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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>8</volume_number>
		<issue_number>4</issue_number>
		<publication_year>2008</publication_year>
	</journal>
	<doi>10.5194/acpd-8-13453-2008</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/8/13453/2008/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/8/13453/2008/acpd-8-13453-2008.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/8/13453/2008/acpd-8-13453-2008.pdf</fulltext_pdf>
	<start_page>13453</start_page>
	<end_page>13478</end_page>
	<publication_date>2008-07-15</publication_date>
	<article_title content_type="html">Methane plume over South Asia during the monsoon season: satellite observation and model simulation</article_title>
	<authors>
		<author numeration="1" affiliations="1,2">
			<name>X. Xiong</name>
			<email>xiaozhen.xiong@noaa.gov</email>
		</author>
		<author numeration="2" affiliations="3">
			<name>S. Houweling</name>
		</author>
		<author numeration="3" affiliations="1,2">
			<name>J. Wei</name>
		</author>
		<author numeration="4" affiliations="1,2">
			<name>E. Maddy</name>
		</author>
		<author numeration="5" affiliations="1,2">
			<name>F. Sun</name>
		</author>
		<author numeration="6" affiliations="1">
			<name>C. Barnet</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">NOAA/NESDIS/Center for Satellite Applications and Res., Camp Springs, Maryland, USA</affiliation>
		<affiliation numeration="2" content_type="html">Perot Systems Government Services, Fairfax, Virginia, USA</affiliation>
		<affiliation numeration="3" content_type="html">Netherlands Institute for Space Research, Utrecht, The Netherlands</affiliation>
	</affiliations>
	<abstract content_type="html">Satellite observations of methane (CH&lt;sub&gt;4&lt;/sub&gt;) using the Atmospheric Infrared
Sounder (AIRS) on the EOS/Aqua platform from 2003–2007 demonstrate a strong,
plume-like enhancement of  CH&lt;sub&gt;4&lt;/sub&gt; in the middle to upper troposphere over
the South Asia during July, August and September, and its maximum occurs in
early September. Simulations using the global tracer model version 3 (TM3)
also show similar seasonal enhancement of  CH&lt;sub&gt;4&lt;/sub&gt; in the same region. The
model results also suggest that this enhancement is associated with
transport process and local surface emissions, thus the observations to
tropospheric CH&lt;sub&gt;4&lt;/sub&gt;during the monsoon season may be used to constrain the
models for a better estimation of Asian CH&lt;sub&gt;4&lt;/sub&gt; sources. Further
comparisons between AIRS observations and the model simulations indicate a
possible overestimate of  CH&lt;sub&gt;4&lt;/sub&gt; emissions from rice paddies in Southeast
Asia. Moreover, the observed tropospheric CH&lt;sub&gt;4&lt;/sub&gt; enhancement from AIRS
provides evidence for the strong transport of atmospheric pollutants from
the lower to the upper troposphere in Asia during the monsoon season, and
the observed rapid disappearance of local CH&lt;sub&gt;4&lt;/sub&gt; maximum in September may
provide valuable information for studying the dissipation of the Tibetan
anticyclone and the withdrawal of monsoon.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Aumann, H. H., Chahine, M. T., Gautier, C., Goldberg, M. D., Kalnay, E., McMillin, L. M., Revercomb, H., Rosenkranz, P. W., Smith, W. L., Staelin, D. H., Strow, L. L., and Susskind, J.: AIRS/AMSU/HSB on the aqua mission: Design, science objectives, data products, and processing systems, IEEE T. Geosci. Remote, 41, 253–264, 2003. </reference>
		<reference numeration="2" content_type="text"> Clerbaux, C., Hadji-Lazaro, J., Turquety, S., Mégie, G., and Coheur, P.-F.: Trace gas measurements from infrared satellite for chemistry and climate applications, Atmos. Chem. Phys., 3, 1495–1508, 2003. </reference>
		<reference numeration="3" content_type="text"> De~Mazière, M., Vigouroux, C., Bernath, P. F., Baron, P., Blumenstock, T., Boone, C., Brogniez, C., Catoire, V., Coffey, M., Duchatelet,~P., Griffith, D., Hannigan, J., Kasai, Y., Kramer, I., Jones, N., Mahieu,~E., Manney, G. L., Piccolo, C., Randall, C., Robert, C., Senten, C., Strong,~K., Taylor, J., Tétard, C., Walker, K. A., and Wood, S.: Validation of ACE-FTS v2.2 methane profiles from the upper troposphere to the lower mesosphere, Atmos. Chem. Phys., 8, 2421–2435, 2008. </reference>
