Atmos. Chem. Phys. Discuss., 7, 17179-17211, 2007
www.atmos-chem-phys-discuss.net/7/17179/2007/
doi:10.5194/acpd-7-17179-2007
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Ozone-enhanced layers in the troposphere over the equatorial Pacific Ocean and the influence of transport of midlatitude UT/LS air
H. Hayashi1, K. Kita1, and S. Taguchi2
1Department of Environmental Sciences, College of Science, Ibaraki University, Mito, Japan
2Research Institute for Environmental Management Technology, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Japan

Abstract. Occurrence of ozone (O3)-enhanced layers in the troposphere over the equatorial Pacific Ocean and their seasonal variation were investigated based on ozonesonde data obtained at three Southern Hemisphere ADditional OZonesondes (SHADOZ) sites, Watukosek, American Samoa and San Cristobal, for 6 years between 1998 and 2003. O3-enhanced layers were found in about 50% of observed O3 profiles at the three sites on yearly average. The formation processes of O3-enhanced layers were investigated by meteorological analyses including backward trajectories. On numerous occasions, O3-enhanced layers resulted from the transport of air masses affected by biomass burning. The contribution of this process was about 30% at San Cristobal during the periods from February to March and from August to September, while it was relatively low, about 10%, at Watukosek and Samoa. A significant number of the O3-enhanced layers were attributed to the transport of midlatitude upper-troposphere and lower-stratosphere (UT/LS) air. Meteorological analyses indicated that these layers originated from equatorward and downward transport of the midlatitude UT/LS air masses through a narrow region between high- and low-pressure systems around the subtropical jet stream. This process accounted for more than 40% at Watukosek between May and December, about 60% or more at Samoa all year around, and about 40% at San Cristobal between November and March, indicating that it was important for O3 budget over the equatorial Pacific Ocean.

Citation: Hayashi, H., Kita, K., and Taguchi, S.: Ozone-enhanced layers in the troposphere over the equatorial Pacific Ocean and the influence of transport of midlatitude UT/LS air, Atmos. Chem. Phys. Discuss., 7, 17179-17211, doi:10.5194/acpd-7-17179-2007, 2007.
 
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