<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys-discuss.net/inc/acpd/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>7</volume_number>
		<issue_number>6</issue_number>
		<publication_year>2007</publication_year>
	</journal>
	<doi>10.5194/acpd-7-15955-2007</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/7/15955/2007/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/7/15955/2007/acpd-7-15955-2007.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/7/15955/2007/acpd-7-15955-2007.pdf</fulltext_pdf>
	<start_page>15955</start_page>
	<end_page>15987</end_page>
	<publication_date>2007-11-14</publication_date>
	<article_title content_type="html">Numerical modeling of Asian dust emission and transport with adjoint inversion using LIDAR network observations</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>K. Yumimoto</name>
			<email>yumimoto@riam.kyushu-u.ac.jp</email>
		</author>
		<author numeration="2" affiliations="2">
			<name>I. Uno</name>
		</author>
		<author numeration="3" affiliations="3">
			<name>N. Sugimoto</name>
		</author>
		<author numeration="4" affiliations="3">
			<name>A. Shimizu</name>
		</author>
		<author numeration="5" affiliations="4">
			<name>Z. Liu</name>
		</author>
		<author numeration="6" affiliations="5">
			<name>D. M. Winker</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Department of Earth System Science and Technology, Kyushu University, Fukuoka, Japan</affiliation>
		<affiliation numeration="2" content_type="html">Research Institute for Applied Mechanics, Kyushu University, Fukuoka, Japan</affiliation>
		<affiliation numeration="3" content_type="html">National Institute for Environmental Study, Tsukuba, Japan</affiliation>
		<affiliation numeration="4" content_type="html">National Institute of Aerospace, Hampton, Virginia, USA</affiliation>
		<affiliation numeration="5" content_type="html">NASA Langley Research Center, Hampton, Virginia, USA</affiliation>
	</affiliations>
	<abstract content_type="html">A four-dimensional variational (4D-Var) data assimilation system for a
regional dust model (RAMS/CFORS-4DVAR; RC4) is applied to a heavy dust event
which occurred between 20 March and 4 April 2007 over eastern Asia. The
vertical profiles of the dust extinction coefficients derived from NIES
LIDAR observation network are directly assimilated. We conduct two
experiments to evaluate impacts of selections of observation sites:
Experiment A uses five Japanese observation sites located only downwind of
dust source regions; the other Experiment B uses these sites together with
two other sites near source regions (China and Korea). Validations using
various observation data (e.g., PM&lt;sub&gt;10&lt;/sub&gt; concentration, MODIS AOT, OMI
Aerosol Index, and the dust extinction coefficient derived by space-based
LIDAR NASA/CALIPSO) are demonstrated. The modeled dust extinction
coefficients are improved considerably through the assimilation.
Assimilation results of Experiment A are consistent with those of Experiment
B, indicating that observations of Experiment A can capture the dust event
correctly and include sufficient information for dust emission inversion.
