Atmos. Chem. Phys. Discuss., 12, 17835-17886, 2012
www.atmos-chem-phys-discuss.net/12/17835/2012/
doi:10.5194/acpd-12-17835-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Dust emission size distribution impact on aerosol budget and radiative forcing over the Mediterranean region: a regional climate model approach
P. Nabat1, F. Solmon2, M. Mallet3, J. F. Kok4, and S. Somot1
1Météo-France, Centre National de Recherches Météorologiques, CNRM-GAME, URA1357, 42 avenue G. Coriolis, 31057 Toulouse cedex 1, France
2The Abdus Salam International Center for Theroretical Physics, Strada Costiera 11, 34100 Trieste, Italy
3Laboratoire d'Aérologie, 16 avenue Édouard Belin, 31400 Toulouse, France
4Advanced Study Program, National Center for Atmospheric Research, Boulder, CO, USA

Abstract. The present study investigates the dust emission and load over the Mediterranean basin using the coupled-chemistry-aerosol regional climate model RegCM-4. The first step of this work focuses on dust particle emission size distribution modeling. We compare a parameterization in which the emission is based on the individual kinetic energy of the aggregates striking the surface to a recent parameterization based on an analogy with the fragmentation of brittle materials. The main difference between the two dust schemes concerns the mass proportion of fine aerosol which is reduced in the case of the new dust parameterization, with consequences for optical properties. At the episodic scale, comparisons between RegCM-4 simulations, satellite and ground-based data show a clear improvement using the new dust distribution in terms of Aerosol Optical Depth (AOD) values and geographic gradients. These results are confirmed at the seasonal scale for the investigated year 2008. A multi-annual simulation is finally carried out using the new dust distribution over the period 2000–2009. This change of dust distribution has sensitive impacts on the simulated regional dust budget, notably dry dust deposition and the regional direct aerosol radiative forcing over the Mediterranean basin. This could clearly modify the possible effects of dust aerosols on the biogeochemical activity and climate of the Mediterranean basin. In particular, we find that the new size distribution produces a higher dust deposition flux, and smaller top of atmosphere (TOA) dust radiative cooling.

Citation: Nabat, P., Solmon, F., Mallet, M., Kok, J. F., and Somot, S.: Dust emission size distribution impact on aerosol budget and radiative forcing over the Mediterranean region: a regional climate model approach, Atmos. Chem. Phys. Discuss., 12, 17835-17886, doi:10.5194/acpd-12-17835-2012, 2012.
 
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