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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-4-991-2004</article-id>
<title-group>
<article-title>Tropospheric ozone budget: regional and global calculations</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>O’Connor</surname>
<given-names>F. M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Law</surname>
<given-names>K. S.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Pyle</surname>
<given-names>J. A.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Barjat</surname>
<given-names>H.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Brough</surname>
<given-names>N.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dewey</surname>
<given-names>K.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Green</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kent</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Phillips</surname>
<given-names>G.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
<xref ref-type="aff" rid="aff8">
<sup>8</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>NCAS-Atmospheric Chemistry Modelling Support Unit, Centre for Atmospheric Science, University of Cambridge, United Kingdom</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Centre for Atmospheric Science, University of Cambridge, United Kingdom</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Met. Research Flight, United Kingdom</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>School of Environmental Sciences, University of East Anglia, United Kingdom</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>Department of Chemistry, University of Leicester, United Kingdom</addr-line>
</aff>
<aff id="aff6">
<label>6</label>
<addr-line>Now at Service d’A&amp;#x00E9;ronomie/IPSL, Paris, France</addr-line>
</aff>
<aff id="aff7">
<label>7</label>
<addr-line>Now at Centre for Atmospheric Science, University of Cambridge, United Kingdom</addr-line>
</aff>
<aff id="aff8">
<label>8</label>
<addr-line>Now at Geophysical Institute, University of Alaska Fairbanks, USA</addr-line>
</aff>
<pub-date pub-type="epub">
<day>11</day>
<month>02</month>
<year>2004</year>
</pub-date>
<volume>4</volume>
<issue>1</issue>
<fpage>991</fpage>
<lpage>1036</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/4/991/2004/acpd-4-991-2004.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/4/991/2004/acpd-4-991-2004.pdf</self-uri>
<abstract>
<p>Results from a tropospheric three-dimensional chemical transport model (TOMCAT) have been used
      to examine the terms of the ozone budget, both regionally and globally. The global calculations
      are discussed in light of other published estimates. Regional budgets are calculated
      for continental regions, including the American Mid-West, Sahara, and central Europe. These are
      compared with regional budgets for oceanic regions, including the Azores High and the Tropical
      Pacific Warm Pool. Furthermore, the coastal region of the UK and Ireland is also considered. The
      validity of these regional budgets from TOMCAT are discussed by comparing TOMCAT with measurements
      from a number of aircraft campaigns. The budgets for central Europe and the American Mid-West
      indicate that continental regions dominate the ozone budget of the northern extratropics. This is
      in spite of the remote oceanic regions being photochemical sinks for ozone. The regional budget
      calculations for the UK and Ireland exhibit net photochemical production of ozone in the boundary
      layer but this is not consistent with available aircraft measurements. This is attributed to the
      coarse horizontal resolution of the TOMCAT model which results in the model&apos;s photochemical budget
      being more typical of a polluted continental region than a relatively remote one. On the other hand,
      the ozone photochemical rates calculated for the Azores High and the Tropical Pacific Warm Pool
      agree rather well with other estimates.</p>
</abstract>
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</front>
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