<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys-discuss.net/inc/acpd/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>7</volume_number>
		<issue_number>5</issue_number>
		<publication_year>2007</publication_year>
	</journal>
	<doi>10.5194/acpd-7-14511-2007</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/7/14511/2007/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/7/14511/2007/acpd-7-14511-2007.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/7/14511/2007/acpd-7-14511-2007.pdf</fulltext_pdf>
	<start_page>14511</start_page>
	<end_page>14542</end_page>
	<publication_date>2007-10-11</publication_date>
	<article_title content_type="html">Trends and variability of midlatitude stratospheric water vapour deduced from the re-evaluated Boulder balloon series and HALOE</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>M. Scherer</name>
		</author>
		<author numeration="2" affiliations="2,3">
			<name>H. Vömel</name>
		</author>
		<author numeration="3" affiliations="4">
			<name>S. Fueglistaler</name>
			<email>s.fueglistaler@damtp.cam.ac.uk</email>
		</author>
		<author numeration="4" affiliations="3">
			<name>S. J. Oltmans</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>J. Staehelin</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Atmospheric and Climate Science, Eidgenössische Technische Hochschule, Zürich, Switzerland</affiliation>
		<affiliation numeration="2" content_type="html">Cooperative Institute for Research in Environmental Science, University of Colorado, Boulder, CO, USA</affiliation>
		<affiliation numeration="3" content_type="html">Global Monitoring Division, Earth System Research Laboratory, NOAA, Boulder, CO, USA</affiliation>
		<affiliation numeration="4" content_type="html">Applied Mathematics and Theoretical Physics, Cambridge University, Cambridge, UK</affiliation>
	</affiliations>
	<abstract content_type="html">This paper presents an updated trend analysis of water vapour in the
lower midlatitude stratosphere from the Boulder balloon-borne NOAA
frostpoint hygrometer measurements and from the Halogen Occulation
Experiment (HALOE).
Two corrections for instrumental bias are applied to homogenise the
frostpoint data series, and a quality assessment of all soundings after
1991 is presented.
Linear trend estimates based on the corrected data
for the period 1980&amp;ndash;2000 are up to  40% lower than previously reported.
Vertically resolved trends and variability are calculated with a multi
regression analysis including the quasi-biennal oscillation and equivalent
latitude as explanatory variables.
In the range of 380 to 640 K potential temperature
(&amp;asymp;14 to 25 km), the frostpoint data from 1981 to 2006 show
positive linear trends between 0.3&amp;plusmn; 0.3 and 0.7&amp;plusmn;0.1%/yr.
The same dataset shows trends between &amp;minus;0.2&amp;plusmn;0.3 and 1.0&amp;plusmn;0.3%/yr
for the period 1992 to 2005.
HALOE data over the same time period suggest negative trends ranging
from &amp;minus;1.1&amp;plusmn;0.2 to &amp;minus;0.1&amp;plusmn;0.1%/yr.
In the lower stratosphere, a rapid drop of water vapour is observed in
2000/2001 with little change since.
At higher altitudes, the transition is more gradual, with slowly
decreasing concentrations between 2001 and 2007.
This pattern is consistent with a change induced by a drop of water
concentrations at entry into the stratosphere.
Previously noted differences in trends and variability between frostpoint
and HALOE remain for the homogenised data.
