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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-4-327-2004</article-id>
<title-group>
<article-title>Technical Note: A diagnostic for ozone contributions of various NO&lt;sub&gt;x&lt;/sub&gt; emissions in multi-decadal chemistry-climate model simulations</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Grewe</surname>
<given-names>V.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Institut für Physik der Atmosphäre, DLR-Oberpfaffenhofen, Wessling, Germany</addr-line>
</aff>
<pub-date pub-type="epub">
<day>19</day>
<month>01</month>
<year>2004</year>
</pub-date>
<volume>4</volume>
<issue>1</issue>
<fpage>327</fpage>
<lpage>342</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<abstract>
<p>Nitrogen oxide
      (NO&lt;sub&gt;x&lt;/sub&gt;=NO+NO&lt;sub&gt;2&lt;/sub&gt;) emissions from various sources contribute to the ozone budget. The identification of these
      contributions is important, e.g.&amp;nbsp; for the assessment of emissions from traffic. The non-linear character of ozone
      chemistry complicates the online diagnosis during multi-decadal chemistry-climate simulations. A methodology
      is suggested, which is efficient enough to be incorporated in multi-decadal simulations. Eight types of
      NO&lt;sub&gt;x&lt;/sub&gt; emissions
      are included in the model. For each a NO&lt;sub&gt;y&lt;/sub&gt; (=all N components, except
      N&lt;sub&gt;2&lt;/sub&gt; and
      N&lt;sub&gt;2&lt;/sub&gt;O)
      tracer and an ozone tracer is included in the model, which experience the same emissions and
      loss processes like the online chemistry fields. To calculate the ozone changes caused by an individual
      NO&lt;sub&gt;x&lt;/sub&gt; emission,
      the assumption is made that the NO&lt;sub&gt;x&lt;/sub&gt; contributions from various sources
      are identical to the NO&lt;sub&gt;y&lt;/sub&gt; contributions. To evaluate
      this method each NO&lt;sub&gt;x&lt;/sub&gt; emission
      has been increased by 5% and a detailed error analysis is given. In the regions of the
      main impact of individual sources the potential error of the calculated contribution
      is significantly smaller than the contribution. Moreover, the changes caused by an increase of the
      emissions of 5% were detected with a higher accuracy than the potential errror of the absolut contribution.</p>
</abstract>
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