Time series of dust AOT calculated by modeled and LIDAR dust extinction
coefficients show good agreement. At Seoul, Matsue, and Toyama, assimilation
reduces the root mean square errors of dust AOT by 31&amp;ndash;32%. Vertical
profiles of the dust layer observed by CALIPSO are also compared with
assimilation results. The dense dust layer was trapped between θ=280&amp;ndash;300 K and elevated higher toward the north; the
model reproduces those characteristics well. The modeled dust AOT along the
orbit paths agrees well with the CALIPSO dust AOT, OMI AI, and the coarse
mode AOT retrieved from MODIS; especially the modeled dust AOT and the MODIS
coarse mode AOT are consistent quantitatively. Assimilation results increase
dust emissions over the Gobi Desert and Mongolia considerably; especially
between 29 and 30 March, emission flux is increased by about 2&amp;ndash;3 times. The
heavy dust event is caused by the heavy dust uplift flux over the Gobi
Desert and Mongolia during those days. We obtain the total optimized dust
emissions of 57.9 Tg (Experiment A; 57.8% larger than before
assimilation) and 56.3 Tg (Experiment B; 53.4% larger).</abstract>
	<references>
		<reference numeration="1" content_type="text"> Awaji, T., Masuda, S., Ishikawa, Y., Sugiura, N., Toyoda, T., and Nakajima, T.: State estimation of the North Pacific Ocean by a four-dimensional variational data assimilation experiment, J. Oceanogr., 59, 931&amp;ndash;943, 2003. </reference>
		<reference numeration="2" content_type="text"> Benjamin, S. G., Dévényi, D., Weygandt, S. S., et al.: An hourly assimilation-forecast cycle: The RUC, Mon. Weather Rev., 132(2), 495&amp;ndash;518, 2004. </reference>
		<reference numeration="3" content_type="text"> Carmichael, G. R., Sandu, A., Chai, T., Daescu, D. N., Constantinescu, E. M., and Tang Y.: Predicting Air Quality: Current Status and Future Directions, J. Comput. Phys., in press, 2007. </reference>
		<reference numeration="4" content_type="text"> Chai, T., Carmichael, G. R., Sandu, A., Tang, Y., and Daescu D. N.: Chemical data assimilation of transport and chemical evolution over the Pacific (TRACE-P) aircraft measurements, J. Geophys. Res., 111, D02301, doi:10.1029/2005JD005883, 2006. </reference>
		<reference numeration="5" content_type="text"> Chai, T., Carmichael, G. R., Tang, Y., et al.: Four-dimensional data assimilation experiments with International Consortium for Atmospheric Research on Transport and Transformation ozone measurement, J. Geophys. Res., 112, D12S15, doi:10.1029/2006JD007763, 2007. </reference>
		<reference numeration="6" content_type="text"> Draxler, R. R. and Hess, G. D.: An overview of the HYSPLIT_4 modelling system for trajectories, dispersion, and deposition, Aust. Meteorol. Mag., 47, 295&amp;ndash;308, 1998. </reference>
		<reference numeration="7" content_type="text"> Elbern, H. and Schmidt, H.: A 4D-Var chemistry data assimilation scheme for Eulerian chemistry transport modeling, J. Geophys. Res., 104(D15), 18 583&amp;ndash;18 598, 1999. </reference>
		<reference numeration="8" content_type="text"> Elbern, H. and Schmidt H.: Ozone episode analysis by four-dimensional variational chemistry data assimilation, J. Geophys. Res., 106(D4), 3569&amp;ndash;3590, 2001. </reference>
		<reference numeration="9" content_type="text"> Elbern, H., Schmidt, H., and Ebel A.: Variational data assimilation for tropospheric chemistry modeling, J. Geophys. Res., 102(D13), 15 967&amp;ndash;15 985, 1997. </reference>
		<reference numeration="10" content_type="text"> Elbern, H., Strunk, A., Schmidt, H., and Talagrand O.: Emission rate and chemical state estimation by 4-dimensional variational inversion, Atmos. Chem. Phys., 7, 3749&amp;ndash;3769, 2007. </reference>
		<reference numeration="11" content_type="text"> Fernald, F. G.: Analysis of atmospheric LIDAR observations: Some comments, Appl. Opt., 23, 652&amp;ndash;653, 1984. </reference>
