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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>7</volume_number>
		<issue_number>6</issue_number>
		<publication_year>2007</publication_year>
	</journal>
	<doi>10.5194/acpd-7-17705-2007</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/7/17705/2007/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/7/17705/2007/acpd-7-17705-2007.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/7/17705/2007/acpd-7-17705-2007.pdf</fulltext_pdf>
	<start_page>17705</start_page>
	<end_page>17739</end_page>
	<publication_date>2007-12-10</publication_date>
	<article_title content_type="html">SALSA &amp;ndash; a Sectional Aerosol module for Large Scale Applications</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>H. Kokkola</name>
		</author>
		<author numeration="2" affiliations="2">
			<name>H. Korhonen</name>
		</author>
		<author numeration="3" affiliations="1,3">
			<name>K. E. J. Lehtinen</name>
		</author>
		<author numeration="4" affiliations="4">
			<name>R. Makkonen</name>
		</author>
		<author numeration="5" affiliations="2">
			<name>A. Asmi</name>
		</author>
		<author numeration="6" affiliations="2,5">
			<name>S. JÃ¤rvenoja</name>
		</author>
		<author numeration="7" affiliations="2">
			<name>T. Anttila</name>
		</author>
		<author numeration="8" affiliations="1">
			<name>A.-I. Partanen</name>
		</author>
		<author numeration="9" affiliations="4">
			<name>M. Kulmala</name>
		</author>
		<author numeration="10" affiliations="2">
			<name>H. JÃ¤rvinen</name>
		</author>
		<author numeration="11" affiliations="2,3">
			<name>A. Laaksonen</name>
		</author>
		<author numeration="12" affiliations="2">
			<name>V.-M. Kerminen</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Finnish Meteorological Institute, Kuopio Unit, P.O. Box 1627,  70211 Kuopio, Finland</affiliation>
		<affiliation numeration="2" content_type="html">Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland</affiliation>
		<affiliation numeration="3" content_type="html">Department of Physics, Univ. of Kuopio, P.O. Box 1672, 70211 Kuopio, Finland</affiliation>
		<affiliation numeration="4" content_type="html">Department of Physical Sciences, P.O. Box 64, 00014 Univ. of Helsinki, Finland</affiliation>
		<affiliation numeration="5" content_type="html">deceased</affiliation>
	</affiliations>
	<abstract content_type="html">The sectional aerosol module SALSA is introduced.
The model has been designed to be implemented in large
scale climate models, which require both accuracy and computational
efficiency. We have used multiple methods to reduce the computational
burden of different aerosol processes to optimize the model
performance without losing physical features relevant to problematics of
climate importance. The optimizations include limiting the chemical compounds
and physical processes available in different size sections of aerosol particles;
 division of the size distribution into size sections
 using size sections of variable width depending on the sensitivity of
 microphysical processing to the particles sizes; the total amount of size sections
to describe the size distribution is kept to the minimum; furthermore, only
the relevant microphysical processes affecting each size section are
calculated. The ability of the module to describe different
microphysical processes was evaluated against explicit microphysical
models and several microphysical models used in air quality
models. The results from the current module show good consistency when
compared to more explicit models. Also, the module was used to simulate a
new particle formation event typical in highly polluted conditions
with comparable results to a more explicit model setup.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Abdul-Razzak, H. and Ghan, S J.: A parameterization of aerosol activation 3. Sectional representation, J. Geophys. Res., 107, \doi10.1029/2001JD000483, 2002. </reference>
