<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-8-14717-2008</article-id>
<title-group>
<article-title>Diffusional and accretional growth of water drops in a rising adiabatic parcel: effects of the turbulent collision kernel</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Grabowski</surname>
<given-names>W. W.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Wang</surname>
<given-names>L.-P.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Mesoscale and Microscale Meteorology Division, National Center for Atmospheric Research, Boulder, CO 80307, USA</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Department of Mechanical Engineering, University of Delaware, Newark, DE 19716, USA</addr-line>
</aff>
<pub-date pub-type="epub">
<day>31</day>
<month>07</month>
<year>2008</year>
</pub-date>
<volume>8</volume>
<issue>4</issue>
<fpage>14717</fpage>
<lpage>14763</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/8/14717/2008/acpd-8-14717-2008.html">This article is available from http://www.atmos-chem-phys-discuss.net/8/14717/2008/acpd-8-14717-2008.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/8/14717/2008/acpd-8-14717-2008.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/8/14717/2008/acpd-8-14717-2008.pdf</self-uri>
<abstract>
<p>A large set of rising adiabatic parcel simulations is executed
to investigate the combined diffusional and accretional growth of
cloud droplets in maritime and continental conditions, and to assess
the impact of enhanced droplet collisions due to small-scale cloud
turbulence. The microphysical model applies the droplet number density
function to represent spectral evolution of cloud and rain/drizzle drops,
and various numbers of bins in the numerical implementation, ranging
from 40 to 320.  Simulations are performed applying two traditional
gravitational collection kernels and two kernels representing collisions
of cloud droplets in the turbulent environment, with turbulent kinetic
energy dissipation rates of 100 and 400 cm&lt;sup&gt;2&lt;/sup&gt; s&lt;sup&gt;&amp;minus;3&lt;/sup&gt;. The overall
result is that the rain initiation time significantly depends on the
number of bins used, with earlier initiation of rain when the number of
bins is low. This is explained as a combination of the increase of the
width of activated droplet spectrum and enhanced numerical spreading
of the spectrum during diffusional and collisional growth when the
number of model bins is low. Simulations applying around 300 bins seem
to produce rain at times which no longer depend on the number of bins,
but the activation spectra are unrealistically narrow. These results call
for an improved representation of droplet activation in numerical models
of the type used in this study.

&lt;br&gt;&lt;br&gt;

Despite the numerical effects that impact the rain initiation time
in different simulations, the turbulent speedup factor, the ratio
of the rain initiation time for the turbulent collection kernel and
the corresponding time for the gravitational kernel, is approximately
independent of aerosol characteristics, parcel vertical velocity, and the
number of bins used in the numerical model. The turbulent speedup factor
is in the range 0.75–0.85 and 0.60–0.75 for the turbulent kinetic
energy dissipation rates of 100 and 400 cm&lt;sup&gt;2&lt;/sup&gt; s&lt;sup&gt;&amp;minus;3&lt;/sup&gt;, respectively.</p>
</abstract>
<counts><page-count count="47"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Ayala, O., Rosa, B., Wang, L.-P., and Grabowski, W. W.: Effects of turbulence on the geometric collision rate of sedimenting droplets: Part 1. Results from direct numerical simulation, New J. Physics, in press, 2008a. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Ayala, A., Rosa, B., and Wang, L.-P.: Effects of turbulence on the geometric collision rate of sedimenting droplets: Part 2. Theory and parameterization, New J. Physics, in press, 2008b. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Beard, K. V.: Terminal velocity and shape of cloud and precipitation drops aloft, J. Atmos. Sci., 33, 851–864, 1976. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Berry, E. X. and Reinhardt, R. L.: An analysis of cloud drop growth by collection: Part I. Double distributions, J. Atmos. Sci., 31, 1814–1824, 1974. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Blyth, A. M.: Entrainment in cumulus clouds, J. Appl. Meteor., 32, 626–640, 1993. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Bott, A.: A flux method for the numerical solution of the stochastic collection equation, J. Atmos. Sci., 55, 2284–2293, 1998. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Brenguier, J.-L. and Chaumat, L.: Droplet spectra broadening in cumulus clouds. Part I: Broadening in adiabatic cores. framework, J. Atmos. Sci., 58, 628–641, 2001. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Chun, J., Koch, D., Rani, S. L., Ahluwalia, A., and Collins, L. R.: Clustering of aerosol particles in isotropic turbulence, J. Fluid Mech., 536, 219–251, 2005. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Clark, T. L.: On modelling nucleation and condensation theory in Eulerian spatial domain, J. Atmos. Sci., 31, 2099–2117, 1974. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Clark, T. L. and Hall, W. D.: A numerical experiment on stochastic condensation theory, J. Atmos. Sci., 36, 470–483, 1979. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Falkovich, G., Fouxon, A., and Stepanov, M. G.: Acceleration of rain initiation by cloud turbulence, Nature, 419, 151–154, 2002. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Ghosh, S., Davila, J., Hunt, J. C. R., Srdic, A., Fernando, H. J. S., and Jonas, P.: How turbulence enhances coalescence of settling particles with applications to rain in clouds, Proc. Roy. Soc. London, 461A, 3059–3088, 2005. