Atmos. Chem. Phys. Discuss., 6, 9003-9032, 2006
www.atmos-chem-phys-discuss.net/6/9003/2006/
doi:10.5194/acpd-6-9003-2006
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Solid particles in the tropical lowest stratosphere
J. K. Nielsen1, N. Larsen1, F. Cairo2, G. Di Donfrancesco3, J. M. Rosen4, G. Durry5,7, G. Held6, and J. P. Pommereau7
1Danish Meteorological Institute, Lyngbyvej 100, 2100 Kbh. Ø, Denmark
2Institute for Atmospheric Science and Climate, CNR, Via del Fosso del Cavaliere 100, 00133 Rome, Italy
3Italian National Agency for New Technologies, Energy and Environment, ENEA C. R. Cassaccia, Via Anguillarese 301, 00060 Rome, Italy
4University of Wyoming, Department of Physics and Astronomy, Laramie, Wyoming 82071
543;Groupe de Spectrometrie Moleculaire et Atmospherique, CNRS, Universite de Reims , 51687 Reims, France
6Instituto de Pesquisas Meteorolgicas, Universidade Estadual Paulista, CX Postal, 281 17015-970 BAURU, S.P., Brasil
7CNRS, Institut Pierre Simon Laplace, Service d’Aeronomie, B.P. 3, 91371 Verrieres le Buisson Cedex, France

Abstract. We report in situ and remote observations proving occasional occurrence of solid particles in the tropical lowest stratosphere, far away from deep convective events. The particles were found during field campaigns in Southeast Brazil (49.03 W 22.36 S). They occur in the altitude range from 17.5 to 20.8 km, at temperatures up to at least 10 K above the expected frost point temperature. While stability of ice particles at these altitudes is unexpected from a theoretical point of view, it is argued that these observations are indications of tropospheric air masses penetrating into the stratosphere during convective overshoots. It is concluded that the intrusion of tropospheric air must have carried a large amount of water with it, which effectively hydrated the lowest stratosphere, and consequently suppressed sublimation. This conclusion is further supported by a separate water vapor mixing ratio profile obtained at the same observation site.

Citation: Nielsen, J. K., Larsen, N., Cairo, F., Di Donfrancesco, G., Rosen, J. M., Durry, G., Held, G., and Pommereau, J. P.: Solid particles in the tropical lowest stratosphere, Atmos. Chem. Phys. Discuss., 6, 9003-9032, doi:10.5194/acpd-6-9003-2006, 2006.
 
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