Atmos. Chem. Phys. Discuss., 12, 32883-32909, 2012
www.atmos-chem-phys-discuss.net/12/32883/2012/
doi:10.5194/acpd-12-32883-2012
© Author(s) 2012. This work is distributed
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Quantitative evaluation of emission control of primary and secondary organic aerosol sources during Beijing 2008 Olympics
S. Guo1,2, M. Hu1, Q. Guo1, X. Zhang1, J. J. Schauer3, and R. Zhang1,2
1State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing, 100871, China
2Department of Atmospheric Science, Texas A&M University, College Station, Texas 77843, USA
3Environmental Chemistry and Technology Program, Wisconsin State Laboratory of Hygiene, University of Wisconsin-Madison, Madison, WI 53706, USA

Abstract. To explore the primary and secondary sources of fine organic particles after the aggressive implementation of air pollution controls during 2008 Beijing Olympic Games, 12-h PM2.5 concentrations were measured at one urban and one upwind rural site during the CAREBeijing-2008 (Campaigns of Air quality REsearch in Beijing and surrounding region) summer field campaign. The PM2.5 concentrations were 72.5±43.6μg m3 and 64.3±36.2μg m−3 at the urban site and rural site, respectively, which were the lowest in recent years due to the implementation of drastic control measures and favorable weather conditions. Five primary and four secondary fine organic particle sources were quantified using a CMB (chemical mass balance) model and tracer-yield method. Compared with previous studies in Beijing, the contribution of vehicle emission increased, with diesel engines contributing 16.2±5.9% and 14.5±4.1% to the total organic carbon (OC) concentrations and gasoline vehicles accounting for 10.3±8.7% and 7.9±6.2% of the OC concentrations at two sites. Due to the implementation of emission control measures, the OC concentrations from important primary sources have been reduced, and secondary formation has become an important contributor to fine organic aerosols. Compared with the non-controlled period, primary vehicle contributions were reduced by 30% and 24% in the urban and regional area, and reductions in the contribution from coal combustion were 57% and 7%, respectively. These results demonstrate the emission control measures significantly alleviated the primary organic particle pollution in and around Beijing. However, the control effectiveness of secondary organic particles was not significant.

Citation: Guo, S., Hu, M., Guo, Q., Zhang, X., Schauer, J. J., and Zhang, R.: Quantitative evaluation of emission control of primary and secondary organic aerosol sources during Beijing 2008 Olympics, Atmos. Chem. Phys. Discuss., 12, 32883-32909, doi:10.5194/acpd-12-32883-2012, 2012.
 
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