Due to  uncertainties in reanalysis temperatures and
stratospheric transport combined with uncertainties in
observations,
 no quantitative inference about changes of water entering the
stratosphere in the tropics could be made with the mid latitude
measurements analysed here.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Andrews, A E., Boering, K A., Wofsy, S C., Daube, B C., Jones, D B., Alex, S., Loewenstein, M., Podolske, J R., and Strahan, S E.: Empirical age spectra for the midlatitude lower stratosphere from in situ observations of CO&lt;sub&gt;2&lt;/sub&gt;: Quantitative evidence for a subtropical &quot;barrier&quot; to horizontal transport, J. Geophys. Res., 106, 10 257&amp;ndash;10 274, \doi10.1029/2000JD900703, 2001. </reference>
		<reference numeration="2" content_type="text"> Austin, J. and Li, F.: On the relationship between the strength of the Brewer-Dobson circulation and the age of stratospheric air, Geophys. Res. Lett., 33, L17807, \doi10.1029/2006GL026867, 2006. </reference>
		<reference numeration="3" content_type="text"> Austin, J., Wilson, J., Feng, L., and Vömel, H.: Evolution of water vapor concentrations and stratsophereic age of air in coupled chemistry-climate model simulations, J. Atmos. Sci., 64, 905&amp;ndash;921, \doi10.1175/JAS3866.1, 2007. </reference>
		<reference numeration="4" content_type="text"> Baldwin, M P., Gray, L J., Dunkerton, T J., Hamilton, K., Haynes, P H., Randel, W J., Holton, J R., Alexander, M J., Hirota, I., Horinouchi, T., Jones, D B A., Kinnersley, J S., Marquardt, C., Sato, K., and Takahashi, M.: The quasi-biennial oscillation, Rev. Geophys., 39, 179&amp;ndash;230, \doi10.1029/1999RG000073, 2001. </reference>
		<reference numeration="5" content_type="text"> Bojkov, R D. and Fioletov, V E.: Estimating the global ozone characteristics during the last 30 years, J. Geophys. Res., 100, 16 537&amp;ndash;16 552, \doi10.1029/95JD00692, 1995. </reference>
		<reference numeration="6" content_type="text"> Butchart, N. and Scaife, A A.: Removal of chlorofluorocarbons by increased mass exchange between the stratosphere and troposphere in a changing climate, Nature, 410, 799&amp;ndash;802, 2001. </reference>
		<reference numeration="7" content_type="text"> Chiou, E W., Thomason, L W., and Chu, W P.: Variability of Stratosphereric Water Vapor Inferred from SAGE II, HALOE, and Boulder (Colorado) Balloon Measurements, J. Climate, 4121&amp;ndash;4133, \doi10.1175/JCLI3841.1, 2006. </reference>
		<reference numeration="8" content_type="text"> Dlugokencky, E J., Houweling, S., Bruhwiler, L., Masarie, K A., Lang, P M., Miller, J B., and Tans, P P.: Atmospheric methane levels off: Temporary pause or a new steady-state?, Geophys. Res. Lett., 30, 1992, doi:10.1029/2003GL018126, 2003. </reference>
		<reference numeration="9" content_type="text"> Dvortsov, V L. and Solomon, S.: Response of the stratospheric temperatures and ozone to past and future increases in stratospheric humidity, J. Geophys. Res., 106, 7505&amp;ndash;7514, \doi10.1029/2000JD900637, 2001. </reference>
		<reference numeration="10" content_type="text"> Forster, P M d F. and Shine, K P.: Assessing the climate impact of trends in stratospheric water vapor, Geophys. Res. Lett., 29, 10&amp;ndash;1, 2002. </reference>
		<reference numeration="11" content_type="text"> Fueglistaler, S. and Haynes, P H.: Control of interannual and longer-term variability of stratospheric water vapor, J. Geophys. Res., 110, D24108, \doi10.1029/2005JD006019, 2005. </reference>
		<reference numeration="12" content_type="text"> Fueglistaler, S., Bonazzola, M., Haynes, P H., and Peter, T.: Stratospheric water vapor predicted from the Lagrangian temperature history of air entering the stratosphere in the tropics, J. Geophys. Res., 110, D08 107, \doi10.1029/2004JD005516, 2005. </reference>
		<reference numeration="13" content_type="text"> Giorgetta, M A. and Bengtsson, L.: Potential role of the quasi-biennial oscillation in the stratosphere-troposphere exchange as found in water vapor in general circulation model experiments, J. Geophys. Res., 104, 6003&amp;ndash;6020, \doi10.1029/1998JD200112, 1999. </reference>
		<reference numeration="14" content_type="text"> Holton, J R.: On the Global Exchange of Mass between the Stratosphere and Troposphere., J. Atmos. Sci., 47, 392&amp;ndash;396, 1990. </reference>
