Atmos. Chem. Phys. Discuss., 12, 15453-15502, 2012
www.atmos-chem-phys-discuss.net/12/15453/2012/
doi:10.5194/acpd-12-15453-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Influence of particle size and shape on the backscattering linear depolarisation ratio of small ice crystals – cloud chamber measurements in the context of contrail and cirrus microphysics
M. Schnaiter, S. Büttner, O. Möhler, J. Skrotzki, M. Vragel, and R. Wagner
Karlsruhe Institute of Technology, Institute for Meteorology and Climate Research, P.O. Box 3640, 76021 Karlsruhe, Germany

Abstract. The article presents the laser scattering and depolarisation instrument SIMONE that is installed at the large aerosol and cloud chamber facility AIDA of the Karlsruhe Institute of Technology. SIMONE uses a 488 nm cw laser to probe simulated atmospheric clouds by measuring the scattered light from the 1.8° and 178.2° directions. At 178.2°, the scattered light is analysed for the linear polarisation state to deduce the linear depolarisation ratio δl which is a common measurement parameter of atmospheric LIDAR applications. The optical setup and the mathematical formalism of the depolarisation detection concept are given. SIMONE depolarisation measurements in spheroidal hematite aerosol and supercooled liquid clouds are used to validate the instrument.

SIMONE data from a series of AIDA ice nucleation experiments at temperatures between 195 and 225 K were analysed in terms of the impact of the ice particle microphysics on δl. We found strong depolarisation values of up to 0.4 in case of small growing and sublimating ice particles with volume equivalent diameters of only a few micrometers.

Modelling runs with the T-matrix method showed that the measured depolarisation ratios can be accurately reproduced assuming spheroidal and cylindrical particles with a size distribution that has been constrained by IR extinction spectroscopy. Based on the T-matrix modelling runs, we demonstrate that in case of small ice crystals the SIMONE depolarisation results are representative for the LIDAR depolarisation ratio which is measured at exact backscattering direction of 180°.

The relevance of our results for the interpretation of recent LIDAR observations in cirrus and contrails is discussed. In view of our results, the high depolarisation ratios observed by the spaceborne LIDAR CALIOP in the tropical upper troposphere might be a hint for the presence of small (sublimating) ice particles in the outflows of deep convective systems.


Citation: Schnaiter, M., Büttner, S., Möhler, O., Skrotzki, J., Vragel, M., and Wagner, R.: Influence of particle size and shape on the backscattering linear depolarisation ratio of small ice crystals – cloud chamber measurements in the context of contrail and cirrus microphysics, Atmos. Chem. Phys. Discuss., 12, 15453-15502, doi:10.5194/acpd-12-15453-2012, 2012.
 
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