		<reference numeration="2" content_type="text"> Abdul-Razzak, H., Ghan, S J., and Rivera-Carpio, C.: A parameterization of aerosol activation 1. Single aerosol type, J. Geophys. Res., 103, 6123&amp;ndash;6131, 1998. </reference>
		<reference numeration="3" content_type="text"> Ackermann, I J., Hass, H., Memmesheimer, M., Ebel, A., Binkowski, F S., and Shankar, U.: Modal Aerosol Dynamics Model for Europe: Development and First Applications, Atmos. Environ., 32, 2981&amp;ndash;2999, 1998. </reference>
		<reference numeration="4" content_type="text"> Adams, P J. and Seinfeld, J H.: Predicting global aerosol size distributions in general circulation models, J. Geophys. Res. Atmos., 107, 4&amp;ndash;1, \doi10.1029/2001JD001010, 2002. </reference>
		<reference numeration="5" content_type="text"> Binkowski, F S. and Roselle, S J.: Models-3 Community Multiscale Air Quality (CMAQ) model aerosol component 1. Model description., J. Geophys. Res., 108, 4183, \doi10.1029/2001JD001409, 2003. </reference>
		<reference numeration="6" content_type="text"> Binkowski, F S. and Shankar, U.: The Regional Particulate Matter Model. 1. Model Description and Preliminary results, J. Geophys. Res., 100, 26 191&amp;ndash;26 209, 1995. </reference>
		<reference numeration="7" content_type="text"> Chen, Y. and Penner, J E.: Uncertainty analysis for estimates of the first indirect aerosol effect, Atmos. Chem. Phys. Discuss., 5, 4507&amp;ndash;4543, 2005. </reference>
		<reference numeration="8" content_type="text"> Dusek, U., Frank, G P., Hildebrandt, L., Curtius, J., Schneider, J., Walter, S., Chand, D., Drewnick, F., Hings, S., Jung, D., Borrmann, S., and Andreae, M O.: Size Matters More Than Chemistry for Cloud-Nucleating Ability of Aerosol Particles, Science, 312, 1375&amp;ndash;1378, \doi10.1126/science.1125261,available at:http://www.sciencemag.org/cgi/content/abstract/312/5778/1375, 2006. </reference>
		<reference numeration="9" content_type="text"> Ghan, S., Laulainen, N., Easter, R., Wagener, R., Nemesure, S., Chapman, E., Zhang, Y., and Leung, R.: Evaluation of aerosol direct radiative forcing in MIRAGE, J. Geophys. Res., 106, 5295&amp;ndash;5316, 2001. </reference>
		<reference numeration="10" content_type="text"> Hamed, A., Joutsensaari, J., Mikkonen, S., Sogacheva, L., Dal~Maso, M., Kulmala, M., Cavalli, F., Fuzzi, S., Facchini, M C., Decesari, S., Mircea, M., Lehtinen, K. E J., and Laaksonen, A.: Nucleation and growth of new particles in Po Valley, Italy, Atmos. Chem. Phys., 7, 355&amp;ndash;376, http://www.atmos-chem-phys.net/7/355/2007/, 2007. </reference>
		<reference numeration="11" content_type="text"> Jacobson, M Z.: Developing, coupling and applying a gas, aerosol, transport and radiation model to study urban and regional air pollution, Ph.D thesis, Dept of Atmospheric Sciences, University of California, Los Angeles, 1994. </reference>
		<reference numeration="12" content_type="text"> Jacobson, M Z.: Studying the effects of calcium and magnesium on size-distributed nitrate and ammonium with EQUISOLV II, Atmos. Environ., 33, 3635&amp;ndash;3649, 1999. </reference>
		<reference numeration="13" content_type="text"> Jacobson, M Z.: GATOR-GCMM: A global through urban scale air pollution and weather forecast model. 1. Model design and treatment of subgrid soil, vegetation, roads, rooftops, water, sea ice, and snow., J. Geophys. Res., 106, 5385&amp;ndash;5402, 2001. </reference>
		<reference numeration="14" content_type="text"> Jacobson, M Z.: Fundamentals of Atmospheric Modeling, Second Edition, Cambridge University Press, New York, 2005. </reference>
		<reference numeration="15" content_type="text"> Jaenicke, R.: Aerosol-cloud-climate interactions, chap. Tropospheric aerosols, 1&amp;ndash;31, Academic Press, San Diego, 1993. </reference>