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Grabowski, W. W.: Numerical experiments on the dynamics of the cloud-environment interface: small cumulus in a shear-free environment, J. Atmos. Sci., 46, 3513–3541, 1989. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Hall, W. D.: A detailed microphysical model within a two-dimensional framework: Model description and preliminary results, J. Atmos. Sci., 37, 2486–2507, 1980. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Kogan, Y. L.: The simulation of a convective cloud in a 3-D model with explicit microphysics. Part I: Model description and sensitivity experiments, J. Atmos. Sci., 48, 1160–1189, 1991. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Liu, Y. and Daum, P. H.: Spectral dispersion of cloud droplet size distributions and the parameterization of cloud droplet effective radius, Geophys. Res. Lett., 27, 1903–1906, 2000. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Long, A. B.: Solutions to the droplet collection equation for polynomial kernels, J. Atmos. Sci., 31, 1040–1052, 1974. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Moeng, C.-H.: Entrainment rate, cloud fraction, and liquid water path of PBL stratocumulus clouds, J. Atmos. Sci., 57, 3627–3643, 2000. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Morrison, H. and Grabowski, W. W.: Comparison of bulk and bin warm rain microphysics models using a kinematic framework, J. Atmos. Sci., 64, 2839–2861, 2007. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Morrison, H. and Grabowski, W. W.: Modeling supersaturation and subgrid-scale mixing with two-moment bulk warm microphysics, J. Atmos. Sci., 65, 792–812, 2008. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Paluch, I. R. and Baumgardner, D. G.: Entrainment and fine-scale mixing in a continental convective cloud, J. Atmos. Sci., 46, 261–278, 1989. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Pawlowska, H., Grabowski, W. W., and Brenguier, J. L.: Observations of the width of cloud droplet spectra in stratocumulus, Geophys. Res. Lett., 33, L19810, doi:10.1029/2006GL026841, 2006. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Pinsky, M. B. and Khain, A. P.: Turbulence effects on droplet growth and size distribution in clouds – A review, J. Aerosol Sci., 28, 1177–1214, 1997. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Pinsky, M. B. and Khain, A. P.: Effects of in-cloud nucleation and turbulence on droplet spectrum formation in cumulus clouds, Q. J. Roy. Meteorol. Soc., 128, 501–533, 2002. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Pinsky, M. B. and Khain, A. P.: Collisions of small drops in a turbulent flow. Part II: Effects of flow accelerations, J. Atmos. Sci., 61, 1926–1939, 2004. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Pinsky, M. B., Khain, A. P., Grits, B., and Shapiro, M.: Collisions of small drops in a turbulent flow. Part III: Relative droplet fluxes and swept volumes, J. Atmos. Sci., 63, 2123–2139, 2006. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Pruppacher, H. R. and Klett, J. D.: Microphysics of Clouds and Precipitation, Kluwer Academic, 954 pp, 1997. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Rauber, R. M., Stevens, B., Ochs, H. T., et al.: Rain in Shallow Cumulus Over the Ocean: The RICO Campaign, B. Am. Meteorol. Soc., 88, 1912–1928, 2007. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Riemer, N. and Wexler, A. S.: Droplets to drops by turbulent coagulation, J. Atmos. Sci., 62, 1962–1975, 2005. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Siebesma, A. P., Bretherton, C. S., Brown, A., et al.: A large eddy simulation intercomparison study of shallow cumulus convection, J. Atmos. Sci., 60, 1201–1219, 2003. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Simmel, M., Trautmann, T., and Tetzlaff, G.: Numerical solution of the stochastic collection equation – comparison of the Linear Discrete Method with other methods, Atmos. Res., 61, 135–148, 2002. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Smolarkiewicz, P. K.: A fully multidimensional positive definite advection transport algorithm with small implicit diffusion, J. Comput. Phys., 54, 325–362, 1984. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Srivastava, R. C.: Growth of cloud drops by condensation: Effect of surface tension on the dispersion of drop sizes, J. Atmos. Sci., 48, 1596–1605, 1991. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Stevens, B., Feingold, G., Cotton, W. R., and Walko, R. L.: Elements of the microphysical structure of numerically simulated nonprecipitating stratocumulus, J. Atmos. Sci., 53, 980–1006, 1996. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> Twomey, S.: The nuclei of natural cloud formation part II: The supersaturation in natural clouds and the variation of cloud droplet concentration, Pure Appl. Geophys., 43, 243–249, 1959. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Wang, L. P., Ayala, O., Kasprzak, S. E., and Grabowski, W. W.: Theoretical formulation of collision rate and collision efficiency of hydrodynamically-interacting cloud droplets in turbulent atmospheres, J. Atmos. Sci., 62, 2433–2450, 2005. </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Wang, L. P., Ayala, O., Xue, T., and Grabowski, W. W.: Comments on &quot;Droplets to drops by turbulent coagulation&quot; by Riemer and Wexler, J. Atmos. Sci., 63, 2397–2401, 2006. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Wang, L.-P., Ayala, O., Rosa, B., and Grabowski, W. W.: Turbulent collision efficiency of cloud droplets, New J. Physics, in press, 2008. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Wang, Q. and Albrecht, B. A.: Observations of cloud-top entrainment in marine stratocumulus clouds, J. Atmos. Sci., 51, 1530–1547, 1994. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Xue, Y., Wang, L. P., and Grabowski, W. W.: Growth of cloud droplets by turbulent collision-coalescence, J. Atmos. Sci., 65, 331–356, 2008. </mixed-citation>
</ref>
</ref-list>
</back>
</article>