Atmos. Chem. Phys. Discuss., 8, 15463-15490, 2008
© Author(s) 2008. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Hydration of the lower stratosphere by ice crystal geysers over land convective systems
S. Khaykin1, J.-P. Pommereau2, L. Korshunov1, V. Yushkov1, J. Nielsen3, N. Larsen3, T. Christensen3, A. Garnier2, A. Lukyanov1, and E. Williams4
1Central Aerological Observatory of Roshydromet 3, Pervomayskaya str. Dolgoprudny, Moscow region, Russian Federation, 141700, Russia
2Service d'Aeronomie, CNRS, University of Versailles St Quentin, BP 3, Verrières le Buisson 91371, France
3Danish Meteorological Institute, Lyngbyvej 100, 2100 Copenhagen, Denmark
4Dept. of Civil & Environmental Engineering, Massachusetts Institute of Technology, 77 Massachusetts Ave., Cambridge, MA 02139-4307, USA

Abstract. The possible impact of deep convective overshooting over land has been explored by six simultaneous soundings of water vapour, particles and ozone in the lower stratosphere next to MesoScale Convective Systems (MCSs) during the monsoon season over West Africa in Niamey, Niger in August 2006. The water vapour measurements were carried out using a fast response FLASH-B Lyman-alpha hygrometer. The high vertical resolution observations of this instrument show the presence of enhanced water vapour layers between the tropopause at 370 K and the 450 K level. Most of these moist layers are shown connected with overshooting events occurring upwind as identified from satellite IR images, over which the air mass probed by the sondes passed during the three previous days. In the case of a local overshoot identified by echo top turrets up to 18.5 km by the MIT C-band radar also in Niamey, tight coincidence was found between enhanced water vapour, ice crystal and ozone dip layers indicative of fast uplift of tropospheric air across the tropopause. The water vapour mixing ratio in the enriched layers, up to 8 ppmv higher than that of saturation at the tropopause, and the coincidence with the presence of ice crystals strongly suggest hydration of the lower stratosphere by geyser-like injection of ice particles over overshooting turrets. The pile-like structure of the water vapour seen by the high-resolution hygrometer in contrast to smooth profiles reported by a coarse vertical-resolution satellite observation, suggests that the hydration mechanism described above may be responsible for the known summer seasonal increase of moisture in the lower stratosphere. If this interpretation is correct, hydration by ice geysers across the tropopause may be an important contributor to the stratospheric water vapour budget.

Citation: Khaykin, S., Pommereau, J.-P., Korshunov, L., Yushkov, V., Nielsen, J., Larsen, N., Christensen, T., Garnier, A., Lukyanov, A., and Williams, E.: Hydration of the lower stratosphere by ice crystal geysers over land convective systems, Atmos. Chem. Phys. Discuss., 8, 15463-15490, doi:10.5194/acpd-8-15463-2008, 2008.
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