Atmos. Chem. Phys. Discuss., 7, 8525-8569, 2007
www.atmos-chem-phys-discuss.net/7/8525/2007/
doi:10.5194/acpd-7-8525-2007
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
The Coupled Aerosol and Tracer Transport model to the Brazilian developments on the Regional Atmospheric Modeling System (CATT-BRAMS) – Part 1: Model description and evaluation
S. R. Freitas1, K. M. Longo1, M. A. F. Silva Dias1,2, R. Chatfield3, P. Silva Dias2, P. Artaxo4, M. O. Andreae5, G. Grell6, L. F. Rodrigues1, A. Fazenda1,7, and J. Panetta1
1Center for Weather Forecasting and Climate Studies (CPTEC), INPE, Cachoeira Paulista, Brazil
2Department of Atmospheric Sciences, University of São Paulo, Brazil
3NASA Ames Research Center, Moffett Field, USA
4Institute of Physics, University of São Paulo, Brazil
5Max Planck Institute for Chemistry, Mainz, Germany
6Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado/NOAA Research-Forecast Systems Laboratory, Boulder, CO, USA
7Department of Computing Science, University of Taubaté, São Paulo, Brazil

Abstract. We introduce the Coupled Aerosol and Tracer Transport model to the Brazilian developments on the Regional Atmospheric Modeling System (CATT-BRAMS). CATT-BRAMS is an on-line transport model fully consistent with the simulated atmospheric dynamics. Emission sources from biomass burning and urban-industrial-vehicular activities for trace gases and aerosol particles are obtained from several published datasets and remote sensing information. The tracer and aerosol mass concentration prognostic includes the effects of sub-grid scale turbulence in the planetary boundary layer, convective transport by shallow and deep moist convection, wet and dry deposition, and plume rise associated with vegetation fires in addition to the grid scale transport. The radiation parameterization takes into account the interaction between aerosol particles and short and long wave radiation. The atmospheric model BRAMS is based on the Regional Atmospheric Modeling System (RAMS), with several improvements associated with cumulus convection representation, soil moisture initialization and surface scheme tuned for the tropics, among others. In this paper the CATT-BRAMS model is used to simulate carbon monoxide and particulate material (PM2.5) surface fluxes and atmospheric transport during the 2002 LBA field campaigns, conducted during the transition from the dry to wet season in the southwest Amazon Basin. Model evaluation is addressed with comparisons between model results and near surface, radiosonde and airborne measurements performed during the field campaign, as well as remote sensing derived products. We show the matching of emissions strengths to observed carbon monoxide in the LBA campaign. A relatively good comparison to the MOPITT data, in spite of the fact that MOPITT a priori assumptions imply several difficulties, is also obtained.

Citation: Freitas, S. R., Longo, K. M., Silva Dias, M. A. F., Chatfield, R., Silva Dias, P., Artaxo, P., Andreae, M. O., Grell, G., Rodrigues, L. F., Fazenda, A., and Panetta, J.: The Coupled Aerosol and Tracer Transport model to the Brazilian developments on the Regional Atmospheric Modeling System (CATT-BRAMS) – Part 1: Model description and evaluation, Atmos. Chem. Phys. Discuss., 7, 8525-8569, doi:10.5194/acpd-7-8525-2007, 2007.
 
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