		<reference numeration="15" content_type="text"> Holton, J R., Haynes, P H., McIntyre, M E., Douglass, A R., Rood, R B., and Pfister, L.: Stratosphere-troposphere exchange, Rev. Geophys., 33, 403&amp;ndash;439, 1995. </reference>
		<reference numeration="16" content_type="text"> Joshi, M M. and Shine, K P.: A GCM Study of Volcanic Eruptions as a Cause of Increased Stratospheric Water Vapor., J. Clim., 16, 3525&amp;ndash;3534, 2003. </reference>
		<reference numeration="17" content_type="text"> Kalnay, E., Kanamitsu, M., Kistler, R., Collins, W., Deaven, D., Gandin, L., Iredell, M., Saha, S., White, G., Woollen, J., Zhu, Y., Leetmaa, A., Reynolds, B., Chelliah, M., Ebisuzaki, W., Higgins, W., Janowiak, J., Mo, K C., Ropelewski, C., Wang, J., Jenne, R., and Joseph, D.: The NCEP/NCAR 40-Year Reanalysis Project., B. Am. Meteorol. Soc., 77, 437&amp;ndash;472, 1996. </reference>
		<reference numeration="18" content_type="text"> Kley, D., Russell III, J M., and Philips, C., eds.: SPARC assessment of upper tropospheric and stratospheric water vapour, WCRP 113, WMO/TD No. 1043, SPARC Report Nr.2, World Meteorol. Organ., 2000. </reference>
		<reference numeration="19" content_type="text"> Layton, E C.: Report of the determination of exactness of fit of thermistor to the equations $\log R = A + B/(T + \Theta)$ and $ \log R = A + B/(T +\Theta) + CT$, Tech. Rep. 2168, U.S. Army Signal Res. and Dev. Lab, 1961. </reference>
		<reference numeration="20" content_type="text"> Le Texier, H., Solomon, S., and Garcia, R R.: The role of molecular hydrogen and methane oxidation in the water vapour budget of the stratosphere, Q. J. Roy. Meteorol. Soc., 114, 281&amp;ndash;295, 1988. </reference>
		<reference numeration="21" content_type="text"> Notholt, J., Luo, B P., Fueglistaler, S., Weisenstein, D., Rex, M., Lawrence, M G., Bingemer, H., Wohltmann, I., Corti, T., Warneke, T., von Kuhlmann, R., and Peter, T.: Influence of tropospheric SO&lt;sub&gt;2&lt;/sub&gt; emissions on particle formation and the stratospheric humidity, Geophys. Res. Lett., 32, L07810, \doi10.1029/2004GL022159, 2005. </reference>
		<reference numeration="22" content_type="text"> Oltmans, S J.: Measurements of water vapor in the stratosphere with a frost point hygrometer, Measurement and Control in Science and Industry, in: Proceedings of the 1985 International Symposium on Moisture and Humidity, pp. 251&amp;ndash;258, Instrument Society of America, Washington, D. C., 1985. </reference>
		<reference numeration="23" content_type="text"> Oltmans, S J. and Hofmann, D J.: Increase in lower-stratospheric water vapour at a mid-latitude Northern Hemisphere site from 1981 to 1994, Nature, 374, 146&amp;ndash;149, 1995. </reference>
		<reference numeration="24" content_type="text"> Oltmans, S J., Vömel, H., Hofmann, D J., Rosenlof, K H., and Kley, D.: The increase in stratospheric water vapor from balloonborne, frostpoint hygrometer measurements at Washington, D.C., and Boulder, Colorado, Geophys. Res. Lett., 27, 3453&amp;ndash;3456, \doi10.1029/2000GL012133, 2000. </reference>
		<reference numeration="25" content_type="text"> Plumb, R A.: A &quot;tropical pipe&quot; model of stratospheric transport, J. Geophys. Res., 101, 3957&amp;ndash;3972, \doi10.1029/95JD03002, 1996. </reference>
		<reference numeration="26" content_type="text"> Randel, W J., Zawodny, J M., and Oltmans, S J.: Seasonal variation of water vapor in the lower stratosphere observed in Halogen Occultation Experiment data, J. Geophys. Res., 106, 14 313&amp;ndash;14 326, \doi10.1029/2001JD900048, 2001. </reference>
		<reference numeration="27" content_type="text"> Randel, W J., Wu, F., Oltmans, S J., Rosenlof, K., and Nedoluha, G E.: Interannual Changes of Stratospheric Water Vapor and Correlations with Tropical Tropopause Temperatures., J. Atmos. Sci., 61, 2133&amp;ndash;2148, 2004. </reference>
		<reference numeration="28" content_type="text"> Randel, W J., Wu, F., Vömel, H., Nedoluha, G E., and Forster, P.: Decreases in stratospheric water vapor after 2001: Links to changes in the tropical tropopause and the Brewer-Dobson circulation, J. Geophys. Res., 111, D12312, \doi10.1029/2005JD006744, 2006. </reference>