		<reference numeration="12" content_type="text"> Gong, S. L., Zhang, X. Y., Zhao, T. L., McKendry, I. G., Jaffe, D. A., and Lu, N. M.: Characterization of soil dust aerosol in China and its transport and distribution during 2001 ACE-Asia: 2. Model simulation and validation, J. Geophys. Res., 108(D9), 4262, doi:10.1029/2002JD002633, 2003. </reference>
		<reference numeration="13" content_type="text"> Hakami, A., Henze, D. K., Seinfeld, J. H., Chai, T., Tang, Y., Carmichael, G. R., and Sandu, A.: Adjoint inverse modeling of black carbon during the Asian Pacific Regional Aerosol Characterization Experiment, J. Geophys. Res., 110, D14301, doi:10.1029/2004JD005671, 2005. </reference>
		<reference numeration="14" content_type="text"> Henze, D. K., Hakami, A., and Seinfeld, J. H.: Development of the adjoint of GEOS-Chem, Atmos. Chem. Phys., 7, 2431&amp;ndash;2433, 2007. </reference>
		<reference numeration="15" content_type="text"> Hu, X. Q., Lu, N. M., Niu, T., and Zhang P.: Operational retrieval of Asian sand and dust storm from FY-2C geostationary meteorological satellite and its application to real time forecast in Asia, Atmos. Chem. Phys. Discuss., 7, 8395&amp;ndash;8421, 2007. </reference>
		<reference numeration="16" content_type="text"> Liu, D. C. and Nocedal J.: On the limited memory BFGS method for large scale optimization, Math. Program., 45, 503&amp;ndash;528, 1989. </reference>
		<reference numeration="17" content_type="text"> Liu, Z., Sugimoto, N., and Murayama T.: Extinction-to-backscatter ratio of Asian dust observed with high-spectral-resolution LIDAR and Raman LIDAR, Appl. Optics, 41, 2760&amp;ndash;2767, 2002. </reference>
		<reference numeration="18" content_type="text"> Liu, Z., Vaughan, M. A., Winker, D. M., Hostetler, C. A., Poole L. R., Hlavka, D., Hart, W., and McGill, M. Use of probability distribution functions for discriminating between cloud and aerosol in lidar backscatter data, J. Geophys. Res., 109, D15202, doi:10.1029/2004JD004732, 2004. </reference>
		<reference numeration="19" content_type="text"> Liu, M., Westphal, D. L., Wang, S., Shimizu, A., Sugimoto, N., Zhou, J., and Chen, Y.: A high-resolution numerical study of the Asian dust storms of April 2001, J. Geophys. Res., 108(D23), 8653, doi:10.1029/2002JD003178, 2003. </reference>
		<reference numeration="20" content_type="text"> Martien, P. T., Harley, R. A., and Cacuci, D. G.: Adjoint sensitivity analysis for a three-dimensional photochemical model: implementation and method comparison, Environ. Sci. Technol., 40(8), 2663&amp;ndash;2670, doi:10.1021/es0510257, 2006. </reference>
		<reference numeration="21" content_type="text"> Müller, J.-F. and Stavrakou, T.: Inversion of CO and NOx emissions using the adjoint of the IMAGES model, Atmos. Chem. Phys., 5, 1157&amp;ndash;1186, 2005. </reference>
		<reference numeration="22" content_type="text"> Niu, T., Gong, S. L., Zhu, G. F., Liu, H. L., Hu, X. Q., Zhou, C. H., and Wang, Y. Q.: Data assimilation of dust aerosol observations for CUACE/Dust forecasting system, Atmos. Chem. Phys. Discuss., 7, 8309&amp;ndash;8332, 2007. </reference>
		<reference numeration="23" content_type="text"> Overpeck, J., Rind, D., Lacis, A., and Healy, R.: Possible role of dust-induced regional warming in abrupt climate change during the last glacial period, Nature, 384, 447&amp;ndash;449, 1996. </reference>
		<reference numeration="24" content_type="text"> Pielke, R. A., Cotton, W. R., Walko, R. L., et al.: A comprehensive meteorological modeling system: RAMS, Meteorol. Atmos. Phys., 49, 69&amp;ndash;91, 1992. </reference>
		<reference numeration="25" content_type="text"> Remer, L. A., Kaufman, Y. J., Tanré, D., et al.: The MODIS Aerosol Algorithm, Products and Validation, J. Atmos. Sci., 62, 947&amp;ndash;973, 2005. </reference>
