Atmos. Chem. Phys. Discuss., 12, 24985-25036, 2012
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The effects of recent control policies on trends in emissions of anthropogenic atmospheric pollutants and CO2 in China
Y. Zhao1, J. Zhang2, and C. P. Nielsen3
1State Key Laboratory of Pollution Control and Resource Reuse and School of the Environment, Nanjing University, 163 Xianlin Ave., Nanjing, Jiangsu 210046, China
2Jiangsu Provincial Academy of Environmental Science, 241 West Fenghuang St., Nanjing, Jiangsu 210036, China
3Harvard China Project, School of Engineering and Applied Sciences, Harvard University, 29 Oxford St, Cambridge, MA 02138, USA

Abstract. To examine the effects of China's national policies of energy conservation and emission control during 2005–2010, inter-annual emission trends of gaseous pollutants, primary aerosols, and CO2 are estimated with a bottom-up framework. The control measures led to improved energy efficiency and/or increased penetration of emission control devices at power plants and other important industrial sources, yielding reduced emission factors for all evaluated species except NOx. The national emissions of anthropogenic SO2, CO, and total primary PM (particulate matter) in 2010 are estimated to have been 89%, 108%, and 86% of those in 2005, respectively, suggesting successful emission control of those species despite fast growth of the economy and energy consumption during the period. The emissions of NOx and CO2, however, are estimated to have increased by 48% and 43%, respectively, indicating that they remain largely determined by the growth of energy use, industrial production, and vehicle populations. Based on application of a Monte-Carlo framework, estimated uncertainties of SO2 and PM emissions increased from 2005 to 2010, resulting mainly from weakly understood average SO2 removal efficiency in flue gas desulfurization (FGD) systems in the power sector, and unclear changes in the penetration levels of dust collectors at industrial sources, respectively. While emission trends determined by bottom-up methods can be generally verified by observations from both ground stations and satellites, clear discrepancies exist for given regions and seasons, indicating a need for more accurate spatial and time distributions of emissions. Limitations of current emission control polices are analyzed based on the estimated emission trends. Compared with control of total PM, there are fewer gains in control of fine particles and carbonaceous aerosols, the PM forms most responsible for damages to public health and effects on radiative forcing. A decrease of alkaline base cations as primary PM that is much faster than that of SO2 may have raised the acidification risks to ecosystems, indicating further control of acid precursors is required. Moreover, with relatively strict controls in developed urban areas, air pollution challenges have been expanding to less-developed neighboring regions. There is a great need in the future for multi-pollutant control strategies that combine recognition of diverse environmental impacts both in urban and rural areas with emission abatement of multiple species in concert.

Citation: Zhao, Y., Zhang, J., and Nielsen, C. P.: The effects of recent control policies on trends in emissions of anthropogenic atmospheric pollutants and CO2 in China, Atmos. Chem. Phys. Discuss., 12, 24985-25036, doi:10.5194/acpd-12-24985-2012, 2012.
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