		<reference numeration="29" content_type="text"> Reinsel, G C., Weatherhead, E., Tiao, G C., Miller, A J., Nagatani, R M., Wuebbles, D J., and Flynn, L E.: On detection of turnaround and recovery in trend for ozone, J. Geophys. Res., 107, n.a., \doi10.1029/2001JD000500, 2002. </reference>
		<reference numeration="30" content_type="text"> Rohs, S., Schiller, C., Riese, M., Engel, A., Schmidt, U., Wetter, T., Levin, I., Nakazawa, T., and Aoki, S.: Long-term changes of methane and hydrogen in the stratosphere in the period 1978-2003 and their impact on the abundance of stratospheric water vapor, J. Geophys. Res., 111, D14315, \doi10.1029/2005JD006877, 2006. </reference>
		<reference numeration="31" content_type="text"> Rosenlof, K H., Chiou, E.-W., Chu, W P., Johnson, D G., Kelly, K. K., Michelsen, H A., Nedoluha, G E., Remsberg, E E., Toon, G C., and McCormick, M P.: Stratospheric water vapor increases over the past half-century, Geophys. Res. Lett., 28, 1195&amp;ndash;1198, \doi10.1029/2000GL012502, 2001. </reference>
		<reference numeration="32" content_type="text"> Russell, III, J M., Gordley, L L., Park, J H., Drayson, S R., Hesketh, W D., Cicerone, R J., Tuck, A F., Frederick, J E., Harries, J E., and Crutzen, P J.: The Halogen Occultation Experiment, J. Geophys. Res., 98, 10 777&amp;ndash;10 797, 1993. </reference>
		<reference numeration="33" content_type="text"> Scaife, A A., Butchart, N., Jackson, D R., and Swinbank, R.: Can changes in ENSO activity help to explain increasing stratospheric water vapor?, Geophys. Res. Lett., 30, 1880, doi:10.1029/2003GL017591, 2003. </reference>
		<reference numeration="34" content_type="text"> Seidel, D J., Ross, R J., Angell, J. K., and Reid, G C.: Climatological characteristics of the tropical tropopause as revealed by radiosondes, J. Geophys. Res., 106, 7857&amp;ndash;7878, \doi10.1029/2000JD900837, 2001. </reference>
		<reference numeration="35" content_type="text"> Sherwood, S.: A Microphysical Connection Among Biomass Burning, Cumulus Clouds, and Stratospheric Moisture, Science, 295, 1272&amp;ndash;1275, \doi10.1126/science.1065080, 2002. </reference>
		<reference numeration="36" content_type="text"> Shindell, D T.: Climate and ozone response to increased stratospheric water vapor, Geophys. Res. Lett., 28, 1551&amp;ndash;1554, \doi10.1029/1999GL011197, 2001. </reference>
		<reference numeration="37" content_type="text"> Sobel, A H., Plumb, R A., and Waugh, D W.: Methods of Calculating Transport across the Polar Vortex Edge., J. Atmos. Sci., 54, 2241&amp;ndash;2260, 1997. </reference>
		<reference numeration="38" content_type="text"> Stenke, A. and Grewe, V.: Simulation of stratospheric water vapor trends: impact on stratospheric ozone chemistry, Atmos. Chem. Phys., 5, 1257&amp;ndash;1272, 2005. </reference>
		<reference numeration="39" content_type="text"> Vömel, H., Oltmans, S J., Hofmann, D J., Deshler, T., and Rosen, J M.: The evolution of the dehydration in the Antarctic stratospheric vortex, J. Geophys. Res., 100, 13 919&amp;ndash;13 926, \doi10.1029/95JD01000, 1995. </reference>
		<reference numeration="40" content_type="text"> Vömel, H., David, D E., and Smith, K.: Accuracy of tropospheric and stratospheric water vapor measurements by the cryogenic frost point hygrometer: Instrumental details and observations, J. Geophys. Res., 112, D08305, \doi10.1029/2006JD007224, 2007a. </reference>
		<reference numeration="41" content_type="text"> Vömel, H., Yushkov, V., Khaykin, S., Korshunov, L., Kyrö, E., and Kivi, R.: Intercomparison of stratospheric water vapor sensors: FLASH-b and NOAA/CMDL frost point hygrometer, J. Atmos. Ocean. Tech., 27, 941&amp;ndash;952, \doi10.1175/JTECH2007.1, 2007b. </reference>
		<reference numeration="42" content_type="text"> Waugh, D. and Hall, T.: Age of stratospheric air: theory, observations, and models, Rev. Geophys., 40, 1&amp;ndash;1, \doi10.1029/2000RG000101, 2002. </reference>
		<reference numeration="43" content_type="text"> Weatherhead, E C. and Andersen, S B.: The search for signs of recovery of the ozone layer, Nature, 441, 39&amp;ndash;45, 2006. </reference>
		<reference numeration="44" content_type="text"> Zhou, X.-L., Geller, M A., and Zhang, M.: Cooling trend of the tropical cold point tropopause temperatures and its implications, J. Geophys. Res., 106, 1511&amp;ndash;1522, \doi10.1029/2000JD900472, 2001. </reference>
	</references>
</article>