		<reference numeration="16" content_type="text"> Kerminen, V.-M. and Kulmala, M.: Analytical formulae connecting the &quot;real&quot; and the &quot;apparent&quot; nucleation rate and the nuclei number concentration for atmospheric nucleation events, J. Aerosol Science, 33, 609&amp;ndash;622, 2002. </reference>
		<reference numeration="17" content_type="text"> Korhonen, H., Kerminen, V.-M., Lehtinen, K. E J., and Kulmala, M.: CCN activation and cloud processing in sectional aerosol models with low size resolution, Atmos. Chem. Phys., 5, 2561&amp;ndash;2570, 2005. </reference>
		<reference numeration="18" content_type="text"> Kulmala, M., Lehtinen, K. E J., and Laaksonen, A.: Cluster activation theory as an explanation of the linear dependence between formation rate of 3 nm particles and sulphuric acid concentration, Atmospheric Chemistry and Physics, 6, 787&amp;ndash;793, available at:http://www.atmos-chem-phys.net/6/787/2006/, 2006. </reference>
		<reference numeration="19" content_type="text"> Lehtinen, K. E J., Rannik, U., Kulmala, M., and Hari, P.: Nucleation rate and vapour concentration estimations using a least squares aerosol dynamics method, J. Geophys. Res., 109, D21209, \doi10.1029/2004JD004893, 2004. </reference>
		<reference numeration="20" content_type="text"> Liao, H. and Seinfeld, J.: Global impacts of gas-phase chemistry-aerosol interactions on direct radiative forcing by anthropogenic aerosols and ozone, J. Geophys. Res., 110, D18208, \doi10.1029/ 2005JD005907, 2005. </reference>
		<reference numeration="21" content_type="text"> Liu, H Q., Pinker, R T., and Holben, B N.: A global view of aerosols from merged transport models, satellite, and ground observations, J. Geophys. Res., 110, D10S15, \doi10.1029/ 2004JD004695, 2005. </reference>
		<reference numeration="22" content_type="text"> McFiggans, G., Artaxo, P., Baltensperger, U., Coe, H., Facchini, M C., Feingold, G., Fuzzi, S., Gysel, M., Laaksonen, A., Lohmann, U., Mentel, T F., Murphy, D M., O&apos;Dowd, C D., Snider, J R., and Weingartner, E.: The effect of physical and chemical aerosol properties on warm cloud droplet activation, Atmos. Chem. Phys., 6, 2593&amp;ndash;2649, available at: http://www.atmos-chem-phys.net/6/2593/2006/, 2006. </reference>
		<reference numeration="23" content_type="text"> McGraw, R.: Description of aerosol dynamics by the quadrature method of moments, Aerosol Sci. Tech., 27, 255&amp;ndash;265, 1997. </reference>
		<reference numeration="24" content_type="text"> Moteki, N., Kondo, Y., Miyazaki, Y., Takegawa, N., Komazaki, Y., Kurata, G., Shirai, T., Blake, D R., R., Miyakawa, T., and Koike, M.: Evolution of mixing state of black carbon particles: Aircraft measurements over the western Pacific in March, Geophys. Res. Lett., 34, doi:10.1029/2006GL028943, 2004. </reference>
		<reference numeration="25" content_type="text"> Myhre, G., Stordahl, F., Berglen, T., Sundet, J., and Isaksen, I.: Uncertainties in the radiative forcing due to sulphate aerosols, J. Atmos. Sci., 61, 485&amp;ndash;498, 2004. </reference>
		<reference numeration="26" content_type="text"> Napari, I., Noppel, M., Vehkamaki, H., and Kulmala, M.: An improved model for ternary nucleation of sulfuric acid&amp;ndash;ammonia&amp;ndash;water, J. Chem. Phys., 116, 4221&amp;ndash;4227, available at:http://link.aip.org/link/?JCP/116/4221/1, 2002a. </reference>
		<reference numeration="27" content_type="text"> Napari, I., Noppel, M., Vehkamäki, H., and Kulmala, M.: Parameterization of ternary nucleation rates for H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt; &amp;ndash; NH&lt;sub&gt;3&lt;/sub&gt; &amp;ndash; H&lt;sub&gt;2&lt;/sub&gt;O vapors., J. Geophys. Res., 107, p 4381, \doi10.1029/2002JD002132, 2002b. </reference>
		<reference numeration="28" content_type="text"> Reddy, M S., Boucher, O., Bellouin, N., Schulz, M., Balkanski, Y., Dufresne, J. L., and Pham, M.: Estimates of global multicomponent aerosol optical depth and direct radiative perturbation in the Laboratoire de Meteorologie Dynamique general circulation model, J. Geophys. Res., 110, D10S16, \doi10.1029/2004JD004757, 2005. </reference>
