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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-4-2089-2004</article-id>
<title-group>
<article-title>A parameterisation of the soot aging for global climate models</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Riemer</surname>
<given-names>N.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Vogel</surname>
<given-names>H.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Vogel</surname>
<given-names>B.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Department of Mechanical and Aeronautical Engineering, University of California, Davis, USA</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Institut für Meteorologie und Klimaforschung, Forschungszentrum Karlsruhe, Karlsruhe, Germany</addr-line>
</aff>
<pub-date pub-type="epub">
<day>16</day>
<month>04</month>
<year>2004</year>
</pub-date>
<volume>4</volume>
<issue>2</issue>
<fpage>2089</fpage>
<lpage>2115</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/4/2089/2004/acpd-4-2089-2004.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/4/2089/2004/acpd-4-2089-2004.pdf</self-uri>
<abstract>
<p>The representation of soot in global climate models is desirable since it
contributes to both the direct and indirect climate effect. While freshly
emitted soot is initially hydrophobic and externally mixed, it can be
transferred into an internal mixture by coagulation, condensation or
photochemical processes. These aging processes affect the hygroscopic
qualities and hence the growth behaviour, the optical properties and
eventually the lifetime of the soot particles. However, due to computational
limits the aging of soot in global climate models is often only
parameterised by an estimated turnover rate resulting in a lifetime of soot
of several days. Based on the results of our simulations with a
comprehensive mesoscale model, we derive the timescale on which diesel soot
is transferred from an external to internal mixture, and propose a
parameterisation for the use in global climate models. This parameterisation
is applicable to continental conditions in industrialised areas as can be
found in Central Europe and North America. For daytime conditions, away from
the sources, condensation is dominant and the aging process occurs very fast
with a timescale of &amp;tau;=2 h. During night time condensation is not
effective. Then coagulation is the most important aging process and our
parameterisation leads to a timescale between 10 h and 40 h.</p>
</abstract>
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</front>
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