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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-5-1829-2005</article-id>
<title-group>
<article-title>Supersaturation, dehydration, and denitrification in Arctic cirrus</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kärcher</surname>
<given-names>B.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Deutsches Zentrum f &amp;uuml;r Luft- und Raumfahrt (DLR), Institut f&amp;uuml;r Physik der Atmosph&amp;auml;re (IPA), Oberpfaffenhofen, Germany</addr-line>
</aff>
<pub-date pub-type="epub">
<day>22</day>
<month>03</month>
<year>2005</year>
</pub-date>
<volume>5</volume>
<issue>2</issue>
<fpage>1829</fpage>
<lpage>1861</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/5/1829/2005/acpd-5-1829-2005.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/5/1829/2005/acpd-5-1829-2005.pdf</self-uri>
<abstract>
<p>A polar cirrus case study is discussed with the help of a one-dimensional model with
explicit aerosol and ice microphysics. It is demonstrated that continuous cooling of air
in regions with small amounts of ice and slow ice deposition rates of water vapor drives
5 significant in-cloud supersaturations over ice, with potentially important consequences
for heterogeneous halogen activation. Radiatively important cloud properties such as
ice crystal size distributions are investigated, showing the presence of high number
concentrations of small crystals in the cloud top region at the tropopause, broad but
highly variable size spectra in the cloud interior, and mostly large crystals at the cloud
10 base. It is found that long-lived and vertically extended Arctic cirrostratus are highly
efficient at dehydrating the upper troposphere. Estimating nitric acid uptake in cirrus
clouds with an unprecedented treatment of diffusional burial in growing ice crystals
suggests that such clouds could also denitrify upper tropospheric air masses efficiently,
but a closer comparison to observations is needed to draw a definite conclusion on this
15 point. It is also shown that low temperatures, high relative humidities, and the absence
of ice above but close to the cloud top region cause efficient uptake of nitric acid in
background aerosol particles.</p>
</abstract>
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</article-meta>
</front>
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