European Center for Medium Range Weather Forecasts (ECMWF), Reading, UK</affiliation>
		<affiliation numeration="3" content_type="html">now at: NASA Goddard Institute for Space Studies (GISS), 2880 Broadway, NY 10025, USA</affiliation>
	</affiliations>
	<abstract content_type="html">Among the numerous atmospheric constituents, aerosols play a unique role on
climate, due to their scattering and absorbing capabilities, visibility
degradation and their effect on incoming and outgoing radiation. The most
important optical properties are the aerosol optical depth (AOD), the
asymmetry parameter (&lt;I&gt;g&lt;/I&gt;) and the single scattering albedo (SSA). Uncertainties
in aerosol microphysics in global models, which in turn affect their optical
properties, propagate to uncertainties on the effect of aerosols on climate.
This study aims to estimate the uncertainty of AOD, &lt;I&gt;g&lt;/I&gt; and SSA attributable to
the aerosol representation in models, namely mixing state, aerosol size and
aerosol associated water. As a reference, the monthly mean output of the
general circulation model LMDz-INCA from the international comparison
exercise AEROCOM B was used. For the optical properties calculations,
aerosols were considered either externally mixed, homogeneously internally
mixed or coated spheres. The radius was allowed to vary by &amp;plusmn;20%
(with 2% intervals) and the aerosol water content by &amp;plusmn;50% (with
5% intervals) with respect to the reference model output. All of these
possible combinations were assumed to be equally likely and the optical
properties were calculated for each one of them. A probability density
function (PDF) was constructed at each model grid point for AOD, &lt;I&gt;g&lt;/I&gt; and SSA.
From this PDF, the 1σ and 2σ uncertainties of the AOD, &lt;I&gt;g&lt;/I&gt; and SSA were
calculated and are available as global maps for each month. For the range of
the cases studied, we derive a maximum 2σ uncertainty range in AOD of 70%,
while for &lt;I&gt;g&lt;/I&gt; and SSA the maxima reach 18% and 28% respectively. The
mixing state was calculated to be important, with the aerosol absorption and
SSA being the most affected properties when absorbing aerosols are present.</abstract>
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</article>

