Atmospheric Chemistry and Physics Discussions
www.atmos-chem-phys-discuss.net
1680-7367
1680-7375
7
4
2007
10.5194/acpd-7-9769-2007
http://www.atmos-chem-phys-discuss.net/7/9769/2007/
http://www.atmos-chem-phys-discuss.net/7/9769/2007/acpd-7-9769-2007.html
http://www.atmos-chem-phys-discuss.net/7/9769/2007/acpd-7-9769-2007.pdf
9769
9793
2007-07-05
Performance of MAX-DOAS measurements of aerosols at Tsukuba, Japan: a comparison with lidar and sky radiometer measurements
H. Irie
irie@jamstec.go.jp
Y. Kanaya
H. Akimoto
H. Iwabuchi
A. Shimizu
K. Aoki
Frontier Research Center for Global Change, Japan Agency for Marine-Earth Science and Technology, 3173-25 Showa-machi, Kanazawa-ku, Yokohama, Kanagawa 236-0001, Japan
National Institute for Environmental Studies, 16-2, Onogawa, Tsukuba, Ibaraki 305-8506, Japan
Department of Earth Science, Faculty of Sciences, University of Toyama, 3190 Gofuku, Toyama 930-8555, Japan
Ground-based Multi-Axis Differential Optical Absorption Spectroscopy
(MAX-DOAS) measurements were performed at Tsukuba, Japan (36.1° N,
140.1° E), in November–December 2006. The measured spectra of scattered
sunlight are analyzed by DOAS and optimal estimation methods to retrieve the
aerosol optical depth (τ) and the vertical profile of the aerosol
extinction coefficient (σ) at 476 nm in the lower troposphere. We
characterize these retrieved quantities through comparisons with coincident
lidar and sky radiometer measurements. The retrieved σ values for
layers of 0–1 and 1–2 km agree with lidar data to within 30% and 60%,
respectively, for most cases, including partly cloudy conditions. Results
similar to σ at 0–1 km are obtained for the retrieved τ
values, demonstrating that MAX-DOAS provides the new, unique aerosol dataset
in the lower troposphere.
Aoki, K. and Fujiyoshi, Y.: Sky radiometer measurements of aerosol optical properties over Sapporo, Japan, J. Meteorol. Soc. Jpn., 81(3), 493–513, 2003.
Aliwell, S. R., van Roozendael, M., Johnston, P. V., Richter, A., Wagner, T., Arlander, D. W., Burrows, J. P., Fish, D. J., Jones, R. L., Tørnkvist, K. K., Lambert, J.-C., Pfeilsticker, K., and Pundt, I.: Analysis for BrO in zenith-sky spectra: An intercomparison exercise for analysis improvement, J. Geophys. Res., 107(D14), 4199, doi:10.1029/2001JD000329, 2002.
Bogumil, K., Orphal, J., Homann, T., Voigt, S., Spietz, P., Fleischmann, O. C., Vogel, A., Hartmann, M., Bovensmann, H., Frerik, J., and Burrows, J. P.: Measurements of molecular absorption spectra with the SCIAMACHY pre-flight model: Instrument characterization and reference data for atmospheric remote-sensing in the 230–2380 nm region, J. Photochem. Photobiol. A., 157, 167–184, 2003.
Cattrall, C., Reagan, J., Thome, K., and Dubovik, O.: Variability of aerosol and spectral lidar and backscatter and extinction ratios of key aerosol types derived from selected Aerosol Robotic Network locations, J. Geophys. Res., 110, D10S11, doi:10.1029/2004JD005124, 2005.
Chance, K. and Spurr, R. J. D.: Ring effect studies: Rayleigh scattering, including molecular parameters for rotational Raman scattering, and the Fraunhofer spectrum, Appl. Opt., 36, 5224–5230, 1997.
Chance, K., Kurosu, T. P., and Sioris, C. E.: Undersampling correction for array detector-based satellite spectrometers, Appl. Opt., 44(7), 1296–1304, 2005.
Fernald, F. G.: Analysis of atmospheric lidar observations: some comments, Appl. Opt., 23(5), 652–653, 1984.
Frieß, U., Monks, P. S., Remedios, J. J., Rozanov, A., Sinreich, R., Wagner, T., and Platt, U.: MAX-DOAS O<sub>4</sub> measurements: A new technique to derive information on atmospheric aerosols: 2. Modeling studies, J. Geophys. Res., 111, D14203, doi:10.1029/2005JD006618, 2006.
Grainger, J. F. and Ring, J.: Anomalous Fraunhofer line profiles, Nature 193, 762, 1962.
Greenblatt, G. D., Orlando, J. J., Burkholder, J. B., and Ravishankara, A. R.: Absorption measurements of oxygen between 330 and 1140 nm, J. Geophys. Res., 95, 11, 18 577–18 582, 1990.
Heckel, A., Richter, A., Tarsu, T., Wittrock, F., Hak, C., Pundt, I., Junkermann, W., and Burrows, J. P.: MAX-DOAS measurements of formaldehyde in the Po-Valley, Atmos. Chem. Phys., 5, 909–918, 2005.
Hendrick, F., van Roozendael, M., Kylling, A., Petritoli, A., Rozanov, A., Sanghavi, S., Schofield, R., von Friedeburg, C., Wagner, T., Wittrock, F., Fonteyn, D., and De Mazière, M.: Intercomparison exercise between different radiative transfer models used for the interpretation of ground-based zenith-sky and multi-axis DOAS observations, Atmos. Chem. Phys., 6, 93–108, 2006.
Hönninger, G., von Friedeburg, C., and Platt, U.: Multi axis differential optical absorption spectroscopy (MAX-DOAS), Atmos. Chem. Phys., 4, 231–254, 2004.