		<reference numeration="29" content_type="text"> Riemer, N., Vogel, H., and Vogel, B.: Soot aging time scales in polluted regions during day and night, Atmos. Chem. Phys., 4, 1885&amp;ndash;1893, 2004. </reference>
		<reference numeration="30" content_type="text"> Riipinen, I., Sihto, S.-L., Kulmala, M., Arnold, F., Dal~Maso, M., Birmili, W., Saarnio, K., Teinilä, K., Kerminen, V.-M., Laaksonen, A., and Lehtinen, K. E J.: Connections between atmospheric sulphuric acid and new particle formation during QUEST III, IV campaigns in Heidelberg and Hyytiälä, Atmos. Chem. Phys., 7, 1899&amp;ndash;1914, available at:http://www.atmos-chem-phys.net/7/1899/2007/, 2007. </reference>
		<reference numeration="31" content_type="text"> Rodriguez, M. and Dabdub, D J.: IMAGES-SCAPE2: A modeling study of size and chemically resolved aerosol thermodynamics in a global chemical transport model, J. Geophys. Res., 109, D02203, \doi10.1029/2003JD003639, 2004. </reference>
		<reference numeration="32" content_type="text"> Seinfeld, J H. and Pandis, S N.: Atmospheric Chemistry and Physics, John Wiley and Sons inc., 1998. </reference>
		<reference numeration="33" content_type="text"> Sihto, S.-L., Kulmala, M., Kerminen, V.-M., Dal~Maso, M., Petäjä, T., Riipinen, I., Korhonen, H., Arnold, F., Janson, R., Boy, M., Laaksonen, A., and Lehtinen, K. E J.: Atmospheric sulphuric acid and aerosol formation: implications from atmospheric measurements for nucleation and early growth mechanisms, Atmos. Chem. Phys., 6, 4079&amp;ndash;4091, available at: http://www.atmos-chem-phys.net/6/4079/2006/, 2006. </reference>
		<reference numeration="34" content_type="text"> Spracklen, D V., Springle, K S., Carslaw, K S., Chipperfield, M P., and Mann, G W.: A global off-line model of size-resolved aerosol microphysics, Atmos. Chem. Phys., 5, 3233&amp;ndash;3250, 2005. </reference>
		<reference numeration="35" content_type="text"> Stier, P., Feichter, J., Kinne, S., Kloster, S., Vignati, E., Wilson, J., Ganzeveld, L., Tegen, I., Werner, M., Balkanski, Y., Schulz, M., Boucher, O., Minikin, A., and Petzold, A.: The aerosol-climate model ECHAM5-HAM, Atmos. Chem. Phys., 5, 1125&amp;ndash;1156, 2005. </reference>
		<reference numeration="36" content_type="text"> Stokes, R H. and Robinson, R A.: Interactions in aqueous nonelectrolyte solutions. I. Solute-solvent equilibria, J. Phys. Chem., 70, 2126&amp;ndash;2130, 1996. </reference>
		<reference numeration="37" content_type="text"> Vehkamäki, H., Kulmala, M., Napari, I., Lehtinen, K. E J., Timmreck, C., Noppel, M., and Laaksonen, A.: An improved parameterization for sulfuric acid-water nucleation rates for tropospheric and stratospheric conditions, J. Geophys. Res., 107, 4622, \doi10.1029/2002JD002184, 2002. </reference>
		<reference numeration="38" content_type="text"> Weisenstein, D K., Penner, J E., Herzog, M., and Liu, X.: Global 2-D intercomparison of sectional and modal aerosol modules, Atmos. Chem. Phys., 7, 2339&amp;ndash;2355, available at:http://www.atmos-chem-phys.net/7/2339/2007/, 2007. </reference>
		<reference numeration="39" content_type="text"> Wilson, J., Cuvelier, C., and Raes, F.: A modeling study of global mixed aerosol fields, J. Geophys. Res., 106, 34 081&amp;ndash;34 108, 2001. </reference>
		<reference numeration="40" content_type="text"> Zhang, Y., Seigneur, C., Seinfeld, J H., Jacobson, M Z., and Binkowski, F S.: Simulation of Aerosol Dynamics: A Comparative Review of Algorithms Used in Air Quality Models, Aerosol Sci. Tech., 31, 487&amp;ndash;514, 1999. </reference>
		<reference numeration="41" content_type="text"> Zuberi, B., Johnson, K., Aleks, G K., Molina, L T., and Molina, M J.: Hydrophilic properties of aged soot, Geophys. Res. Lett., 32, L01807, \doi10.1029/2004GL021496, 2005. </reference>
	</references>
</article>

