Atmos. Chem. Phys. Discuss., 12, 25703-25741, 2012
www.atmos-chem-phys-discuss.net/12/25703/2012/
doi:10.5194/acpd-12-25703-2012
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under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Decadal record of satellite carbon monoxide observations
H. M. Worden1, M. N. Deeter1, C. Frankenberg2, M. George3, F. Nichitiu4, J. Worden2, I. Aben5, K. W. Bowman2, C. Clerbaux3,6, P. F. Coheur6, A. T. J. de Laat5,7, R. Detweiler1, J. R. Drummond8, D. P. Edwards1, J. C. Gille1, D. Hurtmans6, M. Luo2, S. Martínez-Alonso1, S. Massie1, G. Pfister1, and J. X. Warner9
1National Center for Atmospheric Research (NCAR), Boulder, CO, USA
2Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA, USA
3UPMC Univ. Paris 06; Université Versailles St-Quentin; CNRS/INSU, LATMOS-IPSL, Paris, France
4Dept. of Physics and Atmospheric Science, University of Toronto, Toronto, Ontario, Canada
5SRON Netherlands Institute for Space Research, Utrecht, The Netherlands
6Spectroscopie de l'Atmosphère, Service de Chimie Quantique et Photophysique, Libre Université de Bruxelles (ULB), Brussels, Belgium
7Royal Netherlands Meteorological Institute (KNMI), De Bilt, The Netherlands
8Dept. of Physics and Atmospheric Science, Dalhousie University, Halifax, Nova Scotia, Canada
9Dept. of Atmospheric and Oceanic Science, Univ. of Maryland, College Park, MD, USA

Abstract. Atmospheric carbon monoxide (CO) distributions are controlled by anthropogenic emissions, biomass burning, transport and oxidation by reaction with the hydroxyl radical (OH). Quantifying trends in CO is therefore important for understanding changes related to all of these contributions. Here we present a comprehensive record of satellite observations from 2000 through 2011 of total column CO using the available measurements from nadir-viewing thermal infrared instruments: MOPITT, AIRS, TES and IASI. We examine trends for CO in the Northern and Southern Hemispheres along with regional trends for Eastern China, Eastern USA, Europe and India. We find that all the satellite observations are consistent with a modest decreasing trend ∼−1% yr−1 in total column CO over the Northern Hemisphere for this time period and a less significant, but still decreasing trend in the Southern Hemisphere. Although decreasing trends in the United States and Europe have been observed from surface CO measurements, we also find a decrease in CO over E. China that, to our knowledge, has not been reported previously. Some of the interannual variability in the observations can be explained by global fire emissions, but the overall decrease needs further study to understand the implications for changes in anthropogenic emissions.

Citation: Worden, H. M., Deeter, M. N., Frankenberg, C., George, M., Nichitiu, F., Worden, J., Aben, I., Bowman, K. W., Clerbaux, C., Coheur, P. F., de Laat, A. T. J., Detweiler, R., Drummond, J. R., Edwards, D. P., Gille, J. C., Hurtmans, D., Luo, M., Martínez-Alonso, S., Massie, S., Pfister, G., and Warner, J. X.: Decadal record of satellite carbon monoxide observations, Atmos. Chem. Phys. Discuss., 12, 25703-25741, doi:10.5194/acpd-12-25703-2012, 2012.
 
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