Iwabuchi, H.: Efficient Monte Carlo methods for radiative transfer modeling, J. Atmos. Sci., 63(9), 2324–2339, 2006.
Kaufman, Y. J., Tanré, D., and Boucher, O.: A satellite view of aerosols in the climate system, Rev. Nature, 419, 215–223, 2002.
Kim, D.-H., Sohn, B. J., Nakajima, T., and Takamura, T.: Aerosol radiative forcing over east Asia determined from ground-based solar radiation measurements, J. Geophys. Res., 110, D10S22, doi:10.1029/2004JD004678, 2005.
Kurucz, R. L., Furenlid, I., Brault, J., and Testerman, L.: Solar flux atlas from 296 to 1300 nm, Natl. Sol. Obs., Sunspot, New Mexico, 240pp., 1984.
Leigh, R. J., Corlett, G. K., Frieß, U., and Monks, P. S.: Concurrent multiaxis differential optical absorption spectroscopy system for the measurement of tropospheric nitrogen dioxide, Appl. Opt., 45, 28, 7504–7518, 2006.
Nakajima, T., Tonna, G., Rao, R., Boi, P., Kaufman, Y., and Holben, B.: Use of sky brightness measurements from ground for remote sensing of particulate polydispersions, Appl. Opt., 35(15), 2672–2686, 1996.
Platt, U.: Differential optical absorption spectroscopy (DOAS), Air Monitoring by Spectroscopic Techniques, edited by: Sigrist, M. W., John Wiley & Sons, Inc., New York, 127, 27–84, 1994.
Rodgers, C. D.: Inverse methods for atmospheric sounding: Theory and practice, Ser. Atmos. Oceanic Planet. Phys., 2, edited by: Taylor, F. W., World Sci., Hackensack, N. J., 2000.
Rothman, L. S., Barbe, A., Benner, D. C., Brown, L. R., Camy-Peyret, C., Carleer, M. R., Chance, K., Clerbaux, C., Dana, V., Devi, V. M., Fayt, A., Flaud, J.-M., Gamache, R. R., Goldman, A., Jacquemart, D., Jucks, K. W., Lafferty, W. J., Mandin, J.-Y., Massie, S. T., Nemtchinov, V., Newnham, D. A., Perrin, A., Rinsland, C. P., Schroeder, J., Smith, K. M., Smith, M. A. H., Tang, K., Toth, R. A., Vander Auwera, J., Varanasi, P., and Yoshino, K.: The HITRAN molecular spectroscopic database: edition of 2000 including updates through 2001, J. Quant. Spectrosc. Radiat. Transfer, 82, 5–44, 2003.
Shimizu, A., Sugimoto, N., Matsui, I., Arao, K., Uno, I., Murayama, T., Kagawa, N., Aoki, K., Uchiyama, A., and Yamazaki, A.: Continuous observations of Asian dust and other aerosols by polarization lidars in China and Japan during ACE-Asia, J. Geophys. Res., 109, D19S17, doi:10.1029/2002JD003253, 2004.
Sinreich, R., Volkamer, R., Filsinger, F., Frieß, U., Kern, C., Platt, U., Sebastian, O., and Wagner, T.: MAX-DOAS detection of glyoxal during ICARTT 2004, Atmos. Chem. Phys., 7, 1293–1303, 2007.
Tatarov, B., Sugimoto, N., Matsui, I., and Shimizu, A.: Two-year-observations of optical properties of the tropospheric aerosol and clouds by a high-spectral-resolution lidar over Tsukuba, Japan, Reviewed and Revised Papers Presented at the 23rd International Laser Radar Conference, 23ILRC, ISBN 4-9902916-0-3, 451–454, 2006.
Vandaele, A. C., Hermans, C., Simon, P. C., Carleer, M., Colin, R., Fally, S., Mérienne, M. F., Jenouvrier, A., and Coquart, B.: Measurements of the NO<sub>2</sub> absorption cross-section from 42 000 cm<sup>−1</sup> to 10 000 cm<sup>−1</sup> (238–1000 nm) at 220 K and 294 K, J. Quant. Spectrosc. Radiat. Transfer, 59, 171–184, 1998.
Wagner, T., Dix, B., von Friedeburg, C., Frieß, U., Sanghavi, S., Sinreich, R., and Platt, U.: MAX-DOAS O<sub>4</sub> measurements: A new technique to derive information on atmospheric aerosols – Principles and information content, J. Geophys. Res., 109, D22205, doi:10.1029/2004JD004904, 2004.
Wagner, T., Burrows, J. P., Deutschmann, T., Dix, B., von Friedeburg, C., Frieß, U., Hendrick, F., Heue, K.-P., Irie, H., Iwabuchi, H., Kanaya, Y., Keller, J., McLinden, C. A., Oetjen, H., Palazzi, E., Petritoli, A., Platt, U., Postylyakov, O., Pukite, J., Richter, A., van Roozendael, M., Rozanov, A., Rozanov, V., Sinreich, R., Sanghavi, S., and Wittrock, F.: Comparison of box-air-mass-factors and radiances for multiple-axis differential optical absorption spectroscopy (MAX-DOAS) geometries calculated from different UV/visible radiative transfer models, Atmos. Chem. Phys., 7, 1809–1833, 2007.
Wittrock, F., Oetjen, H., Richter, A., Fietkau, S., Medeke, T., Rozanov, A., and Burrows, J. P.: MAX-DOAS measurements of atmospheric trace gases in Ny-Ålesund – Radiative transfer studies and their application, Atmos. Chem. Phys., 4, 955–966, 2004.