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10.5194/acpd-7-12067-2007
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http://www.atmos-chem-phys-discuss.net/7/12067/2007/acpd-7-12067-2007.pdf
12067
12095
2007-08-15
MIPAS measurements of upper tropospheric C<sub>2</sub>H<sub>6</sub> and O<sub>3</sub> during the Southern hemispheric biomass burning season in 2003
T. von Clarmann
N. Glatthor
G. P. Stiller
U. Grabowski
M. Höpfner
S. Kellmann
A. Linden
M. Milz
T. Steck
H. Fischer
B. Funke
M. E. Koukouli
Forschungszentrum Karlsruhe, Institut für Meteorologie und Klimaforschung, Karlsruhe, Germany
Instituto de Astrofίsica de Andalucίa CSIC, Granada, Spain
Laboratory of Atmospheric Physics, Physics Department, Aristotle University of Thessaloniki, Thessaloniki, Greece
now at: Institutionen för Rymdvetenskap, Luleå Tekniska Universitet, Kiruna, Sweden
Under cloud free conditions, the Michelson Interferometer
for Passive Atmospheric Sounding (MIPAS) provides measurements
of spectrally resolved limb radiances down to the upper troposphere.
These are used to infer global distributions of mixing ratios of
atmospheric constituents in the upper troposphere and the stratosphere.
From 21 October to 14 November 2003, MIPAS observed enhanced
amounts of upper tropospheric
C<sub>2</sub>H<sub>6</sub> (up to about 400 pptv, depending on spectroscopic data chosen)
and ozone (up to about 80 ppbv). By means of trajectory
calculations, the enhancements observed in the Southern hemisphere
are, at least partly, attributed to a biomass burning plume, which
covers wide parts of the Southern hemisphere, from South America,
the Atlantic ocean, Africa, the Indian Ocean to Australia.
The chemical composition of the part of the plume-like pollution
belt associated with South American rainforest burning appears
different from the part associated with Southern African savanna
burning. In particular, African savanna fires lead to a larger ozone
enhancement than South American rainforest fires.
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