		<reference numeration="26" content_type="text"> Shao, Y., Yang, Y., Wang, J., et al.: Northeast Asian dust storms: Real-time numerical prediction and validation, J. Geophys. Res., 108(D22), 4691, doi:10.1029/2003JD003667, 2003. </reference>
		<reference numeration="27" content_type="text"> Shimizu, A., Sugimoto, N., Matsui, I., et al.: Continuous observations of Asian dust and other aerosols by polarization lidars in China and Japan during ACE-Asia, J. Geophys. Res., 109(D19S17), doi:10.1029/2002JD003253, 2004. </reference>
		<reference numeration="28" content_type="text"> Sokolik, I. N. and Toon, O. B.: Direct radiative forcing by anthropogenic airborne mineral aerosols, Nature, 381, 681&amp;ndash;683, 1996. </reference>
		<reference numeration="29" content_type="text"> Sugimoto, N., Matsui, I., Shimizu, A., Uno, I., Arai, K., Endoh, T., and Nakajima, T.: Observation of dust and anthropogenic aerosol plumes in the Northwest Pacific with a two-wavelength polarization lidar on board the research vessel Mirai, Geophys. Res. Lett., 29(19), 1901, doi:10.1029/2002GL015112, 2002. </reference>
		<reference numeration="30" content_type="text"> Sugimoto, N., Shimizu, A., Matsui, I., Dong, X., Zhou, J., Bai, X., Zhou, J., Lee, C.-H., Yoon, S.-C., Okamoto, H., and Uno, I.: NetworkObservations of Asian Dust and Air Pollution Aerosols UsingTwo-Wavelength Polarization Lidars, 23rd International Laser Radar Conference, July 2006 Nara, Japan (23ILRC, ISBN 4-9902916-0-3), 851&amp;ndash;854, 2006. </reference>
		<reference numeration="31" content_type="text"> Stavrakou, T. and Müller, J.-F.: Grid-based versus big region approach for inverting CO emissions using Measurement of Pollution in the Troposphere (MOPITT) data, J. Geophys. Res., 111, D15304, doi:10.1029/2005JD006896, 2006. </reference>
		<reference numeration="32" content_type="text"> Takemura, T., Okamura, H., Maruyama, Y., Numaguti, A., Higurashi, A., and Nakajima, T.: Global three-dimensional simulation of aerosol optimal thickness distribution of various origins, J. Geophys. Res., 105(17), 853&amp;ndash;17873, 2000. </reference>
		<reference numeration="33" content_type="text"> Tanaka, T. Y. and Chiba, M.: Global simulation of dust aerosol with a chemical transport model, MASINGAR, J. Meteorol. Soc. Jpn., 83A, 255&amp;ndash;278, 2005. </reference>
		<reference numeration="34" content_type="text"> Uno, I., Carmichael, G. R., Streets, D. G., et al.: Numerical study of Asian dust transport during the springtime of 2001 simulated with the Chemical Weather Forecasting System (CFORS) model, J. Geophys. Res., 109, D19S24, doi:10.1029/2003JD00422, 2004. </reference>
		<reference numeration="35" content_type="text"> Uno, I., Harada, K., Satake, S., Hara, Y., and Wang, Z.: Meteorological Characteristics and Dust Distribution of the Tarim Basin Simulated by the RAMS/CFORS Dust Model, J. Meteorol. Soc. Jpn., 83A, 219&amp;ndash;239, 2005. </reference>
		<reference numeration="36" content_type="text"> Uno, I., Wang, Z., Chiba, M., et al.: Dust model intercomparison (DMIP) study over Asia: Overview, J. Geophys. Res., 111, D12213, doi:10.1029/2005JD006575, 2006. </reference>
		<reference numeration="37" content_type="text"> Winker, D. M., Hunt, W. H., and McGill, M. J.: Initial performance assessment of CALIOP, Geophys. Res. Lett., 34, L19803, doi:10.1029/2007GL030135, 2007. </reference>
		<reference numeration="38" content_type="text"> Yumimoto, K. and Uno, I.: Adjoint inverse modeling of CO emissions over the East Asian region using four dimensional variational data assimilation, Atmos. Environ. 40, 6836&amp;ndash;6845, 2006. </reference>
		<reference numeration="39" content_type="text"> Yumimoto, K., Uno, I., Sugimoto, N., Shimizu, A., and Satake, S.: Adjoint inverse modeling of dust emission and transport over East Asia, Geophys. Res. Lett., 34, L00806, doi:10.029/2006GL028551, 2007. </reference>
	</references>
</article>