		<reference numeration="4" content_type="text"> Fasullo, J. and Webster, P. J.: A hydrological definition of indian monsoon onset and withdrawal, J. Climate, 16, 3200-3211, 2003. </reference>
		<reference numeration="5" content_type="text"> Filipiak, M. J., Harwood, R. S., Jiang, J. H., Li, Q. B., Livesey, N. J., Manney, G. L., Read, W. G., Schwartz, M. J., Waters, J. W., and Wu, D. L.: Carbon monoxide measured by the EOS microwave limb sounder on Aura: First results, Geophys. Res. Lett., 32, L14825, doi:10.1029/2005GL02276, 2005. </reference>
		<reference numeration="6" content_type="text"> Frankenberg, C., Meirink, J. F., van Weele, M., Platt, U., and Wagner, T.: Assessing methane emissions from global space-borne observations, Science, 308, 1010-1014, 2005. </reference>
		<reference numeration="7" content_type="text"> Fu, R., Hu, Y., Wright, J. S., Jiang, J. H. , Dickinson, R. E. , Chen, M. , Filipiak, M. , Read, W. G., Waters, J. W., and Wu, D. L.: Short circuit of water vapor and polluted air to the global stratosphere by convective transport over the Tibetan Plateau, Proceedings of the National Academy of Sciences (PNAS), 103, 5664–5669, 2006. </reference>
		<reference numeration="8" content_type="text"> Heimann, M. and KÖrner, S.: The global atmospheric tracer model TM3, Max Planck Institute of Biogeochemistry, Model description and user&apos;s manual, Release 3.8a, 2003. </reference>
		<reference numeration="9" content_type="text"> Houweling, S., Rockmann, T., Aben, I., Keppler, F., Krol, M., Meirink, J. F., Dlugokencky, E. J., and Frankenberg, C.: Atmospheric constraints on global emissions of methane from plants, Geophys. Res. Lett., 33, L15821, doi:10.1029/2006GL026162, 2006. </reference>
		<reference numeration="10" content_type="text"> Huang, Y., Zhang, W., Zheng, X. H., Li, J., and Yu, Y. Q.: Modeling methane emission from rice paddies with various agricultural practices, J. Geophys. Res.-Atmos., 109, D08113, doi:10.1029/2003JD004401, 2004. </reference>
		<reference numeration="11" content_type="text"> Intergovernmental Panel on Climate Change: Climate Change 2007: The Physical Science Basis, Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 500–590, 2007. </reference>
		<reference numeration="12" content_type="text"> Kalnay, E., Kanamitsu, M., Kistler, R., Collins, W., Deaven, D., Gandin, L., Iredell, M., Saha, S., White, G., Woollen, J., Zhu, Y., Chelliah, M., Ebisuzaki, W., Higgins, W., Janowiak, J., Mo, K. C., Ropelewski, C., Wang, J., Leetmaa, A., Reynolds, R., Jenne, R., and Joseph, D.: The NCEP/NCAR 40-year reanalysis project, B. Am. Meteorol. Soc., 77, 437–471, 1996. </reference>
		<reference numeration="13" content_type="text"> Kar, J., Bremer, H., Drummond, J. R., Rochon, Y. J., Jones, D. B. A., Nichitiu, F., Zou, J., Liu, J., Gille, J. C., Edwards, D. P., Deeter, M. N., Francis, G., Ziskin, D., and Warner, J.: Evidence of vertical transport of carbon monoxide from measurements of pollution in the troposphere (MOPITT), Geophys. Res. Lett., 31, L23105, doi:10.1029/2004GL021128, 2004. </reference>
		<reference numeration="14" content_type="text"> Khalil, M. A. K., Rasmussen, R. A., Shearer, M. J., Dalluge, R. W., Ren, L. X., and Duan, C. L.: Measurements of methane emissions from rice fields in China, J. Geophys. Res.-Atmos., 103, 25 181–25 210, 1998. </reference>
		<reference numeration="15" content_type="text"> Lawrence, M. G., Rasch, P. J., von Kuhlmann, R., Williams, J., Fischer, H., de Reus, M., Lelieveld, J., Crutzen, P. J., Schultz, M., Stier, P., Huntrieser, H., Heland, J., Stohl, A., Forster, C., Elbern, H., Jakobs, H., and Dickerson, R. R.: Global chemical weather forecasts for field campaign planning: Predictions and observations of large-scale features during minos, contrace, and indoex, Atmos. Chem. Phys., 3, 267–289, 2003. </reference>
