Atmos. Chem. Phys. Discuss., 12, 441-478, 2012
www.atmos-chem-phys-discuss.net/12/441/2012/
doi:10.5194/acpd-12-441-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Transport of short-lived species into the Tropical Tropopause Layer
M. J. Ashfold1, N. R. P. Harris1, E. L. Atlas2, A. J. Manning3, and J. A. Pyle1,4
1Department of Chemistry, University of Cambridge, Cambridge, UK
2Rosenstiel School of Marine and Atmospheric Science, University of Miami, Miami, Florida, USA
3Met Office, Exeter, UK
4National Centre for Atmospheric Science, University of Cambridge, Cambridge, UK

Abstract. We use NAME, a trajectory model, to investigate the routes and timescales over which air parcels reach the tropical tropopause layer (TTL). Our aim is to assist the planning of aircraft campaigns focussed on improving knowledge of such transport. We investigate the conditions which might occur during one such campaign, SHIVA, which takes place in Borneo during November 2011. We first study the TTL above Borneo in November 2008, under neutral El Niño/Southern Oscillation (ENSO) conditions. Air parcels (trajectories) arriving in the lower TTL (below ~15 km) are most likely to have travelled from the boundary layer (BL; <1 km) above the West Pacific. Few air parcels found above ~16 km travelled from the BL in the previous 15 days. We then perform similar calculations for moderate El Niño (2006) and La Niña (2007) conditions and find year-to-year variability consistent with the phase of ENSO. Under El Niño conditions fewer air parcels travel from the BL to the TTL above Borneo. During the La Niña year, more air parcels travel from the BL to the mid and upper TTL (above ~15 km) than in the ENSO-neutral year, and again they do so from the BL above the West Pacific. We also find intra-month variability in all years, with day-to-day differences of up to an order of magnitude in the fraction of an idealised short-lived tracer travelling from the BL to the TTL above Borneo. Finally, we consider measurements made in two previous campaigns in order to validate our approach. The features of vertical profiles of short-lived species observed in the TTL during CR-AVE and TC4 are in broad agreement with calculated vertical profiles of idealised short-lived tracers. It will require large numbers of observations to fully describe the statistical distribution of short-lived species in the TTL. This modelling approach should prove valuable in planning flights for the long-duration aircraft capable of making such measurements.

Citation: Ashfold, M. J., Harris, N. R. P., Atlas, E. L., Manning, A. J., and Pyle, J. A.: Transport of short-lived species into the Tropical Tropopause Layer, Atmos. Chem. Phys. Discuss., 12, 441-478, doi:10.5194/acpd-12-441-2012, 2012.
 
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