Atmos. Chem. Phys. Discuss., 4, 5831-5854, 2004
www.atmos-chem-phys-discuss.net/4/5831/2004/
doi:10.5194/acpd-4-5831-2004
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Fluorescence from atmospheric aerosol detected by a lidar indicates biogenic particles in the stratosphere
F. Immler1, D. Engelbart2, and O. Schrems1
1Alfred Wegener Institute for Polar and Marine Research, Am Handelshafen 12, 27570 Bremerhaven, Germany
2German Weather Service, Meteorological Observatory Lindenberg, Am Observatorium 12, 15848 Lindenberg, Germany

Abstract. With a lidar system that was installed in Lindenberg/Germany, we observed in June 2003, an extended aerosol layer at 13 km altitude in the lowermost stratosphere. This layer created an inelastic backscatter signal which we interpret as laser induced fluorescence from aerosol particles. Also, we find evidence for inelastic scattering in a smoke plume from a forest fire that we observed in the troposphere. Fluorescence from ambient aerosol had not yet been considered detectable by lidar. However, organic compounds such as polycyclic aromatic hydrocarbons sticking to the aerosol particles, or bioaerosol such as bacteria, spores or pollen fluoresce when excited with UV-radiation in a way that is detectable by our lidar system. Therefore, we conclude that fluorescence from organic material released by biomass burning creates the inelastic backscatter signal that we measured with our instrument and thus demonstrate a new and powerful way to characterize aerosols by a remote sensing technique. The stratospheric aerosol layer that we have observed in Lindenberg for three consecutive days is likely to be a remnant from Siberian forest fire plumes lifted across the tropopause and transported around the globe.

Citation: Immler, F., Engelbart, D., and Schrems, O.: Fluorescence from atmospheric aerosol detected by a lidar indicates biogenic particles in the stratosphere, Atmos. Chem. Phys. Discuss., 4, 5831-5854, doi:10.5194/acpd-4-5831-2004, 2004.
 
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