Atmos. Chem. Phys. Discuss., 12, 1687-1732, 2012
www.atmos-chem-phys-discuss.net/12/1687/2012/
doi:10.5194/acpd-12-1687-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Strong sensitivity of aerosol concentrations to convective wet scavenging parameterizations in a global model
B. Croft1, J. R. Pierce1, R. V. Martin1,2, C. Hoose3, and U. Lohmann4
1Department of Physics and Atmospheric Science, Dalhousie University, Halifax, Canada
2Harvard-Smithsonian Center for Astrophysics, Cambridge, MA, USA
3Karlsruhe Institute of Technology, Karlsruhe, Germany
4Institute of Atmospheric and Climate Science, ETH Zurich, Zurich, Switzerland

Abstract. This study examines the influences of assumptions in convective wet scavenging parameterizations on global climate model simulations of aerosol concentrations and wet deposition. To facilitate this study, an explicit representation of the uptake of aerosol mass and number into convective cloud droplets and ice crystals by the processes of activation, collisions, freezing and evaporation is introduced into the ECHAM5-HAM model. This development replaces the prescribed aerosol cloud-droplet-borne/ice-crystal-borne fractions of the standard model. Relative to the standard model, the more consistent treatment between convective aerosol-cloud microphysical processes yields a reduction of aerosol wet removal in mixed liquid and ice phase convective clouds by at least a factor of two, and the global, annual mean aerosol burdens are increased by at least 20%. Two limiting cases regarding the wet scavenging of entrained aerosols are considered. In the first case, aerosols entering convective clouds at their bases are the only aerosols that are scavenged into cloud droplets, and are susceptible to removal by convective precipitation formation. In the second case, aerosols that are entrained into the cloud above the cloud base layer can activate, can collide with existing cloud droplets and ice crystals, and can subsequently be removed by precipitation formation. The limiting case that allows aerosols entrained above cloud base to become cloud-droplet-borne and ice-crystal-borne reduces the annual and global mean aerosol burdens by 30% relative to the other limiting case, and yields the closest agreement with global aerosol optical depth retrievals, and black carbon vertical profiles from aircraft campaigns (changes of about one order of magntiude in the upper troposphere). Predicted convective cloud droplet number concentrations are doubled in the tropical middle troposphere when aerosols entrained above cloud base are allowed to activate. These results show that aerosol concentrations and wet deposition predicted in a global model are strongly sensitive to the assumptions made regarding the wet scavenging of aerosols in convective clouds.

Citation: Croft, B., Pierce, J. R., Martin, R. V., Hoose, C., and Lohmann, U.: Strong sensitivity of aerosol concentrations to convective wet scavenging parameterizations in a global model, Atmos. Chem. Phys. Discuss., 12, 1687-1732, doi:10.5194/acpd-12-1687-2012, 2012.
 
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