Atmos. Chem. Phys. Discuss., 13, 18277-18306, 2013
© Author(s) 2013. This work is distributed
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Aerosol measurements at a high elevation site: composition, size, and cloud condensation nuclei activity
B. Friedman1, A. Zelenyuk2, J. Beránek2, G. Kulkarni2, M. Pekour2, A. G. Hallar3, I. B. McCubbin3, J. A. Thornton1, and D. J. Cziczo4
1Department of Atmospheric Sciences, University of Washington, Seattle, WA, USA
2Pacific Northwest National Laboratory, Richland, WA, USA
3Storm Peak Laboratory, Desert Research Institute, Steamboat Springs, CO, USA
4Earth, Atmospheric, and Planetary Sciences Department, Massachusetts Institute of Technology, Cambridge, MA, USA

Abstract. Measurements of cloud condensation nuclei (CCN) concentrations, single particle composition and size distributions at a high-elevation research site from March 2011 are presented.

The temporal evolution of detailed single particle composition is compared with changes in CCN activation on four days, two of which include new particle formation and growth events. Sulfate-containing particles dominated the single particle composition by number; biomass burning particles, sea salt particles, and particles containing organic components also were present. CCN activation largely followed the behavior of the sulfate-containing particle types; biomass burning particle types also likely contained hygroscopic material that impacted CCN activation. Newly formed particles also may contribute to CCN activation at higher supersaturation conditions. Derived aerosol hygroscopicity parameters from the size distribution and CCN concentration measurements are within the range of previous reports of remote continental kappa values.

Citation: Friedman, B., Zelenyuk, A., Beránek, J., Kulkarni, G., Pekour, M., Hallar, A. G., McCubbin, I. B., Thornton, J. A., and Cziczo, D. J.: Aerosol measurements at a high elevation site: composition, size, and cloud condensation nuclei activity, Atmos. Chem. Phys. Discuss., 13, 18277-18306, doi:10.5194/acpd-13-18277-2013, 2013.
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