Atmos. Chem. Phys. Discuss., 7, 10799-10835, 2007
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Vertical profiles of urban aerosol complex refractive index in the frame of ESQUIF airborne measurements
J.-C. Raut and P. Chazette
Laboratoire des Sciences du Climat et de l'Environnement, Laboratoire mixte CEA-CNRS-UVSQ, CEA Saclay, 91191 Gif-sur-Yvette, France

Abstract. A synergy between lidar, sunphotometer and in situ measurements has been applied to airborne observations performed during the Etude et Simulation de la QUalité de l'air en Ile-de-France (ESQUIF), enabling the retrieval of vertical profiles for the aerosol complex refractive index (ACRI) and single-scattering albedo with a vertical resolution of 200 m over Paris area. The averaged value over the entire planetary boundary layer (PBL) for the ACRI is close to 1.51(±0.02)–i0.017(±0.003) at 532 nm. The single-scattering albedo of the corresponding aerosols is found to be ~0.9 at the same wavelength. A good agreement is found with previous studies for urban aerosols. A comparison of vertical profiles of ACRI with simulations combining in situ measurements and relative humidity (RH) profiles has highlighted a modification in aerosol optical properties linked to their history and the origin of the air mass. The determination of ACRI in the atmospheric column enabled to retrieve vertical profiles of extinction coefficient in accordance with lidar profiles measurements.

Citation: Raut, J.-C. and Chazette, P.: Vertical profiles of urban aerosol complex refractive index in the frame of ESQUIF airborne measurements, Atmos. Chem. Phys. Discuss., 7, 10799-10835, doi:10.5194/acpd-7-10799-2007, 2007.
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