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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-6-8553-2006</article-id>
<title-group>
<article-title>Multi-model simulations of the impact of international shipping on atmospheric chemistry and climate in 2000 and 2030</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Eyring</surname>
<given-names>V.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Stevenson</surname>
<given-names>D. S.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Lauer</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dentener</surname>
<given-names>F. J.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Butler</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Collins</surname>
<given-names>W. J.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ellingsen</surname>
<given-names>K.</given-names>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Gauss</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hauglustaine</surname>
<given-names>D. A.</given-names>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Isaksen</surname>
<given-names>I. S. A.</given-names>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Lawrence</surname>
<given-names>M. G.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Richter</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff8">
<sup>8</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Rodriguez</surname>
<given-names>J. M.</given-names>
</name>
<xref ref-type="aff" rid="aff9">
<sup>9</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Sanderson</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Strahan</surname>
<given-names>S. E.</given-names>
</name>
<xref ref-type="aff" rid="aff9">
<sup>9</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Sudo</surname>
<given-names>K.</given-names>
</name>
<xref ref-type="aff" rid="aff10">
<sup>10</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Szopa</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>van Noije</surname>
<given-names>T. P. C.</given-names>
</name>
<xref ref-type="aff" rid="aff11">
<sup>11</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Wild</surname>
<given-names>O.</given-names>
</name>
<xref ref-type="aff" rid="aff10">
<sup>10</sup>
</xref>
<xref ref-type="aff" rid="aff12">
<sup>12</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>DLR, Institut für Physik der Atmosphäre, Oberpfaffenhofen, Germany</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>University of Edinburgh, School of GeoSciences, Edinburgh, United Kingdom</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>European Commission, Joint Research Centre, Institute for Environment and Sustainability, Ispra, Italy</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>Max Planck Institute for Chemistry, Mainz, Germany</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>Met Office, Exeter, United Kingdom</addr-line>
</aff>
<aff id="aff6">
<label>6</label>
<addr-line>University of Oslo, Department of Geosciences, Oslo, Norway</addr-line>
</aff>
<aff id="aff7">
<label>7</label>
<addr-line>Laboratoire des Sciences du Climat et de l’Environnement, Gif-sur-Yvette, France</addr-line>
</aff>
<aff id="aff8">
<label>8</label>
<addr-line>University of Bremen, Institute for Environmental Physics, Bremen, Germany</addr-line>
</aff>
<aff id="aff9">
<label>9</label>
<addr-line>Goddard Earth Science &amp; Technology Center (GEST), Maryland, Washington, DC, USA</addr-line>
</aff>
<aff id="aff10">
<label>10</label>
<addr-line>Frontier Research Center for Global Change, JAMSTEC, Yokohama, Japan</addr-line>
</aff>
<aff id="aff11">
<label>11</label>
<addr-line>Royal Netherlands Meteorological Institute (KNMI), Atmospheric Composition Research, De Bilt, the Netherlands</addr-line>
</aff>
<aff id="aff12">
<label>12</label>
<addr-line>now at: University of Cambridge, Centre for Atmospheric Science, Cambridge, UK</addr-line>
</aff>
<pub-date pub-type="epub">
<day>12</day>
<month>09</month>
<year>2006</year>
</pub-date>
<volume>6</volume>
<issue>5</issue>
<fpage>8553</fpage>
<lpage>8604</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/6/8553/2006/acpd-6-8553-2006.html">This article is available from http://www.atmos-chem-phys-discuss.net/6/8553/2006/acpd-6-8553-2006.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/6/8553/2006/acpd-6-8553-2006.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/6/8553/2006/acpd-6-8553-2006.pdf</self-uri>
<abstract>
<p>The global impact of shipping on atmospheric chemistry and radiative
forcing, as well as the associated uncertainties, have been quantified using
an ensemble of ten state-of-the-art atmospheric chemistry models and a
pre-defined set of emission data. The analysis is performed for present-day
conditions (year 2000) and for two future ship emission scenarios. In one
scenario emissions stabilize at 2000 levels; in the other emissions increase
with a constant annual growth rate of 2.2% up to 2030 (termed the
&quot;Constant Growth Scenario&apos;&apos;). The first key question addressed by this study
is how NO&lt;sub&gt;x&lt;/sub&gt; and SO&lt;sub&gt;2&lt;/sub&gt; emissions from international shipping might
influence atmospheric chemistry in the next three decades if these emissions
increase unabated. The models show future increases in NO&lt;sub&gt;x&lt;/sub&gt; and ozone
burden which scale almost linearly with increases in NO&lt;sub&gt;x&lt;/sub&gt; emission
totals. For the same ship emission totals but higher emissions from other
sources a slightly smaller response is found. The most pronounced changes in
annual mean tropospheric NO&lt;sub&gt;2&lt;/sub&gt; and sulphate columns are simulated over
the Baltic and North Seas; other significant changes occur over the North
Atlantic, the Gulf of Mexico and along the main shipping lane from Europe to
Asia, across the Red and Arabian Seas. Maximum contributions from shipping
to annual mean near-surface ozone are found over the Atlantic (5&amp;ndash;6 ppbv in
2000 reaching up to 8ppbv in the 2030 Constant Growth Scenario). Large
increases in tropospheric ozone column are found over the Atlantic and even
stronger over the Indian Ocean (1 DU in 2000 and up to 1.8 DU in 2030).
Tropospheric ozone forcings due to shipping are 9.8&amp;plusmn;2.0 mW/m&lt;sup&gt;2&lt;/sup&gt; in
2000 and 13.6&amp;plusmn;2.3 mW/m&lt;sup&gt;2&lt;/sup&gt; in 2030. Whilst increasing ozone, ship
NO&lt;sub&gt;x&lt;/sub&gt; simultaneously enhances OH, reducing the CH&lt;sub&gt;4&lt;/sub&gt; lifetime by 0.13 yr in 2000, and by up to 0.17 yr in 2030, introducing a negative radiative
forcing. Over Europe, the increase in ship emissions under the &quot;Constant
Growth Scenario&apos;&apos; will enhance the positive trend in NO&lt;sub&gt;2&lt;/sub&gt; over land up to
2030. In addition, efforts to lower European sulphate levels through
reductions in SO&lt;sub&gt;2&lt;/sub&gt; emissions from anthropogenic sources on land will be
partly counteracted by the rise in ship emissions. Globally, shipping
contributes with 3% to increases in ozone burden until 2030 and with
4.5% to increases in sulphate. The results discussed above are calculated
under the assumption that all other emissions follow the IPCC SRES A2
scenario. However, if future ground based emissions follow a more stringent
scenario, the relative importance of ship emissions becomes larger. The
second key issue of this work is to examine the range of results given by
the individual models compared to the ensemble mean. Uncertainties in the
different model approaches in the simulated ozone contributions from ships
are found to be significantly smaller than estimated uncertainties stemming
from the ship emission inventory, mainly the ship emission totals, the
neglect of ship plume dispersion, and the distribution of the emissions over
the globe.</p>
</abstract>
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</article-meta>
</front>
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