Atmos. Chem. Phys. Discuss., 3, 2465-2497, 2003
www.atmos-chem-phys-discuss.net/3/2465/2003/
doi:10.5194/acpd-3-2465-2003
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Trace gas transport in the 1999/2000 Arctic winter: comparison of nudged GCM runs with observations
M. K. van Aalst1, M. M. P. van den Broek2, A. Bregman3, C. Brühl4, B. Steil4, G. C. Toon5, S. Garcelon6, G. M. Hansford6, R. L. Jones6, T. D. Gardiner7, G. J. Roelofs1, J. Lelieveld4, and P. J. Crutzen4
1Institute for Marine and Atmospheric Research (IMAU), Utrecht, The Netherlands
2Space Research Organisation of the Netherlands (SRON), Utrecht, The Netherlands
3Royal Netherlands Meteorological Institute (KNMI), De Bilt, The Netherlands
4Max Planck Institut für Chemie (MPI), Mainz, Germany
5Jet Propulsion Laboratory (JPL), Pasadena, CA, USA
6Cambridge University, Cambridge, UK
7National Physical Laboratory (NPL), Teddington, UK

Abstract. We have compared satellite and balloon observations of methane (CH4) and hydrogen fluoride (HF) during the Arctic winter 1999/2000 with results from the MA-ECHAM4 middle atmospheric general circulation model (GCM). For this purpose, the meteorology in the model was nudged towards ECMWF analyses. This nudging technique is shown to work well for this middle atmospheric model, and offers good opportunities for the simulation of realistic chemistry and transport processes. The current study focuses on transport of HF and CH4, initialized with satellite measurements from the HALOE instrument aboard the UARS satellite. We have compared the model results with HALOE data and balloon measurements throughout the winter, and analyzed the uncertainties associated with tracer initialization, boundary conditions and the passive tracer assumption. This comparison shows that the model represents the Arctic vortex well, including relatively small-scale features. However, while profiles outside the vortex match well, the model underestimates HF and overestimates CH4 concentrations inside the vortex, particularly in the middle stratosphere. This problem is also evident in a comparison of vortex descent rates based upon vortex average tracer profiles from MA-ECHAM4, and various observations, respectively. This could be due to an underestimate of diabatic subsidence in the model, or due to too much mixing between vortex and non-vortex air.

Citation: van Aalst, M. K., van den Broek, M. M. P., Bregman, A., Brühl, C., Steil, B., Toon, G. C., Garcelon, S., Hansford, G. M., Jones, R. L., Gardiner, T. D., Roelofs, G. J., Lelieveld, J., and Crutzen, P. J.: Trace gas transport in the 1999/2000 Arctic winter: comparison of nudged GCM runs with observations, Atmos. Chem. Phys. Discuss., 3, 2465-2497, doi:10.5194/acpd-3-2465-2003, 2003.
 
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