		<reference numeration="16" content_type="text"> Li, Q. B., Jacob, D. J., Logan, J. A., Bey, I., Yantosca, R. M., Liu, H. Y., Martin, R. V., Fiore, A. M., Field, B. D., Duncan, B. N., and Thouret, V.: A tropospheric ozone maximum over the middle east, Geophys. Res. Lett., 28, 3235–3238, 2001. </reference>
		<reference numeration="17" content_type="text"> Li, Q. B., Jiang, J. H., Wu, D. L., Read, W. G., Livesey, N. J., Waters, J. W., Zhang, Y. S., Wang, B., Filipiak, M. J., Davis, C. P., Turquety, S., Wu, S. L., Park, R. J., Yantosca, R. M., and Jacob, D. J.: Convective outflow of south asian pollution: A global ctm simulation compared with EOS MLS observations, Geophys. Res. Lett., 32, L14826, doi:10.1029/2005GL022762, 2005. </reference>
		<reference numeration="18" content_type="text"> Liu, Y., Li, W. L., Zhou, X. J., Isaksen, I. S. A., Sundet, J. K., and He, J. H.: The possible influences of the increasing anthropogenic emissions in India on tropospheric ozone and \chemOH, Adv. Atmos. Sci., 20, 968–977, 2003. </reference>
		<reference numeration="19" content_type="text"> Maddy, E. S. and Barnet, C. D.: Vertical resolution estimates in Version 5 of AIRS operational retrievals, IEEE T. Geosci. Remote, 46, 8, 2008. </reference>
		<reference numeration="20" content_type="text"> Nassar, R., Bernath, P.F., Boone, C. D., Manney, G. L., McLeod, S. D., Rinsland, C. P., Skelton, R., and Walker, K. A., Stratospheric abundances of water and methane based on ACE-FTS measurements, Geophys. Res. Lett., 32, L15S04, doi:10.1029/2005GL022383, 2005. </reference>
		<reference numeration="21" content_type="text"> Payan, S., Camy-Peyret, C., Oelhaf, H., Wetzel, G., Maucher, G., Keim, C., Pirre, M., Huret, N., Engel, A., Volk, M. C., Kuellmann, H., Kuttippurath, J., Cortesi, U., Bianchini, G., Mencaraglia, F., Raspollini, P., Redaelli, G., Vigouroux, C., De Mazière, M., Mikuteit, S., Blumenstock, T., Velazco, V., Notholt, J., Mahieu,~M., Duchatelet, P., Smale, D., Wood, S., Jones, N., Piccolo, C., Payne, V., Bracher, A., Glatthor, N., Stiller, G., Grunow, K., Jeseck, P., Te, Y., Pfeilsticker, K., and Butz, A.: Validation and data characteristics of methane and nitrous oxide profiles observed by MIPAS and processed with Version 4.61 algorithm, Atmos. Chem. Phys. Discuss., 7, 18 043–18 111, 2007. </reference>
		<reference numeration="22" content_type="text"> Park, M., Randel, W. J., Kinnison, D. E., Garcia, R. R., and Choi, W.: Seasonal variation of methane, water vapor, and nitrogen oxides near the tropopause: Satellite observations and model simulations, J. Geophys. Res.-Atmos., 109, D03302, doi:10.1029/2003JD003706, 2004. </reference>
		<reference numeration="23" content_type="text"> Randel, W. J. and Park, M.: Deep convective influence on the asian summer monsoon anticyclone and associated tracer variability observed with atmospheric infrared sounder (AIRS), J. Geophys. Res.-Atmos., 111, D12314, doi:10.1029/2005JD006490., 2006. </reference>
		<reference numeration="24" content_type="text"> Rodgers, C. D.: Inverse Methods for Atmospheric Sounding, World Sci., Hackensack, N. J., 2000. </reference>
		<reference numeration="25" content_type="text"> Strow, L. L., Hannon, S. E., De Souza-Machado, S., Motteler, H. E., and Tobin, D.: An overview of the airs radiative transfer model, IEEE T. Geosci. Remote, 41, 303–313, 2003. </reference>
		<reference numeration="26" content_type="text"> Taniguchi, K. and Koike, T.: Seasonal Variation of Cloud Activity and Atmospheric Profiles over the Eastern Part of the Tibetan Plateau, J. Geophys. Res., 113, D10104, doi:10.1029/2007JD009321, 2008 </reference>
		<reference numeration="27" content_type="text"> Xiong, X., Barnet, C. D., Maddy, E. , Sweeney, C. , Liu, X. , Zhou, L., and Goldberg, M.: Characterization and Validation of Methane Products from the Atmospheric Infrared Sounder (AIRS), J. Geophys. Res., 113, G00A01, doi:10.1029/2007JG000500, 2008. </reference>
		<reference numeration="28" content_type="text"> Ye, D. Z. and Wu, G. X.: The role of the heat source of the tibetan plateau in the general circulation, Meteorol. Atmos. Phys., 67, 181–198, 1998. </reference>
	</references>
</article>

