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<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-3-5777-2003</article-id>
<title-group>
<article-title>Problems regarding the tropospheric O&lt;sub&gt;3&lt;/sub&gt; residual method and its interpretation in Fishman et al. (2003)</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>de Laat</surname>
<given-names>A. D. J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Aben</surname>
<given-names>I.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>National Institute for Space Research (SRON) Utrecht, The Netherlands</addr-line>
</aff>
<pub-date pub-type="epub">
<day>14</day>
<month>11</month>
<year>2003</year>
</pub-date>
<volume>3</volume>
<issue>6</issue>
<fpage>5777</fpage>
<lpage>5802</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/3/5777/2003/acpd-3-5777-2003.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/3/5777/2003/acpd-3-5777-2003.pdf</self-uri>
<abstract>
<p>In this article we will show that the Total Ozone Residuals (TOR) method as presented
      by Fishman et al. (2003) contains an erroneous assumption, due to which the TOR as
      presented in this article reflects mainly a tropospheric O&lt;sub&gt;3&lt;/sub&gt; climatology (Logan, 1999),
      scaled to the layer between the surface and the tropopause height, rather than a satellite
      measured TOR. We will show that it is possible to obtain a tropospheric O&lt;sub&gt;3&lt;/sub&gt;&amp;nbsp;
      column that is very similar to what is being presented in Fishman et al.
      (2003), solely based on the Logan (1999) tropospheric O&lt;sub&gt;3&lt;/sub&gt;&amp;nbsp; climatology and an estimate for the tropopause heights
      without using satellite data. Furthermore, we will show that one of the interpretations of
      observed O&lt;sub&gt;3&lt;/sub&gt;&amp;nbsp; variability (high TOR values over Southeast Asia) is not the result of
      pollution, but primarily of tropopause height variations. We suggest adjusting the method
      in such a way that the final retrieved TOR product becomes independent of the actual
      values of the Logan (1999) O&lt;sub&gt;3&lt;/sub&gt;&amp;nbsp; climatology. The proposed adjustments are also more in
      line with the original methodology suggested by Fishman and Balok (1999) in a previous
      paper. We furthermore show that the assumption that the stratospheric O&lt;sub&gt;3&lt;/sub&gt;&amp;nbsp;
      column is nearly constant within a 5-day period is not always valid. This can introduce errors in the
      final TOR product, although we recognize that these errors may become small when
      averaging the TOR product over longer periods of time.  However, we feel that a detailed
      study on this assumption is also needed.</p>
</abstract>
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