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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>7</volume_number>
		<issue_number>2</issue_number>
		<publication_year>2007</publication_year>
	</journal>
	<doi>10.5194/acpd-7-5595-2007</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/7/5595/2007/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/7/5595/2007/acpd-7-5595-2007.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/7/5595/2007/acpd-7-5595-2007.pdf</fulltext_pdf>
	<start_page>5595</start_page>
	<end_page>5615</end_page>
	<publication_date>2007-04-26</publication_date>
	<article_title content_type="html">CALIPSO observations of stratospheric aerosols: a preliminary assessment</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>L. W. Thomason</name>
			<email>l.w.thomason@nasa.gov</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>M. C. Pitts</name>
		</author>
		<author numeration="3" affiliations="1">
			<name>D. M. Winker</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">NASA Langley Research Center, Hampton, VA, USA</affiliation>
	</affiliations>
	<abstract content_type="html">We have examined the 532-nm aerosol backscatter coefficient measurements by
the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations
(CALIPSO) for their use in the observation of stratospheric aerosol. CALIPSO
makes observations that span from 82&amp;deg; S to 82&amp;deg; N each day and, for
each profile, backscatter coefficient values reported up to ~40 km.
The possibility of using CALIPSO for stratospheric aerosol observations is
demonstrated by the clear observation of the 20 May 2006 eruption of
Montserrat in the earliest CALIPSO data in early June as well as by
observations showing the 7 October 2006 eruption of Tavurvur (Rabaul).
However, the very low aerosol loading within the stratosphere makes routine
observations of the stratospheric aerosol far more difficult than relatively
dense volcanic plumes. Nonetheless, we found that averaging a complete days
worth of nighttime only data into 5-deg latitude by 1-km vertical bins
reveals a stratospheric aerosol layer centered near an altitude of 20 km,
the clean wintertime polar vortices, and a small maximum in the lower
tropical stratosphere. However, the derived values are clearly too small and
often negative in much of the stratosphere. The data can be significantly
improved by increasing the measured backscatter (molecular and aerosol) by
approximately 5% suggesting that the current method of calibrating to a
pure molecular atmosphere at 30 km is most likely the source of the low
values.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Bloom, S., da Silva, A. M., Bosilovich, D. Dee, Chern, J.-D., Pawson, S., Schubert, S., Sienkiewicz, M., ,Stajner, I., Tan, W.-W., and Wu, M.-L.: Documentation and Validation of the Goddard Earth Observing System (GEOS) Data Assimilation System &amp;ndash; Version 4 . Technical Report Series on Global Modeling and Data Assimilation 104606, 26, 2005. </reference>
		<reference numeration="2" content_type="text"> Carn, S. A., Krotkov, N. A., Yang, K., Hoff, R. M., Prata, A. J., Krueger, A. J., Loughlin, S. C., and Levelt, P. F.: Extended observations of volcanic SO2 and sulfate aerosol in the stratosphere, Atmos. Chem. Phys. Discuss., 7, 2857&amp;ndash;2871, 2007. </reference>
		<reference numeration="3" content_type="text"> Deshler, T., Anderson-Sprecher, R., Jager, H., Barnes, J., Hofmann, D. J., Clemesha, B., Simonich, D., Osborn, M., Grainger, R. G., and Godin-Beekmann, S.: Trends in the nonvolcanic component of stratospheric aerosol over the period 1971&amp;ndash;2004, J. Geophys. Res., 111, D01201, doi:10.1029/2005JD006089, 2006. </reference>
		<reference numeration="4" content_type="text"> Hostetler, C. A., Z. Liu, J. Reagan, M. Vaughan, D. Winker, M. Osborn, W. H. Hunt, K. A. Powell, and C. Trepte: &quot;CALIOP Algorithm Theoretical Basis Document &amp;ndash; Part 1: Calibration and Level 1 Data Products&quot;, PC-SCI-201, NASA Langley Research Center, Hampton, VA ,available at http://www-calipso.larc.nasa.gov/resources/project_documentation.php, 2006. </reference>
