Atmos. Chem. Phys. Discuss., 12, 14927-14957, 2012
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Sensitivity of cirrus and mixed-phase clouds to the ice nuclei spectra in McRAS-AC: single column model simulations
R. Morales Betancourt1, D. Lee2,3, L. Oreopoulos3, Y. C. Sud3, D. Barahona4, and A. Nenes1,5
1School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, Georgia, USA
2USRA Goddard Earth Sciences Technology and Research, 10211 Wincopin Circle, Suite 500, Columbia, Maryland 21044, USA
3NASA Goddard Space Flight Center, NASA/GSFC, Greenbelt, Maryland 20771, USA
4NASA Goddard Space Flight Center, I.M. Systems Group, Maryland, USA
5School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, Atlanta, Georgia, USA

Abstract. The salient features of mixed-phase and ice clouds in a GCM cloud scheme are examined using the ice formation parameterizations of Liu and Penner (LP) and Barahona and Nenes (BN). The performance of LP and BN ice nucleation parameterizations were assessed in the GEOS-5 AGCM using the McRAS-AC cloud microphysics framework in single column mode. Four dimensional assimilated data from the intensive observation period of ARM TWP-ICE campaign was used to drive the fluxes and lateral forcing. Simulation experiments where established to test the impact of each parameterization in the resulting cloud fields. Three commonly used IN spectra were utilized in the BN parameterization to described the availability of IN for heterogeneous ice nucleation. The results show large similarities in the cirrus cloud regime between all the schemes tested, in which ice crystal concentrations were within a factor of 10 regardless of the parameterization used. In mixed-phase clouds there are some persistent differences in cloud particle number concentration and size, as well as in cloud fraction, ice water mixing ratio, and ice water path. Contact freezing in the simulated mixed-phase clouds contributed to transfer liquid to ice efficiently, so that on average, the clouds were fully glaciated at T~260 K, irrespective of the ice nucleation parameterization used. Comparison of simulated ice water path to available satellite derived observations were also performed, finding that all the schemes tested with the BN parameterization predicted average values of IWP within ±15% of the observations.

Citation: Morales Betancourt, R., Lee, D., Oreopoulos, L., Sud, Y. C., Barahona, D., and Nenes, A.: Sensitivity of cirrus and mixed-phase clouds to the ice nuclei spectra in McRAS-AC: single column model simulations, Atmos. Chem. Phys. Discuss., 12, 14927-14957, doi:10.5194/acpd-12-14927-2012, 2012.
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