Atmospheric Chemistry and Physics Discussions www.atmos-chem-phys-discuss.net 1680-7367 1680-7375 6 5 2006 10.5194/acpd-6-9967-2006 http://www.atmos-chem-phys-discuss.net/6/9967/2006/ http://www.atmos-chem-phys-discuss.net/6/9967/2006/acpd-6-9967-2006.html http://www.atmos-chem-phys-discuss.net/6/9967/2006/acpd-6-9967-2006.pdf 9967 9994 2006-10-10 A study of polar ozone depletion based on sequential assimilation of satellite data from the ENVISAT/MIPAS and Odin/SMR instruments J. D. Rösevall D. P. Murtagh J. Urban A. K. Jones Department of Radio & Space Science, Chalmers Univ. of Technology, Göteborg, Sweden A fire storm that occured on 28 May 2001 devastated the town of Chisholm, ~150 km north of Edmonton, Alberta, induced a violent fire-invigorated cumulonimbus cloud. This pyro-cumulonimbus (pyro-Cb) had overshooting tops of 2.5&ndash;3 km above the tropopause, and injected massive amounts of smoke into the lower stratosphere. Fortunately, this event occurred under good coverage of radar, rain gauge, lightning and satellite measurements, which allowed in-depth documentation of the event. <br><br> The combination of heat and smoke created a cloud with extremely small drops, which ascended rapidly in violent updrafts. There appeared to be little freezing up to the homogeneous freezing isotherm level of &ndash;38&deg;C. A cloud with such small and short-lived highly supercooled drops is incapable of producing precipitation except for few large graupel and hail, which produced the observed radar echoes and charged the cloud with positive lightning. The small cloud drops froze homogeneously to equally small ice particles, for which there is no mechanism to aggregate into precipitation particles that hence remain in the anvil. The small precipitation efficiency implies that only a small fraction of the smoke is scavenged, so that most of it is exhausted through the anvil to the upper troposphere and lower stratosphere. <br><br> Comparisons with other cases suggest that a pyro-Cb does not have to be as violent as the Chisholm case to have strongly suppressed precipitation. However, this level of convective vigor is necessary to create the overshooting updraft that injects the smoke into the lower stratosphere.