Atmos. Chem. Phys. Discuss., 12, 18459-18497, 2012
www.atmos-chem-phys-discuss.net/12/18459/2012/
doi:10.5194/acpd-12-18459-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Regional and monthly and clear-sky aerosol direct radiative effect (and forcing) derived from the GlobAEROSOL-AATSR satellite aerosol product
G. E. Thomas1, N. Chalmers2, B. Harris2, R. G. Grainger1, and E. J. Highwood2
1Atmospheric, Oceanic and Planetary Physics, University of Oxford, Oxford, UK
2Department of Meteorology, University of Reading, Reading, UK

Abstract. Using the GlobAEROSOL-AATSR dataset, estimates of the instantaneous, clear-sky, direct aerosol radiative effect and radiative forcing have been produced for the year 2006. Aerosol Robotic Network sun-photometer measurements have been used to characterise the random and systematic error in the GlobAEROSOL product for 22 regions covering the globe. Representative aerosol properties for each region have been derived from the results of a wide range of literature sources and, along with the de-biased GlobAEROSOL AODs, were used to drive an offline version of the Met Office unified model radiation scheme. In addition to the mean AOD, best-estimate run of the radiation scheme, a range of additional calculations were done to propagate uncertainty estimates in the AOD, optical properties, surface albedo and errors due to the temporal and spatial averaging of the AOD fields. This analysis produced monthly, regional estimates of the clear-sky aerosol radiative effect and its uncertainty, which produce annual, global mean values of (−6.7 ± 3.9) W m−2 at the top of atmosphere (TOA) and (−12 ± 6) W m−2 at the surface. These results were then used to produce estimates of regional, clear-sky aerosol direct radiative forcing, using modelled pre-industrial AOD fields for 1750 calculated for the AEROCOM PRE experiment. However, as it was not possible to quantify the uncertainty in the pre-industrial aerosol loading, these figures can only be taken as indicative and their uncertainties as lower bounds on the likely errors. Although the uncertainty on aerosol radiative effect presented here is considerably larger than most previous estimates, the explicit inclusion of the major sources of error in the calculations suggest that they are closer to the true constraint on this figure from similar methodologies, and point to the need for more, improved estimates of both global aerosol loading and aerosol optical properties.

Citation: Thomas, G. E., Chalmers, N., Harris, B., Grainger, R. G., and Highwood, E. J.: Regional and monthly and clear-sky aerosol direct radiative effect (and forcing) derived from the GlobAEROSOL-AATSR satellite aerosol product, Atmos. Chem. Phys. Discuss., 12, 18459-18497, doi:10.5194/acpd-12-18459-2012, 2012.
 
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