Atmos. Chem. Phys. Discuss., 7, 9013-9051, 2007
www.atmos-chem-phys-discuss.net/7/9013/2007/
doi:10.5194/acpd-7-9013-2007
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Intercontinental transport of pollution and dust aerosols: implications for regional air quality
Mian Chin1, T. Diehl2, P. Ginoux3, and W. Malm4
1NASA Goddard Space Flight Center, Greenbelt, MD, USA
2University of Maryland Baltimore County, Baltimore, MD, USA
3NOAA Geophysical Fluid Dynamics Laboratory, Princeton, NJ, USA
4National Parck Service, CIRA, Colorado State University, Fort Collins, CO, USA

Abstract. We use the global model GOCART to examine the impact of pollution and dust aerosols emitted from their major sources on surface fine particulate matter concentrations at regional and hemispheric scales. Focusing on the North America region in 2001, we use measurements from the IMPROVE network in the United States to evaluate the model-simulated surface concentrations of the "reconstructed fine mass" (RCFM) and its components of ammonium sulfate, black carbon (BC), organic matter (OM), and fine mode dust. We then quantify the RCFM budget in terms of the RCFM composition, type, and origin to find that in the eastern U.S., ammonium sulfate is the dominant RCFM component (~60%) whereas in the western U.S., dust and OM are just as important as sulfate but have considerable seasonal variations, especially in the NW. On an annual average, North America regional pollution accounts for nearly 30–40% of the surface RCFM in the western U.S., and for a much higher proportion of 65–70% in the eastern U.S. By contrast, pollution from outside of North America contributes to just 2–6% (~0.2 μg m−3) of the total RCFM over the U.S. on an annual average. In comparison, long-range transport of dust is more efficient than that of pollution, which brings 3 to 4 times more fine particles to the U.S. (0.5–0.8 μg m−3 on an annual average) with a maximum influence in spring and over the NW. Of the major pollution regions, Europe has the largest potential to affect the surface aerosol concentrations in other continents due to its shorter distance from receptor continents and its larger fraction of sulfate-producing precursor gas in the outflow. With the IPCC emission scenario for the year 2000, we find that European emissions increase levels of ammonium sulfate by 1–5 μg m−3 over the surface of northern Africa and western Asia, and its contribution to eastern Asia (≥0.2 μg m−3) is twice as much as the Asian contribution to North America. Asia and North America pollution emissions exert strong impacts on their neighboring oceans, but their influences on other continents are relatively small (≤10%) due to the long traveling distance across the oceans and efficient removal during transport. Among the major dust source regions, Asia displays a significant influence over large areas in the Northern Hemisphere except over the North Atlantic and the tropics, where African dust dominates. The trans-Pacific transport of Asian dust is much more efficient than that of Asian pollution because of the higher elevation and lower removal rate of dust. We notice that the African dust can travel eastward through a pathway spanning across Asia and North Pacific to settle down over the surface of western North America. African dust transported through such a pathway is difficult to detect because it usually merges and travels together with the Asian dust.

Citation: Mian Chin, Diehl, T., Ginoux, P., and Malm, W.: Intercontinental transport of pollution and dust aerosols: implications for regional air quality, Atmos. Chem. Phys. Discuss., 7, 9013-9051, doi:10.5194/acpd-7-9013-2007, 2007.
 
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