		<reference numeration="5" content_type="text"> Jäger, H. and Deshler, T.: Lidar backscatter to extinction, mass and area conversions for stratospheric aerosols based on midlatitude balloonborne size distribution measurements, Geophys. Res. Lett., 29(19), 1929, doi:10.1029/2002GL015609, 2002. </reference>
		<reference numeration="6" content_type="text"> Kärcher, B.: Properties of subvisible cirrus clouds formed by homogeneous freezing, Atmos. Chem. Phys., 2, 161&amp;ndash;170, 2002. </reference>
		<reference numeration="7" content_type="text"> Kent, G. S., Winkler, D. M., Osborn, M. T., and Skeens, K. M.: A model for the separation of cloud and aerosol in SAGE II occultation data, J. Geophys. Res., 98, 20 725&amp;ndash;20 735, 1993. </reference>
		<reference numeration="8" content_type="text"> Lin, S. J.: A &quot;Vertically Lagrangian&quot; Finite-Volume Dynamical Core for Global Models. Mon. Wea. Rev., 132, 2293&amp;ndash;2307, 2004. </reference>
		<reference numeration="9" content_type="text"> Notholt, J., Luo, B.-P., Fueglistatler, S., Weisenstein, D., et al.: Influence of tropospheric SO2 emissions on particle formation and the stratospheric humidity, Geophys. Res. Lett., 32, L07810, doi:10.1029/2004GL022159, 2005. %</reference>
		<reference numeration="10" content_type="text"> %Pitts, M. C., Thomason, L. W., and Poole, L. R.: Characterizations of polar %stratospheric clouds by the CALIPSO spaceborne lidar: The 2006 Antarctic %season, submitted, 2007. </reference>
		<reference numeration="11" content_type="text"> Powell, K., Hunt, B., and Winker, D.: Simulations of CALIPSO Lidar Data, ILRC 2002, Quebec City, Quebec, 2002. </reference>
		<reference numeration="12" content_type="text"> Stern, D. I.: Global sulfur emissions in the 1990s, Rensselaer Working Papers in Economics No. 0311, Rensselaer Polytechnic Institute, Troy, N.Y., USA, 33 pp, 2003. </reference>
		<reference numeration="13" content_type="text"> Thomason, L. W., Herber, A. B., Yamanouchi, T., and Sato, K.: Arctic Study on Tropospheric Aerosol and Radiation: Comparison of tropospheric aerosol extinction profiles measured by airborne photometer and SAGE II, Geophys. Res. Lett., 30, 1328&amp;ndash;1331, doi:10.1029/2002GL016453, 2003. </reference>
		<reference numeration="14" content_type="text"> Thomason, L. W. and Peter, T. (Eds.): Assessment of Stratospheric Aerosol Properties (ASAP), SPARC Report No. 4, WCRP-124, WMO/TD-No. 1295, http://www.atmosp.physics.ca/SPARC/, February 2006. </reference>
		<reference numeration="15" content_type="text"> Thomason, L. W., Poole, L. R., and Randall, C. E.: SAGE III aerosol extinction validation in the Arctic winter: comparisons with SAGE II and POAM III Atmos. Chem. Phys., 7, 1423&amp;ndash;1433, 2007. %</reference>
		<reference numeration="16" content_type="text"> %Thomason, L. W., Burton, S. P., Luo, B.-P., and Peter, T.: SAGE II measurements %of stratospheric aerosol properties at non-volcanic levels, Atmos. Chem. Phys. Discuss, submitted, 2007. </reference>
		<reference numeration="17" content_type="text"> Vaughan, G. and Wareing, D. P.: Stratospheric aerosol measurements by dual polarization lidar, Atmos. Chem. Phys., 4, 2441&amp;ndash;2447, 2004. </reference>
		<reference numeration="18" content_type="text"> Vaughan, M., Young, S., Winker, D., Powell, K., Omar, A., Liu, Z., Hu, Y., and Hostetler, C.: Fully automated analysis of space-based lidar data: an overview of the CALIPSO retrieval algorithms and data products. Proc. SPIE, 5575, 16&amp;ndash;30, 2004. %</reference>
		<reference numeration="19" content_type="text"> %Winker, D. M., McGill, M., and Hunt, W. H.: Initial Performance %Assessment of CALIOP, Geophys. Res. Lett., submitted\blackbox\bf status?, 2007. </reference>
	</references>
</article>

